Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols

This study investigates the dynamics of thermal plumes interacting with the liquid–air interface in straight-chain alcohols and their mixtures using a photothermal imaging technique based on thermal lensing. This method enables the indirect measurement of temperature gradients via changes in refract...

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Main Authors: Reese W. Anderson, Allison I. Anderson, Mark W. Gealy, Darin J. Ulness
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Liquids
Subjects:
Online Access:https://www.mdpi.com/2673-8015/4/4/41
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author Reese W. Anderson
Allison I. Anderson
Mark W. Gealy
Darin J. Ulness
author_facet Reese W. Anderson
Allison I. Anderson
Mark W. Gealy
Darin J. Ulness
author_sort Reese W. Anderson
collection DOAJ
description This study investigates the dynamics of thermal plumes interacting with the liquid–air interface in straight-chain alcohols and their mixtures using a photothermal imaging technique based on thermal lensing. This method enables the indirect measurement of temperature gradients via changes in refractive index caused by localized laser heating. Employing a collimated laser beam, the results show the formation and evolution of cylindrical heated zones and their interactions with the liquid–air interface. The study reveals that, while some alcohols exhibit stable surface behaviors, others demonstrate complex dynamical behaviors, including strong stable steady-state oscillations. The findings contribute to understanding fluid dynamics in molecular liquids near their liquid–air interfaces.
format Article
id doaj-art-f51aeabd19d24a93b26d5d58872748d1
institution Kabale University
issn 2673-8015
language English
publishDate 2024-11-01
publisher MDPI AG
record_format Article
series Liquids
spelling doaj-art-f51aeabd19d24a93b26d5d58872748d12024-12-27T14:36:26ZengMDPI AGLiquids2673-80152024-11-014473274310.3390/liquids4040041Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain AlcoholsReese W. Anderson0Allison I. Anderson1Mark W. Gealy2Darin J. Ulness3Department of Chemistry, Concordia College, Moorhead, MN 56562, USADepartment of Chemistry, Concordia College, Moorhead, MN 56562, USADepartment of Physics, Concordia College, Moorhead, MN 56562, USADepartment of Chemistry, Concordia College, Moorhead, MN 56562, USAThis study investigates the dynamics of thermal plumes interacting with the liquid–air interface in straight-chain alcohols and their mixtures using a photothermal imaging technique based on thermal lensing. This method enables the indirect measurement of temperature gradients via changes in refractive index caused by localized laser heating. Employing a collimated laser beam, the results show the formation and evolution of cylindrical heated zones and their interactions with the liquid–air interface. The study reveals that, while some alcohols exhibit stable surface behaviors, others demonstrate complex dynamical behaviors, including strong stable steady-state oscillations. The findings contribute to understanding fluid dynamics in molecular liquids near their liquid–air interfaces.https://www.mdpi.com/2673-8015/4/4/41thermal lensingphotothermal techniquesconvective heat transferthermal plumesstraight-chain alcoholsliquid–air interfaces
spellingShingle Reese W. Anderson
Allison I. Anderson
Mark W. Gealy
Darin J. Ulness
Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
Liquids
thermal lensing
photothermal techniques
convective heat transfer
thermal plumes
straight-chain alcohols
liquid–air interfaces
title Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
title_full Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
title_fullStr Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
title_full_unstemmed Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
title_short Interactions of Laser-Induced Thermal Plume with Liquid–Air Interfaces in Straight-Chain Alcohols
title_sort interactions of laser induced thermal plume with liquid air interfaces in straight chain alcohols
topic thermal lensing
photothermal techniques
convective heat transfer
thermal plumes
straight-chain alcohols
liquid–air interfaces
url https://www.mdpi.com/2673-8015/4/4/41
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AT markwgealy interactionsoflaserinducedthermalplumewithliquidairinterfacesinstraightchainalcohols
AT darinjulness interactionsoflaserinducedthermalplumewithliquidairinterfacesinstraightchainalcohols