Hydrogen radical-boosted electrocatalytic CO2 reduction using Ni-partnered heteroatomic pairs

Abstract The electrocatalytic reduction of CO2 to CO is slowed by the energy cost of the hydrogenation step that yields adsorbed *COOH intermediate. Here, we report a hydrogen radical (H•)-transfer mechanism that aids this hydrogenation step, enabled by constructing Ni-partnered hetero-diatomic pair...

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Bibliographic Details
Main Authors: Zhibo Yao, Hao Cheng, Yifei Xu, Xinyu Zhan, Song Hong, Xinyi Tan, Tai-Sing Wu, Pei Xiong, Yun-Liang Soo, Molly Meng-Jung Li, Leiduan Hao, Liang Xu, Alex W. Robertson, Bingjun Xu, Ming Yang, Zhenyu Sun
Format: Article
Language:English
Published: Nature Portfolio 2024-11-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-024-53529-2
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