Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries

Abstract Amorphous FePO4 (AFP) is a promising cathode material for lithium‐ion and sodium‐ion batteries (LIBs & SIBs) due to its stability, high theoretical capacity, and cost‐effective processing. However, challenges such as low electronic conductivity and volumetric changes seriously hinder it...

Full description

Saved in:
Bibliographic Details
Main Authors: Peng Tang, John Prochest Kachenje, Xiaoping Qin, Huihui Li, Xiangdong Zeng, Haiyang Tian, Wei Cao, Ying Zhou, Di Heng, Shishi Yuan, Xun Jia, Xiaolong Zhang, Xiaoyu Zhao
Format: Article
Language:English
Published: Wiley-VCH 2024-12-01
Series:ChemElectroChem
Subjects:
Online Access:https://doi.org/10.1002/celc.202400484
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846143825048764416
author Peng Tang
John Prochest Kachenje
Xiaoping Qin
Huihui Li
Xiangdong Zeng
Haiyang Tian
Wei Cao
Ying Zhou
Di Heng
Shishi Yuan
Xun Jia
Xiaolong Zhang
Xiaoyu Zhao
author_facet Peng Tang
John Prochest Kachenje
Xiaoping Qin
Huihui Li
Xiangdong Zeng
Haiyang Tian
Wei Cao
Ying Zhou
Di Heng
Shishi Yuan
Xun Jia
Xiaolong Zhang
Xiaoyu Zhao
author_sort Peng Tang
collection DOAJ
description Abstract Amorphous FePO4 (AFP) is a promising cathode material for lithium‐ion and sodium‐ion batteries (LIBs & SIBs) due to its stability, high theoretical capacity, and cost‐effective processing. However, challenges such as low electronic conductivity and volumetric changes seriously hinder its practical application. To overcome these hurdles, core‐shell structure synthesis emerges as a useful solution. In this work, we for the first time made this comprehensive review on the progresses of core‐shell amorphous FePO4 (CS‐AFP). This review summarizes 1) various synthesis methods such as template method, microemulsion method, and other methods, 2) characterization techniques, and 3) their involvement in improving electrochemical performance in LIBs and SIBs. In terms of further understanding the underlying mechanisms of advancing electrochemical performance of CS‐AFP, the future perspective on two main aspects were insighted: (i) in situ characterization and (ii) novel designs of materials and structure for CS‐AFP.
format Article
id doaj-art-e1ab5b6a25b1401b9a2a52ec47125483
institution Kabale University
issn 2196-0216
language English
publishDate 2024-12-01
publisher Wiley-VCH
record_format Article
series ChemElectroChem
spelling doaj-art-e1ab5b6a25b1401b9a2a52ec471254832024-12-02T10:01:24ZengWiley-VCHChemElectroChem2196-02162024-12-011123n/an/a10.1002/celc.202400484Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion BatteriesPeng Tang0John Prochest Kachenje1Xiaoping Qin2Huihui Li3Xiangdong Zeng4Haiyang Tian5Wei Cao6Ying Zhou7Di Heng8Shishi Yuan9Xun Jia10Xiaolong Zhang11Xiaoyu Zhao12School of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaCollege of Materials and Chemistry & Chemical Engineering Chengdu University of Technology Chengdu, Sichuan 610059 PR ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaSchool of Chemical Engineering Sichuan University of Science and Engineering Zigong, Sichuan 643000 ChinaTianjin Key Laboratory of Brine Chemical Engineering and Resource Eco-Utilization Tianjin University of Science and Technology Tianjin 300457 ChinaAbstract Amorphous FePO4 (AFP) is a promising cathode material for lithium‐ion and sodium‐ion batteries (LIBs & SIBs) due to its stability, high theoretical capacity, and cost‐effective processing. However, challenges such as low electronic conductivity and volumetric changes seriously hinder its practical application. To overcome these hurdles, core‐shell structure synthesis emerges as a useful solution. In this work, we for the first time made this comprehensive review on the progresses of core‐shell amorphous FePO4 (CS‐AFP). This review summarizes 1) various synthesis methods such as template method, microemulsion method, and other methods, 2) characterization techniques, and 3) their involvement in improving electrochemical performance in LIBs and SIBs. In terms of further understanding the underlying mechanisms of advancing electrochemical performance of CS‐AFP, the future perspective on two main aspects were insighted: (i) in situ characterization and (ii) novel designs of materials and structure for CS‐AFP.https://doi.org/10.1002/celc.202400484Amorphous FePO4Core-shell structureLithium-ion batteriesSodium-ion batteries
spellingShingle Peng Tang
John Prochest Kachenje
Xiaoping Qin
Huihui Li
Xiangdong Zeng
Haiyang Tian
Wei Cao
Ying Zhou
Di Heng
Shishi Yuan
Xun Jia
Xiaolong Zhang
Xiaoyu Zhao
Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
ChemElectroChem
Amorphous FePO4
Core-shell structure
Lithium-ion batteries
Sodium-ion batteries
title Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
title_full Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
title_fullStr Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
title_full_unstemmed Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
title_short Core‐Shell Amorphous FePO4 as Cathode Material for Lithium‐Ion and Sodium‐Ion Batteries
title_sort core shell amorphous fepo4 as cathode material for lithium ion and sodium ion batteries
topic Amorphous FePO4
Core-shell structure
Lithium-ion batteries
Sodium-ion batteries
url https://doi.org/10.1002/celc.202400484
work_keys_str_mv AT pengtang coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT johnprochestkachenje coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT xiaopingqin coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT huihuili coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT xiangdongzeng coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT haiyangtian coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT weicao coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT yingzhou coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT diheng coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT shishiyuan coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT xunjia coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT xiaolongzhang coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries
AT xiaoyuzhao coreshellamorphousfepo4ascathodematerialforlithiumionandsodiumionbatteries