Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites

SO<sub>2</sub> fumigation treatment (commonly known as sulfur treatment, ST) is a key method in the postharvest preservation of imported and exported fresh longan fruits, effectively reducing pericarp browning and enhancing color. Nonetheless, distinctive aromas, often referred to as “su...

Full description

Saved in:
Bibliographic Details
Main Authors: Rob Md Mahfuzur, Dongmei Han, Jianhang Xu, Yuqiong Lin, Xiaomeng Guo, Tao Luo, Zhenxian Wu, Shilian Huang, Xinmin Lv, Junbin Wei
Format: Article
Language:English
Published: MDPI AG 2024-10-01
Series:Plants
Subjects:
Online Access:https://www.mdpi.com/2223-7747/13/21/3061
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846173277845716992
author Rob Md Mahfuzur
Dongmei Han
Jianhang Xu
Yuqiong Lin
Xiaomeng Guo
Tao Luo
Zhenxian Wu
Shilian Huang
Xinmin Lv
Junbin Wei
author_facet Rob Md Mahfuzur
Dongmei Han
Jianhang Xu
Yuqiong Lin
Xiaomeng Guo
Tao Luo
Zhenxian Wu
Shilian Huang
Xinmin Lv
Junbin Wei
author_sort Rob Md Mahfuzur
collection DOAJ
description SO<sub>2</sub> fumigation treatment (commonly known as sulfur treatment, ST) is a key method in the postharvest preservation of imported and exported fresh longan fruits, effectively reducing pericarp browning and enhancing color. Nonetheless, distinctive aromas, often referred to as “sulfur flavor”, may develop in the aril during the extended preservation period. This study employed “Caopu” longan as the test material and patented SO<sub>2</sub>-releasing paper (ZL201610227848.7) as a treatment to perform a 35-day low-temperature (5 °C) storage of the fruit. The changes in glucosinolates (GSLs) and associated metabolites in the aril of treated fruit (ST) were examined utilizing ultra-high-performance liquid chromatography-tandem mass spectrometry (UPLC-MS/MS) detection and widely targeted metabolomics technology. The findings indicated that following 35 days of storage, nearly all control (CK) fruit pericarp turned to brown, resulting in an edible fruit rate of 75.41% and a commercial fruit rate of 0%. In contrast, the treated (ST) fruit demonstrated an edible fruit rate and a commercial rate of 99.44%, while the pericarp color changed from dark yellow-brown to light earthy yellow. The sulfur-containing metabolites identified in longan fruit aril predominantly consist of amino acids and their derivatives (60.44%), followed by alkaloids (15.38%), nucleotides and their derivatives (1.10%), and other types (23.08%), which include GSLs. SO<sub>2</sub> treatment significantly reduced the content of oxidized glutathione in fruit aril but increased the content of GSLs and related amino acids and their derivatives. Via screening, 19 differential sulfur-containing metabolites were obtained between ST and CK, including 11 GSLs. The identified differential metabolites of GSLs were all increased, primarily comprising aliphatic GSLs, such as 1-hydroxymethyl glucosinolate, 2-Propenyl glucosinolate (Sinigrin), and 4-Methylsulfinylbutyl glucosinolate (Glucoraphanin). Pathway analysis showed that these differential metabolites were mainly involved in coenzyme factor synthesis, cysteine and methionine metabolism, and amino acid synthesis, among other pathways. To the best of our knowledge, this is the first study to reveal the causes of the special flavor of longan aril after SO<sub>2</sub> treatment, which is a great concern for longan consumers. Moreover, this study provides a scientific basis for exploring the reasons and mechanisms for the development of the sulfur flavor in the SO<sub>2</sub>-treated fruits during postharvest storage.
format Article
id doaj-art-eaa2dc66b83b44f7815b36a0f992d073
institution Kabale University
issn 2223-7747
language English
publishDate 2024-10-01
publisher MDPI AG
record_format Article
series Plants
spelling doaj-art-eaa2dc66b83b44f7815b36a0f992d0732024-11-08T14:39:30ZengMDPI AGPlants2223-77472024-10-011321306110.3390/plants13213061Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate MetabolitesRob Md Mahfuzur0Dongmei Han1Jianhang Xu2Yuqiong Lin3Xiaomeng Guo4Tao Luo5Zhenxian Wu6Shilian Huang7Xinmin Lv8Junbin Wei9College of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaInstitute of Fruit Tree Research, Guangdong Academy of Agricultural Sciences, Key Laboratory of South Subtropical Fruit Biology and Genetic Resources Utilization, Ministry of Agriculture and Rural Affairs, Guangdong Key Laboratory of Fruit Science and Technology Research, Guangzhou 510640, ChinaCollege of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaCollege of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaCollege of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaCollege of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaCollege of Horticulture, South China Agricultural University, Guangzhou 510642, ChinaInstitute of Fruit Tree Research, Guangdong Academy of Agricultural Sciences, Key Laboratory of South Subtropical Fruit Biology and Genetic Resources Utilization, Ministry of Agriculture