Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone

This study investigates the thermal stability and structural changes of AB-type carbonate-hydroxyapatite (AB-type CHA) prepared from heat-treated bovine bone occurring during calcination at 1000, 1100, 1200, and 1300 °C. The structural phase changes and morphological properties of the calcined AB-ty...

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Main Authors: Hassanen Jaber, Mohanad H. Mousa, Awais Qadir, Ján Dusza, László Tóth, Péter Pinke, Tünde Kovács
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Open Ceramics
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Online Access:http://www.sciencedirect.com/science/article/pii/S2666539524001652
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author Hassanen Jaber
Mohanad H. Mousa
Awais Qadir
Ján Dusza
László Tóth
Péter Pinke
Tünde Kovács
author_facet Hassanen Jaber
Mohanad H. Mousa
Awais Qadir
Ján Dusza
László Tóth
Péter Pinke
Tünde Kovács
author_sort Hassanen Jaber
collection DOAJ
description This study investigates the thermal stability and structural changes of AB-type carbonate-hydroxyapatite (AB-type CHA) prepared from heat-treated bovine bone occurring during calcination at 1000, 1100, 1200, and 1300 °C. The structural phase changes and morphological properties of the calcined AB-type CHA samples were assessed by SEM/EDX, XRD, FTIR, and Raman spectroscopy. The findings highlighted that the decomposition of AB-type CHA undergoes three stages: Dehydroxylation, formation of A-type carbonate-hydroxyapatite (A-type CHA), and decomposition. Pure AB-type CHA was stable in a vacuum atmosphere, and no decomposition occurred at temperatures up to 1000 °C. Dehydroxylation and formation of A-type CHA occurred at 1100 °C. The AB-type CHA partially decomposed at a temperature of 1200 °C. A-type CHA, tricalcium phosphate (α-TCP), and tetracalcium phosphate (TTCP) were the main products of the decomposition reactions, and tricalcium phosphate (β-TCP) was also detected in the system. After sintering at 1300 °C, the AB-type CHA was completely decomposed and converted into α-TCP, β-TCP, and TTCP.
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publishDate 2024-12-01
publisher Elsevier
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series Open Ceramics
spelling doaj-art-e2359e29e5eb4aea8084d0aef1b8e6352024-12-08T06:13:01ZengElsevierOpen Ceramics2666-53952024-12-0120100701Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine boneHassanen Jaber0Mohanad H. Mousa1Awais Qadir2Ján Dusza3László Tóth4Péter Pinke5Tünde Kovács6Banki Donat Faculty of Mechanical and Safety Engineering, Óbuda University, Budapest, Hungary; Biomedical Engineering Department, College of Engineering, University of Thi-Qar, Nasiriyah, Iraq; Corresponding author.Shatrah Technical Institute, Southern Technical University (STU), Basra, IraqInstitute of Materials Science, Technische Universität Bergakademie Freiberg, Gustav-Zeuner Straße 5, 09599 Freiberg, GermanyBanki Donat Faculty of Mechanical and Safety Engineering, Óbuda University, Budapest, Hungary; Institute of Materials Research, Slovak Academy of Sciences, Watsonova 47, 04001 Košice, SlovakiaBanki Donat Faculty of Mechanical and Safety Engineering, Óbuda University, Budapest, HungaryBanki Donat Faculty of Mechanical and Safety Engineering, Óbuda University, Budapest, HungaryBanki Donat Faculty of Mechanical and Safety Engineering, Óbuda University, Budapest, HungaryThis study investigates the thermal stability and structural changes of AB-type carbonate-hydroxyapatite (AB-type CHA) prepared from heat-treated bovine bone occurring during calcination at 1000, 1100, 1200, and 1300 °C. The structural phase changes and morphological properties of the calcined AB-type CHA samples were assessed by SEM/EDX, XRD, FTIR, and Raman spectroscopy. The findings highlighted that the decomposition of AB-type CHA undergoes three stages: Dehydroxylation, formation of A-type carbonate-hydroxyapatite (A-type CHA), and decomposition. Pure AB-type CHA was stable in a vacuum atmosphere, and no decomposition occurred at temperatures up to 1000 °C. Dehydroxylation and formation of A-type CHA occurred at 1100 °C. The AB-type CHA partially decomposed at a temperature of 1200 °C. A-type CHA, tricalcium phosphate (α-TCP), and tetracalcium phosphate (TTCP) were the main products of the decomposition reactions, and tricalcium phosphate (β-TCP) was also detected in the system. After sintering at 1300 °C, the AB-type CHA was completely decomposed and converted into α-TCP, β-TCP, and TTCP.http://www.sciencedirect.com/science/article/pii/S2666539524001652HydroxyapatiteCalcium phosphateTetracalcium phosphateTricalcium phosphateThermal stability
spellingShingle Hassanen Jaber
Mohanad H. Mousa
Awais Qadir
Ján Dusza
László Tóth
Péter Pinke
Tünde Kovács
Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
Open Ceramics
Hydroxyapatite
Calcium phosphate
Tetracalcium phosphate
Tricalcium phosphate
Thermal stability
title Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
title_full Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
title_fullStr Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
title_full_unstemmed Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
title_short Comprehensive investigation into thermal stability of AB-type bio- carbonate hydroxyapatite synthesized via heat-treated bovine bone
title_sort comprehensive investigation into thermal stability of ab type bio carbonate hydroxyapatite synthesized via heat treated bovine bone
topic Hydroxyapatite
Calcium phosphate
Tetracalcium phosphate
Tricalcium phosphate
Thermal stability
url http://www.sciencedirect.com/science/article/pii/S2666539524001652
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