Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method

This study aimed to determine the caffeine and L-theanine contents in tea infusions prepared under varying fermentation degrees, brewing conditions (temperature and time), and serving methods (tea bag/loose-leaf). Infusions of six tea types (green, white, yellow, oolong, black, and Pu-erh) and vario...

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Main Authors: Gamze Ayakdaş, Duygu Ağagündüz
Format: Article
Language:English
Published: MDPI AG 2025-06-01
Series:Foods
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Online Access:https://www.mdpi.com/2304-8158/14/13/2313
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author Gamze Ayakdaş
Duygu Ağagündüz
author_facet Gamze Ayakdaş
Duygu Ağagündüz
author_sort Gamze Ayakdaş
collection DOAJ
description This study aimed to determine the caffeine and L-theanine contents in tea infusions prepared under varying fermentation degrees, brewing conditions (temperature and time), and serving methods (tea bag/loose-leaf). Infusions of six tea types (green, white, yellow, oolong, black, and Pu-erh) and various serving forms of green, white, and black tea were brewed at 80 °C and 100 °C for 2, 5, and 10 min. Contents were analyzed using reversed-phase high-performance liquid chromatography. Caffeine levels were highest in black and yellow tea (14 ± 1.0 mg/200 mL and 13.8 ± 0.2 mg/200 mL, respectively), both of which were significantly higher than the levels in green, white, and oolong tea (11 ± 2.1 mg/200 mL; 5.8 ± 0.7 mg/200 mL; and 4 ± 1.6 mg/200 mL, respectively; <i>p</i> < 0.001), whereas Pu-erh tea (13 ± 2.9 mg/200 mL) had caffeine levels comparable to that of black tea (<i>p</i> > 0.05). L-Theanine levels were highest in black and green tea (12.3 ± 2.8 mg/200 mL and 12.5 ± 2.5 mg/200 mL, respectively), and these levels were significantly higher than those in the other tea types (<i>p</i> < 0.001). Brewing temperature only affected caffeine levels n, whereas L-oolong tea (4.4 → 13.5 mg/200 mL, <i>p</i> < 0.05); theanine remained stable (<i>p</i> > 0.05). Longer brewing times significantly raised both components (e.g., yellow tea caffeine levels rose to 53 ± 16.9 mg/200 mL at 10 min; <i>p</i> < 0.05). In black tea, cup-sized bags yielded higher caffeine levels (39 ± 9.9 mg/200 mL) than loose-leaf (24 ± 7.2 mg/200 mL) and teapot bags (<i>p</i> < 0.001). Serving method had no effect on green and white teas (<i>p</i> > 0.05). In conclusion, fermentation rate, brewing conditions, and serving method were found to influence the caffeine and L-theanine levels of tea infusions.
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publishDate 2025-06-01
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spelling doaj-art-f838e6008e0a4c8c9b35e225b34b84a82025-08-20T03:28:37ZengMDPI AGFoods2304-81582025-06-011413231310.3390/foods14132313Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic MethodGamze Ayakdaş0Duygu Ağagündüz1Department of Nutrition and Dietetics, Acıbadem University, Kerem Aydınlar Campus, Ataşehir, Istanbul 34755, TurkeyDepartment of Nutrition and Dietetics, Gazi University, Emek, Ankara 06490, TurkeyThis study aimed to determine the caffeine and L-theanine contents in tea infusions prepared under varying fermentation degrees, brewing conditions (temperature and time), and serving methods (tea bag/loose-leaf). Infusions of six tea types (green, white, yellow, oolong, black, and Pu-erh) and various serving forms of green, white, and black tea were brewed at 80 °C and 100 °C for 2, 5, and 10 min. Contents were analyzed using reversed-phase high-performance liquid chromatography. Caffeine levels were highest in black and yellow tea (14 ± 1.0 mg/200 mL and 13.8 ± 0.2 mg/200 mL, respectively), both of which were significantly higher than the levels in green, white, and oolong tea (11 ± 2.1 mg/200 mL; 5.8 ± 0.7 mg/200 mL; and 4 ± 1.6 mg/200 mL, respectively; <i>p</i> < 0.001), whereas Pu-erh tea (13 ± 2.9 mg/200 mL) had caffeine levels comparable to that of black tea (<i>p</i> > 0.05). L-Theanine levels were highest in black and green tea (12.3 ± 2.8 mg/200 mL and 12.5 ± 2.5 mg/200 mL, respectively), and these levels were significantly higher than those in the other tea types (<i>p</i> < 0.001). Brewing temperature only affected caffeine levels n, whereas L-oolong tea (4.4 → 13.5 mg/200 mL, <i>p</i> < 0.05); theanine remained stable (<i>p</i> > 0.05). Longer brewing times significantly raised both components (e.g., yellow tea caffeine levels rose to 53 ± 16.9 mg/200 mL at 10 min; <i>p</i> < 0.05). In black tea, cup-sized bags yielded higher caffeine levels (39 ± 9.9 mg/200 mL) than loose-leaf (24 ± 7.2 mg/200 mL) and teapot bags (<i>p</i> < 0.001). Serving method had no effect on green and white teas (<i>p</i> > 0.05). In conclusion, fermentation rate, brewing conditions, and serving method were found to influence the caffeine and L-theanine levels of tea infusions.https://www.mdpi.com/2304-8158/14/13/2313L-theaninecaffeineteabrewingHPLC
spellingShingle Gamze Ayakdaş
Duygu Ağagündüz
Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
Foods
L-theanine
caffeine
tea
brewing
HPLC
title Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
title_full Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
title_fullStr Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
title_full_unstemmed Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
title_short Determination of L-Theanine and Caffeine Contents in Tea Infusions with Different Fermentation Degrees and Brewing Conditions Using the Chromatographic Method
title_sort determination of l theanine and caffeine contents in tea infusions with different fermentation degrees and brewing conditions using the chromatographic method
topic L-theanine
caffeine
tea
brewing
HPLC
url https://www.mdpi.com/2304-8158/14/13/2313
work_keys_str_mv AT gamzeayakdas determinationofltheanineandcaffeinecontentsinteainfusionswithdifferentfermentationdegreesandbrewingconditionsusingthechromatographicmethod
AT duyguagagunduz determinationofltheanineandcaffeinecontentsinteainfusionswithdifferentfermentationdegreesandbrewingconditionsusingthechromatographicmethod