and Rural Affairs, Guangdong Key Laboratory of Fruit Science and Technology Research, Guangzhou 510640, ChinaInstitute of Fruit Tree Research, Guangdong Academy of Agricultural Sciences, Key Laboratory of South Subtropical Fruit Biology and Genetic Resources Utilization, Ministry of Agriculture and Rural Affairs, Guangdong Key Laboratory of Fruit Science and Technology Research, Guangzhou 510640, ChinaInstitute of Fruit Tree Research, Guangdong Academy of Agricultural Sciences, Key Laboratory of South Subtropical Fruit Biology and Genetic Resources Utilization, Ministry of Agriculture and Rural Affairs, Guangdong Key Laboratory of Fruit Science and Technology Research, Guangzhou 510640, ChinaSO<sub>2</sub> fumigation treatment (commonly known as sulfur treatment, ST) is a key method in the postharvest preservation of imported and exported fresh longan fruits, effectively reducing pericarp browning and enhancing color. Nonetheless, distinctive aromas, often referred to as “sulfur flavor”, may develop in the aril during the extended preservation period. This study employed “Caopu” longan as the test material and patented SO<sub>2</sub>-releasing paper (ZL201610227848.7) as a treatment to perform a 35-day low-temperature (5 °C) storage of the fruit. The changes in glucosinolates (GSLs) and associated metabolites in the aril of treated fruit (ST) were examined utilizing ultra-high-performance liquid chromatography-tandem mass spectrometry (UPLC-MS/MS) detection and widely targeted metabolomics technology. The findings indicated that following 35 days of storage, nearly all control (CK) fruit pericarp turned to brown, resulting in an edible fruit rate of 75.41% and a commercial fruit rate of 0%. In contrast, the treated (ST) fruit demonstrated an edible fruit rate and a commercial rate of 99.44%, while the pericarp color changed from dark yellow-brown to light earthy yellow. The sulfur-containing metabolites identified in longan fruit aril predominantly consist of amino acids and their derivatives (60.44%), followed by alkaloids (15.38%), nucleotides and their derivatives (1.10%), and other types (23.08%), which include GSLs. SO<sub>2</sub> treatment significantly reduced the content of oxidized glutathione in fruit aril but increased the content of GSLs and related amino acids and their derivatives. Via screening, 19 differential sulfur-containing metabolites were obtained between ST and CK, including 11 GSLs. The identified differential metabolites of GSLs were all increased, primarily comprising aliphatic GSLs, such as 1-hydroxymethyl glucosinolate, 2-Propenyl glucosinolate (Sinigrin), and 4-Methylsulfinylbutyl glucosinolate (Glucoraphanin). Pathway analysis showed that these differential metabolites were mainly involved in coenzyme factor synthesis, cysteine and methionine metabolism, and amino acid synthesis, among other pathways. To the best of our knowledge, this is the first study to reveal the causes of the special flavor of longan aril after SO<sub>2</sub> treatment, which is a great concern for longan consumers. Moreover, this study provides a scientific basis for exploring the reasons and mechanisms for the development of the sulfur flavor in the SO<sub>2</sub>-treated fruits during postharvest storage.https://www.mdpi.com/2223-7747/13/21/3061longansulfur dioxidepostharvest storagesulfur flavormetabolic profileglucosinolates
spellingShingle Rob Md Mahfuzur
Dongmei Han
Jianhang Xu
Yuqiong Lin
Xiaomeng Guo
Tao Luo
Zhenxian Wu
Shilian Huang
Xinmin Lv
Junbin Wei
Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
Plants
longan
sulfur dioxide
postharvest storage
sulfur flavor
metabolic profile
glucosinolates
title Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
title_full Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
title_fullStr Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
title_full_unstemmed Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
title_short Effects of Postharvest SO<sub>2</sub> Treatment on Longan Aril Flavor and Glucosinolate Metabolites
title_sort effects of postharvest so sub 2 sub treatment on longan aril flavor and glucosinolate metabolites
topic longan
sulfur dioxide
postharvest storage
sulfur flavor
metabolic profile
glucosinolates
url https://www.mdpi.com/2223-7747/13/21/3061
work_keys_str_mv AT robmdmahfuzur effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT dongmeihan effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT jianhangxu effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT yuqionglin effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT xiaomengguo effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT taoluo effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT zhenxianwu effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT shilianhuang effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT xinminlv effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites
AT junbinwei effectsofpostharvestsosub2subtreatmentonlonganarilflavorandglucosinolatemetabolites