Reducing the V oc Loss of Hole Transport Layer-Free Carbon-Based Perovskite Solar Cells via Dual Interfacial Passivation

Reducing the V oc Loss of Hole Transport Layer-Free Carbon-Based Perovskite Solar Cells via Dual Interfacial Passivation

Highlights Li2CO3 is used to modify conformal SnO2 as electron transport layer for hole transport layer-free carbon-based perovskite solar cells (C-PSCs). CO3 2− can induce MA release from the perovskite layer, resulting in PbI2 at the grain boundary of top interface of perovskite film which can pas...

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Bibliographic Details
Main Authors: Xian Zhang, Fangzhou Liu, Yan Guan, Yu Zou, Cuncun Wu, Dongchang Shi, Hongkai Zhang, Wenjin Yu, Dechun Zou, Yangyang Zhang, Lixin Xiao, Shijian Zheng
Format: Article
Language:English
Published: SpringerOpen 2025-05-01
Series:Nano-Micro Letters
Subjects:
Perovskite solar cells
Carbon electrode
Hole transport layer-free
Open-circuit voltage
Indoor photovoltaic
Online Access:https://doi.org/10.1007/s40820-025-01775-4
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Summary:Highlights Li2CO3 is used to modify conformal SnO2 as electron transport layer for hole transport layer-free carbon-based perovskite solar cells (C-PSCs). CO3 2− can induce MA release from the perovskite layer, resulting in PbI2 at the grain boundary of top interface of perovskite film which can passivate the grain boundary and the top surface defects. The Li2CO3-modified C-PSC exhibits a high power conversion efficiency (PCE) of 19.1%, with a V oc of 1.142 V. A record-high PCE of 33.2% is obtained under weak light-emitting diode illumination (2000 lx, 3000 K).
ISSN:2311-6706
2150-5551

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