Near-Unity Nitrate to Ammonia conversion via reactant enrichment at the solid-liquid interface

Abstract Electroreduction of nitrate (NO3 ‒) to ammonia (NH3) is a promising approach for addressing energy challenges. However, the activity is limited by NO3 ‒ mass transfer, particularly at reduction potential, where an abundance of electrons on the cathode surface repels NO3 ‒ from the inner Hel...

Full description

Saved in:
Bibliographic Details
Main Authors: Wanru Liao, Jun Wang, Yao Tan, Xin Zi, Changxu Liu, Qiyou Wang, Li Zhu, Cheng-Wei Kao, Ting-Shan Chan, Hongmei Li, Yali Zhang, Kang Liu, Chao Cai, Junwei Fu, Beidou Xi, Emiliano Cortés, Liyuan Chai, Min Liu
Format: Article
Language:English
Published: Nature Portfolio 2025-07-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-025-60671-y
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Abstract Electroreduction of nitrate (NO3 ‒) to ammonia (NH3) is a promising approach for addressing energy challenges. However, the activity is limited by NO3 ‒ mass transfer, particularly at reduction potential, where an abundance of electrons on the cathode surface repels NO3 ‒ from the inner Helmholtz plane (IHP). This constraint becomes pronounced as NO3 ‒ concentration decreases, impeding practical applications in the conversion of NO3 ‒-to-NH3. Herein, we propose a generic strategy of catalyst bandstructure engineering for the enrichment of negatively charged ions through solid-liquid (S-L) junction-mediated charge rearrangement within IHP. Specifically, during NO3 ‒ reduction, the formation of S-L junction induces hole transfer from Ag-doped MoS2 (Ag-MoS2) to electrode/electrolyte interface, triggering abundant positive charges on the IHP to attract NO3 ‒. Thus, Ag-MoS2 exhibits a ~ 28.6-fold NO3 ‒ concentration in the IHP than the counterpart without junction, and achieves near-100% NH3 Faradaic efficiency with an NH3 yield rate of ~20 mg h‒1 cm‒2 under ultralow NO3 ‒ concentrations.
ISSN:2041-1723