Complexation of trivalent lanthanide cations with amino(<i>O</i>-alkyl)methylenephosphonic acids as the closest organophosphorus analogues of nitrilotriacetic acid

The complexation of new complexones, analogues of nitrilotriacetic (H3NTA) and nitrilotrimethylenephosphonic (H6NTP) acids containing monobasic (O-alkyl)methylenephosphonic fragments as donor groups, with trivalent cations of lanthanides was studied. The stability and deprotonation constants of 1:1...

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Main Authors: A. R. Garifzyanov, I. I. Mirzayanov, I. D. Shurygin, E. O. Chibirev, F. V. Devyatov
Format: Article
Language:English
Published: Kazan Federal University 2025-06-01
Series:Учёные записки Казанского университета: Серия Естественные науки
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Online Access:https://uzakuesc.elpub.ru/jour/article/view/342
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Summary:The complexation of new complexones, analogues of nitrilotriacetic (H3NTA) and nitrilotrimethylenephosphonic (H6NTP) acids containing monobasic (O-alkyl)methylenephosphonic fragments as donor groups, with trivalent cations of lanthanides was studied. The stability and deprotonation constants of 1:1 complexes and the fractional distribution of complex forms were determined using pH-metric titration in combination with mathematical modeling. The complexation properties of N-[(O-butyl)hydroxyphosphorylmethyl]iminodiacetic acid were compared with those of H3NTA based on the linear free-energy relationships.
ISSN:2542-064X
2500-218X