Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films

Abstract The coupling of photovoltaic and pyroelectric effects is a common phenomenon in ferroelectric films and often results in coupling enhancements. Although the coupling effects of a variety of ferroelectric films have been examined in terms of improved performance, they have yet to be quantita...

Full description

Saved in:
Bibliographic Details
Main Authors: Chaosheng Hu, Xingyue Liu, Huiyu Dan, Chong Guo, Maoyi Zhang, Chris R. Bowen, Ya Yang
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-56233-x
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1832594537454764032
author Chaosheng Hu
Xingyue Liu
Huiyu Dan
Chong Guo
Maoyi Zhang
Chris R. Bowen
Ya Yang
author_facet Chaosheng Hu
Xingyue Liu
Huiyu Dan
Chong Guo
Maoyi Zhang
Chris R. Bowen
Ya Yang
author_sort Chaosheng Hu
collection DOAJ
description Abstract The coupling of photovoltaic and pyroelectric effects is a common phenomenon in ferroelectric films and often results in coupling enhancements. Although the coupling effects of a variety of ferroelectric films have been examined in terms of improved performance, they have yet to be quantitatively ranked and assessed. Here, by taking the charge coupling factor, the Yang’s charge, and output energy as metrics to evaluate the coupling performance, a methodology is developed for evaluating the performance of a range ferroelectric films when the pyroelectric and photovoltaic effects are coupled. By experimentally measuring and quantitatively ranking the evaluation metrics, the influence of coupling effects on the output charge and the energy harvesting capabilities of various ferroelectric films can be readily visualized. In addition, the analysis of the underlying reasons for the coupling enhancement enables optimization of the methods to quantify the charge coupling factor. This work provides a unique reference for the selection of materials, optimization of performance, and energy harvesting for coupled ferroelectric film-based generators.
format Article
id doaj-art-29903f3df0f548648980a64d47fc2f04
institution Kabale University
issn 2041-1723
language English
publishDate 2025-01-01
publisher Nature Portfolio
record_format Article
series Nature Communications
spelling doaj-art-29903f3df0f548648980a64d47fc2f042025-01-19T12:32:19ZengNature PortfolioNature Communications2041-17232025-01-0116111210.1038/s41467-025-56233-xQuantifying the pyroelectric and photovoltaic coupling series of ferroelectric filmsChaosheng Hu0Xingyue Liu1Huiyu Dan2Chong Guo3Maoyi Zhang4Chris R. Bowen5Ya Yang6CAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-Nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of SciencesCAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-Nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of SciencesCAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-Nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of SciencesCAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-Nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of SciencesSchool of Nanoscience and Technology, University of Chinese Academy of SciencesDepartment of Mechanical Engineering, University of BathCAS Center for Excellence in Nanoscience, Beijing Key Laboratory of Micro-Nano Energy and Sensor, Beijing Institute of Nanoenergy and Nanosystems, Chinese Academy of SciencesAbstract The coupling of photovoltaic and pyroelectric effects is a common phenomenon in ferroelectric films and often results in coupling enhancements. Although the coupling effects of a variety of ferroelectric films have been examined in terms of improved performance, they have yet to be quantitatively ranked and assessed. Here, by taking the charge coupling factor, the Yang’s charge, and output energy as metrics to evaluate the coupling performance, a methodology is developed for evaluating the performance of a range ferroelectric films when the pyroelectric and photovoltaic effects are coupled. By experimentally measuring and quantitatively ranking the evaluation metrics, the influence of coupling effects on the output charge and the energy harvesting capabilities of various ferroelectric films can be readily visualized. In addition, the analysis of the underlying reasons for the coupling enhancement enables optimization of the methods to quantify the charge coupling factor. This work provides a unique reference for the selection of materials, optimization of performance, and energy harvesting for coupled ferroelectric film-based generators.https://doi.org/10.1038/s41467-025-56233-x
spellingShingle Chaosheng Hu
Xingyue Liu
Huiyu Dan
Chong Guo
Maoyi Zhang
Chris R. Bowen
Ya Yang
Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
Nature Communications
title Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
title_full Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
title_fullStr Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
title_full_unstemmed Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
title_short Quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
title_sort quantifying the pyroelectric and photovoltaic coupling series of ferroelectric films
url https://doi.org/10.1038/s41467-025-56233-x
work_keys_str_mv AT chaoshenghu quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT xingyueliu quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT huiyudan quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT chongguo quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT maoyizhang quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT chrisrbowen quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms
AT yayang quantifyingthepyroelectricandphotovoltaiccouplingseriesofferroelectricfilms