Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials

High-magnesium nickel slag (HMNS) is a type of metallurgical waste that has the potential for cementitious activity, and its high content of olivine minerals also makes it a potential for CO2 sequestration. We prepared HMNS-based cementitious backfill materials (HMNS-CBMs) using mechanical activatio...

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Main Authors: Qianqian Wang, Kang Ma, Zequn Yao, Mingliang Tang, Xiaodong Li, Xiaodong Shen, Lijie Guo, Shuguang Hou
Format: Article
Language:English
Published: Wiley 2024-01-01
Series:Advances in Civil Engineering
Online Access:http://dx.doi.org/10.1155/adce/4747710
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author Qianqian Wang
Kang Ma
Zequn Yao
Mingliang Tang
Xiaodong Li
Xiaodong Shen
Lijie Guo
Shuguang Hou
author_facet Qianqian Wang
Kang Ma
Zequn Yao
Mingliang Tang
Xiaodong Li
Xiaodong Shen
Lijie Guo
Shuguang Hou
author_sort Qianqian Wang
collection DOAJ
description High-magnesium nickel slag (HMNS) is a type of metallurgical waste that has the potential for cementitious activity, and its high content of olivine minerals also makes it a potential for CO2 sequestration. We prepared HMNS-based cementitious backfill materials (HMNS-CBMs) using mechanical activation and chemical activation methods. Furthermore, we explored the sequestration efficiency of CO2 under accelerated carbonation conditions. The hydration products and carbonation products of the test blocks were analyzed by using a thermogravimetric-differential scanning calorimeter and X-ray diffraction. Additionally, the microstructure of the materials was analyzed by using mercury intrusion porosimetry and backscattered electron microscopy. Results showed that under carbonation conditions at 80°C for 72 h, the HMNS-CBM had a CO2 adsorption content (CAC) of 6.62 wt.% after a 28-day water curing period. Moreover, under the same curing conditions, the compressive strength of HMNS-CBM treated with citric acid activation reached 49.35 MPa, which was the highest among all the studied samples. The addition of citric acid facilitated CO2 adsorption during the early water curing period and enhanced the development of compressive strength during the later water curing period.
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institution Kabale University
issn 1687-8094
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publishDate 2024-01-01
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series Advances in Civil Engineering
spelling doaj-art-b84f88b5f5264515934133ed050aacc02025-01-04T00:00:03ZengWileyAdvances in Civil Engineering1687-80942024-01-01202410.1155/adce/4747710Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill MaterialsQianqian Wang0Kang Ma1Zequn Yao2Mingliang Tang3Xiaodong Li4Xiaodong Shen5Lijie Guo6Shuguang Hou7College of Materials Science and EngineeringCollege of Materials Science and EngineeringCollege of Materials Science and EngineeringCollege of Materials Science and EngineeringCollege of Materials Science and EngineeringCollege of Materials Science and EngineeringBGRIMM Technology GroupCollege of Transportation EngineeringHigh-magnesium nickel slag (HMNS) is a type of metallurgical waste that has the potential for cementitious activity, and its high content of olivine minerals also makes it a potential for CO2 sequestration. We prepared HMNS-based cementitious backfill materials (HMNS-CBMs) using mechanical activation and chemical activation methods. Furthermore, we explored the sequestration efficiency of CO2 under accelerated carbonation conditions. The hydration products and carbonation products of the test blocks were analyzed by using a thermogravimetric-differential scanning calorimeter and X-ray diffraction. Additionally, the microstructure of the materials was analyzed by using mercury intrusion porosimetry and backscattered electron microscopy. Results showed that under carbonation conditions at 80°C for 72 h, the HMNS-CBM had a CO2 adsorption content (CAC) of 6.62 wt.% after a 28-day water curing period. Moreover, under the same curing conditions, the compressive strength of HMNS-CBM treated with citric acid activation reached 49.35 MPa, which was the highest among all the studied samples. The addition of citric acid facilitated CO2 adsorption during the early water curing period and enhanced the development of compressive strength during the later water curing period.http://dx.doi.org/10.1155/adce/4747710
spellingShingle Qianqian Wang
Kang Ma
Zequn Yao
Mingliang Tang
Xiaodong Li
Xiaodong Shen
Lijie Guo
Shuguang Hou
Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
Advances in Civil Engineering
title Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
title_full Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
title_fullStr Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
title_full_unstemmed Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
title_short Study on the Carbon Dioxide Sequestration Properties of High-Magnesium Nickel Slag-Based Cementitious Backfill Materials
title_sort study on the carbon dioxide sequestration properties of high magnesium nickel slag based cementitious backfill materials
url http://dx.doi.org/10.1155/adce/4747710
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