Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities

Household dust is a major reservoir for indoor pollutants, yet its epigenetic effects remain poorly characterized. This study investigated household airborne dust’s total DNA demethylation potential (TDP) and its association with 14 priority polybrominated diphenyl ethers (PBDEs) in 43 residences ac...

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Main Authors: Xiaotong Zhang, Wenying Zhang, Fengjing Song, Tingting Liu, Chengyu Chen, Xiaomin Xie, Chao Wang, Hang Du, Lin Fan, Weiyi Zhang, Yiming Sun, Xianliang Wang
Format: Article
Language:English
Published: Elsevier 2025-09-01
Series:Environment International
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Online Access:http://www.sciencedirect.com/science/article/pii/S0160412025004842
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author Xiaotong Zhang
Wenying Zhang
Fengjing Song
Tingting Liu
Chengyu Chen
Xiaomin Xie
Chao Wang
Hang Du
Lin Fan
Weiyi Zhang
Yiming Sun
Xianliang Wang
author_facet Xiaotong Zhang
Wenying Zhang
Fengjing Song
Tingting Liu
Chengyu Chen
Xiaomin Xie
Chao Wang
Hang Du
Lin Fan
Weiyi Zhang
Yiming Sun
Xianliang Wang
author_sort Xiaotong Zhang
collection DOAJ
description Household dust is a major reservoir for indoor pollutants, yet its epigenetic effects remain poorly characterized. This study investigated household airborne dust’s total DNA demethylation potential (TDP) and its association with 14 priority polybrominated diphenyl ethers (PBDEs) in 43 residences across Lanzhou, Suzhou, and Harbin. The median TDP (5-AZA-CdR equivalent) was 0.016 (range: 0–1.006), while the median Σ14PBDEs concentration was 2085.73 ng/g (range: 64.51–26,746.47 ng/g), with BDE-209 dominating (>90 %). Exploratory factor analysis identified three principal components explaining 80.59 % of the variance, with PBDE levels significantly influenced by socioeconomic status, building materials, household products, and occupant behaviors (P < 0.05). Linear regression models revealed significant negative associations between TDP and BDE-153 (β = -0.020; 95 % CI: −0.035 to −0.005, β = -0.003; 95 % CI = −0.045 to −0.016), BDE-183 (β = -0.003; 95 % CI: −0.006 to −0.001), BDE-209 (β = -0.000; 95 % CI: −0.000 to −0.000), and Factor 2-derived congeners (β = -0.389; 95 % CI = -0.626 to −0.152, β = -0.389; 95 % CI = −0.616 to −0.162). In contrast, BDE-66 exhibited a positive association (β = 0.052; 95 % CI: 0.022 to 0.082). The findings suggest that household dust and its PBDE components may pose epigenetic health risks through DNA demethylation alterations.
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spelling doaj-art-db4687e266f644c8b0b2e096ee3100f92025-08-20T05:04:13ZengElsevierEnvironment International0160-41202025-09-0120310973310.1016/j.envint.2025.109733Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese citiesXiaotong Zhang0Wenying Zhang1Fengjing Song2Tingting Liu3Chengyu Chen4Xiaomin Xie5Chao Wang6Hang Du7Lin Fan8Weiyi Zhang9Yiming Sun10Xianliang Wang11China CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, China; School of Public Health, Nanjing Medical University, Nanjing, Jiangsu Province 210000, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, China; School of Public Health, Nanjing Medical University, Nanjing, Jiangsu Province 210000, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, ChinaChina CDC Key Laboratory of Environment and Population Health, National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, Beijing 100021, China; School of Public Health, Nanjing Medical University, Nanjing, Jiangsu Province 210000, China; Corresponding author at: National Institute of Environmental Health, Chinese Center for Disease Control and Prevention, #7 Panjiayuan Nanli Road, Chaoyang District, Beijing 100021, PR China.Household dust is a major reservoir for indoor pollutants, yet its epigenetic effects remain poorly characterized. This study investigated household airborne dust’s total DNA demethylation potential (TDP) and its association with 14 priority polybrominated diphenyl ethers (PBDEs) in 43 residences across Lanzhou, Suzhou, and Harbin. The median TDP (5-AZA-CdR equivalent) was 0.016 (range: 0–1.006), while the median Σ14PBDEs concentration was 2085.73 ng/g (range: 64.51–26,746.47 ng/g), with BDE-209 dominating (>90 %). Exploratory factor analysis identified three principal components explaining 80.59 % of the variance, with PBDE levels significantly influenced by socioeconomic status, building materials, household products, and occupant behaviors (P < 0.05). Linear regression models revealed significant negative associations between TDP and BDE-153 (β = -0.020; 95 % CI: −0.035 to −0.005, β = -0.003; 95 % CI = −0.045 to −0.016), BDE-183 (β = -0.003; 95 % CI: −0.006 to −0.001), BDE-209 (β = -0.000; 95 % CI: −0.000 to −0.000), and Factor 2-derived congeners (β = -0.389; 95 % CI = -0.626 to −0.152, β = -0.389; 95 % CI = −0.616 to −0.162). In contrast, BDE-66 exhibited a positive association (β = 0.052; 95 % CI: 0.022 to 0.082). The findings suggest that household dust and its PBDE components may pose epigenetic health risks through DNA demethylation alterations.http://www.sciencedirect.com/science/article/pii/S0160412025004842Household dustTotal DNA demethylation potential (TDP)Polybrominated diphenyl ethers (PBDEs)Influential factors
spellingShingle Xiaotong Zhang
Wenying Zhang
Fengjing Song
Tingting Liu
Chengyu Chen
Xiaomin Xie
Chao Wang
Hang Du
Lin Fan
Weiyi Zhang
Yiming Sun
Xianliang Wang
Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
Environment International
Household dust
Total DNA demethylation potential (TDP)
Polybrominated diphenyl ethers (PBDEs)
Influential factors
title Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
title_full Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
title_fullStr Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
title_full_unstemmed Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
title_short Characterization of total DNA demethylation potential and its PBDE components of household airborne dust in three Chinese cities
title_sort characterization of total dna demethylation potential and its pbde components of household airborne dust in three chinese cities
topic Household dust
Total DNA demethylation potential (TDP)
Polybrominated diphenyl ethers (PBDEs)
Influential factors
url http://www.sciencedirect.com/science/article/pii/S0160412025004842
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