Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet

A novel green ultra high performance liquid chromatography (UHPLC) method was validated and estimated the measurement uncertainty for simultaneous determination of metoprolol tartrate (MET) and hydrochlorothiazide (HCT) in binary tablet. A Zorbax® SB-C18 column with isocratic elution (flow rate 0.9 ...

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Main Authors: Claudia Vilela de Oliveira, Adriano Peron, Anas Rashid, Frank Alonso Gavilano Fajardo, Felipe Rebello Lourenço, Marina Franco Maggi Tavares, María Segunda Aurora Prado
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Journal of Taibah University for Science
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Online Access:https://www.tandfonline.com/doi/10.1080/16583655.2024.2339010
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author Claudia Vilela de Oliveira
Adriano Peron
Anas Rashid
Frank Alonso Gavilano Fajardo
Felipe Rebello Lourenço
Marina Franco Maggi Tavares
María Segunda Aurora Prado
author_facet Claudia Vilela de Oliveira
Adriano Peron
Anas Rashid
Frank Alonso Gavilano Fajardo
Felipe Rebello Lourenço
Marina Franco Maggi Tavares
María Segunda Aurora Prado
author_sort Claudia Vilela de Oliveira
collection DOAJ
description A novel green ultra high performance liquid chromatography (UHPLC) method was validated and estimated the measurement uncertainty for simultaneous determination of metoprolol tartrate (MET) and hydrochlorothiazide (HCT) in binary tablet. A Zorbax® SB-C18 column with isocratic elution (flow rate 0.9 mL min−1) at 25°C was used. Analytes and HCT degradation product were separated in approximately 1 min using acetonitrile:water:triethylamine (17:83:0.2, v/v) as mobile phase. Analytical curves were linear with (R2 > 0.99 for MET and HCT)  with detection limits of 2.42 and 1.05 µg mL−1 for MET and HCT, respectively.  Precision measurements showed RSD% from 0.39 to 1.2% and method accuracy by recovery tests was 100 ± 2%. Measurement uncertainties using Eurachem procedure were 100.1 ± 2.8% and 100.3 ± 2.4% for MET and HCT, respectively. This UHPLC method was accurate, precise, linear and selective, making it suitable for pharmaceutical quality control. It also proved eco-friendly compared to other reported methods.
format Article
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institution Kabale University
issn 1658-3655
language English
publishDate 2024-12-01
publisher Taylor & Francis Group
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series Journal of Taibah University for Science
spelling doaj-art-c1abe8a0144243a9b058afb8e7d660592024-12-17T11:38:48ZengTaylor & Francis GroupJournal of Taibah University for Science1658-36552024-12-0118110.1080/16583655.2024.2339010Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tabletClaudia Vilela de Oliveira0Adriano Peron1Anas Rashid2Frank Alonso Gavilano Fajardo3Felipe Rebello Lourenço4Marina Franco Maggi Tavares5María Segunda Aurora Prado6Department of Pharmacy, School of Pharmaceutical Sciences, University of São Paulo, São Paulo, BrazilAB Sciex Comércio de Instrumentos Laboratoriais Ltda, São Paulo, BrazilDepartment of Neuroscience “Rita Levi Montalcini”, School of Medicine and Surgery, University of Torino, Torino, ItalyDepartment of Pharmacy, School of Pharmaceutical Sciences, University of São Paulo, São Paulo, BrazilDepartment of Pharmacy, School of Pharmaceutical Sciences, University of São Paulo, São Paulo, BrazilDepartment of Fundamental Chemistry, Institute of Chemistry, University of São Paulo, São Paulo, BrazilDepartment of Pharmacy, School of Pharmaceutical Sciences, University of São Paulo, São Paulo, BrazilA novel green ultra high performance liquid chromatography (UHPLC) method was validated and estimated the measurement uncertainty for simultaneous determination of metoprolol tartrate (MET) and hydrochlorothiazide (HCT) in binary tablet. A Zorbax® SB-C18 column with isocratic elution (flow rate 0.9 mL min−1) at 25°C was used. Analytes and HCT degradation product were separated in approximately 1 min using acetonitrile:water:triethylamine (17:83:0.2, v/v) as mobile phase. Analytical curves were linear with (R2 > 0.99 for MET and HCT)  with detection limits of 2.42 and 1.05 µg mL−1 for MET and HCT, respectively.  Precision measurements showed RSD% from 0.39 to 1.2% and method accuracy by recovery tests was 100 ± 2%. Measurement uncertainties using Eurachem procedure were 100.1 ± 2.8% and 100.3 ± 2.4% for MET and HCT, respectively. This UHPLC method was accurate, precise, linear and selective, making it suitable for pharmaceutical quality control. It also proved eco-friendly compared to other reported methods.https://www.tandfonline.com/doi/10.1080/16583655.2024.2339010UHPLCmetoprolol tartratehydrochlorothiazidemeasurement uncertaintygreenness
spellingShingle Claudia Vilela de Oliveira
Adriano Peron
Anas Rashid
Frank Alonso Gavilano Fajardo
Felipe Rebello Lourenço
Marina Franco Maggi Tavares
María Segunda Aurora Prado
Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
Journal of Taibah University for Science
UHPLC
metoprolol tartrate
hydrochlorothiazide
measurement uncertainty
greenness
title Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
title_full Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
title_fullStr Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
title_full_unstemmed Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
title_short Validation, measurement uncertainty estimation and evaluation of UHPLC greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
title_sort validation measurement uncertainty estimation and evaluation of uhplc greenness for simultaneous determination of metoprolol tartrate and hydrochlorothiazide in binary tablet
topic UHPLC
metoprolol tartrate
hydrochlorothiazide
measurement uncertainty
greenness
url https://www.tandfonline.com/doi/10.1080/16583655.2024.2339010
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