The hybridization of Ag2CO3 rods with g-C3N4 sheets with improved photocatalytic activity

A series of graphitic carbon nitride/silver carbonate (g-C3N4/Ag2CO3) rod-like composites with different weight contents of g-C3N4 have been prepared by a facile precipitation method. The g-C3N4/Ag2CO3 rod-like composites exhibited higher photocatalytic activity than pure Ag2CO3 toward degradation o...

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Bibliographic Details
Main Authors: Konglin Wu, Yanwei Cui, Xianwen Wei, Xinjie Song, Jiarui Huang
Format: Article
Language:English
Published: Springer 2015-09-01
Series:Journal of Saudi Chemical Society
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Online Access:http://www.sciencedirect.com/science/article/pii/S1319610315000903
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Summary:A series of graphitic carbon nitride/silver carbonate (g-C3N4/Ag2CO3) rod-like composites with different weight contents of g-C3N4 have been prepared by a facile precipitation method. The g-C3N4/Ag2CO3 rod-like composites exhibited higher photocatalytic activity than pure Ag2CO3 toward degradation of rhodamine B (RhB) and methylene blue (MB) under visible-light irradiation. The photocatalytic reaction follows a pseudo-first-order reaction and the rate constants for the degradation of RhB and MB by 3.5% g-C3N4/Ag2CO3 are about 2 times and 1.7 times that of pure Ag2CO3, respectively. A possible photocatalytic mechanism was proposed based on the photoluminescence (PL) spectra and a series of radical trapping experimental analyses. The remarkably improved photocatalytic performance should be ascribed to the heterostructure between Ag2CO3 and g-C3N4, which greatly promoted the photoinduced charge transfer and inhibited the recombination of electrons and holes.
ISSN:1319-6103