Bidirectional nuclear polarization through electric dipole spin resonance enabled by spin-orbit interaction in a single hole planar quantum dot device

Abstract Spin exchange between confined holes and nuclei has been demonstrated for zero-dimensional quantum dots by optical techniques but has not been observed for gated planar structures. Here, enabled by strong spin-orbit interaction, and under microwave (MW) illumination, we report hyperfine int...

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Bibliographic Details
Main Authors: Sergei Studenikin, Jordan Ducatel, Olivia Ellis, Marek Korkusinski, Alex Bogan, Piotr Zawadzki, D. Guy Austing, Andrew Sachrajda
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:npj Quantum Information
Online Access:https://doi.org/10.1038/s41534-025-01075-0
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Summary:Abstract Spin exchange between confined holes and nuclei has been demonstrated for zero-dimensional quantum dots by optical techniques but has not been observed for gated planar structures. Here, enabled by strong spin-orbit interaction, and under microwave (MW) illumination, we report hyperfine interaction and dynamic polarization of the nuclei with confined heavy-holes in a GaAs/AlGaAs double quantum dot device. Distinct signatures of the resultant hyperfine field on the electron dipole spin resonance (EDSR) signal include: hysteresis on sweeping the magnetic (B-) field up and down with characteristics that are strongly dependent on both MW power and B-field sweep rate; free bidirectional dragging of the EDSR condition; stable locking on resonance on a timescale of hours; slow temporal change as the hyperfine field decays (T1 nuclear decay time ~ 100 s); and oscillations in time commensurate with Larmor precession of the 75As nuclei. We attain pumped nuclear (Overhauser) fields ~ 25 mT (~20% nuclear polarization).
ISSN:2056-6387