Coherent multistep rovibrational excitation using intense midinfrared pulses
We experimentally demonstrate coherent multistep rovibrational excitation in gas-phase carbon dioxide using intense midinfrared laser pulses. Ultrafast pump-probe spectroscopy directly observes excited-state rovibrational lines up to V=11 state with rotational quantum numbers of J=0−40. The observed...
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| Main Authors: | , , |
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| Format: | Article |
| Language: | English |
| Published: |
American Physical Society
2024-12-01
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| Series: | Physical Review Research |
| Online Access: | http://doi.org/10.1103/PhysRevResearch.6.L042058 |
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