Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design
Developing Electrophoretic Deposition (EPD) for Composite Structural Batteries (CSBs) could revolutionise energy storage technology. CSBs offer an innovative solution by seamlessly integrating batteries into structures and effectively reducing weight and space constraints. Despite its successful imp...
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| Format: | Article |
| Language: | English |
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Elsevier
2024-11-01
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| Series: | Materials & Design |
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| Online Access: | http://www.sciencedirect.com/science/article/pii/S0264127524008219 |
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| author | Stefano Russo Marzio Grasso Jian Huang Stevin S. Pramana Francesco Gucci Christopher Shaw Glenn J. Leighton |
| author_facet | Stefano Russo Marzio Grasso Jian Huang Stevin S. Pramana Francesco Gucci Christopher Shaw Glenn J. Leighton |
| author_sort | Stefano Russo |
| collection | DOAJ |
| description | Developing Electrophoretic Deposition (EPD) for Composite Structural Batteries (CSBs) could revolutionise energy storage technology. CSBs offer an innovative solution by seamlessly integrating batteries into structures and effectively reducing weight and space constraints. Despite its successful implementation across various fields, EPD method still lacks comprehensive understanding of the underlying physical and chemical processes due to the number of variables involved. In this study the effects of key parameters associated with the process are investigated with a coupled FEM and analytical approach to find correlations with the deposition process. A Taguchi Design of Experiment with five parameters, namely voltage, concentration, relative weight ratio of LiFePO4 – carbon black particles, length and perimeter of the electrodes is implemented to identify the correlations with mass deposited, thickness of the coating and yield rate when LiFePO4 and Carbon Black particles in ethanol suspension are used. In order to capture the variation over time, each parameter is studied at six different time of deposition. A concentration that optimises yield rate resulting in thickness and mass deposition is identified. The resistivity of the suspension dictates the yield rate dynamics, allowing it to be designed within a specific range to meet requirements of different applications. |
| format | Article |
| id | doaj-art-b6e0afabfd2b4f9881049f6f5cb03ea1 |
| institution | Kabale University |
| issn | 0264-1275 |
| language | English |
| publishDate | 2024-11-01 |
| publisher | Elsevier |
| record_format | Article |
| series | Materials & Design |
| spelling | doaj-art-b6e0afabfd2b4f9881049f6f5cb03ea12024-12-05T05:19:20ZengElsevierMaterials & Design0264-12752024-11-01247113446Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi designStefano Russo0Marzio Grasso1Jian Huang2Stevin S. Pramana3Francesco Gucci4Christopher Shaw5Glenn J. Leighton6Faculty of Engineering and Applied Science, Cranfield University, Cranfield MK43 0AL, UK; Corresponding authors.Faculty of Engineering and Applied Science, Cranfield University, Cranfield MK43 0AL, UK; Corresponding authors.School of Engineering, Newcastle University, Newcastle upon Tyne NE17RU, UKSchool of Engineering, Newcastle University, Newcastle upon Tyne NE17RU, UKFaculty of Engineering and Applied Science, Cranfield University, Cranfield MK43 0AL, UKFaculty of Engineering and Applied Science, Cranfield University, Cranfield MK43 0AL, UKFaculty of Engineering and Applied Science, Cranfield University, Cranfield MK43 0AL, UKDeveloping Electrophoretic Deposition (EPD) for Composite Structural Batteries (CSBs) could revolutionise energy storage technology. CSBs offer an innovative solution by seamlessly integrating batteries into structures and effectively reducing weight and space constraints. Despite its successful implementation across various fields, EPD method still lacks comprehensive understanding of the underlying physical and chemical processes due to the number of variables involved. In this study the effects of key parameters associated with the process are investigated with a coupled FEM and analytical approach to find correlations with the deposition process. A Taguchi Design of Experiment with five parameters, namely voltage, concentration, relative weight ratio of LiFePO4 – carbon black particles, length and perimeter of the electrodes is implemented to identify the correlations with mass deposited, thickness of the coating and yield rate when LiFePO4 and Carbon Black particles in ethanol suspension are used. In order to capture the variation over time, each parameter is studied at six different time of deposition. A concentration that optimises yield rate resulting in thickness and mass deposition is identified. The resistivity of the suspension dictates the yield rate dynamics, allowing it to be designed within a specific range to meet requirements of different applications.http://www.sciencedirect.com/science/article/pii/S0264127524008219Structural BatteryElectrophoretic DepositionLiFePO4 coatingNumerical modelStructural Cathode |
| spellingShingle | Stefano Russo Marzio Grasso Jian Huang Stevin S. Pramana Francesco Gucci Christopher Shaw Glenn J. Leighton Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design Materials & Design Structural Battery Electrophoretic Deposition LiFePO4 coating Numerical model Structural Cathode |
| title | Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design |
| title_full | Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design |
| title_fullStr | Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design |
| title_full_unstemmed | Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design |
| title_short | Electrophoretic deposition of LiFePO4 and carbon black: A numerical study to explore longitudinal trends using Taguchi design |
| title_sort | electrophoretic deposition of lifepo4 and carbon black a numerical study to explore longitudinal trends using taguchi design |
| topic | Structural Battery Electrophoretic Deposition LiFePO4 coating Numerical model Structural Cathode |
| url | http://www.sciencedirect.com/science/article/pii/S0264127524008219 |
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