Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography

The magnetic molecularly imprinted polymers had been synthesized for the selective extraction and clean-up of 4-methylimidazole in cola, the most popular soft beverage. The magnetic molecularly imprinted polymers were prepared by means of suspension polymerization, using Fe 3 O 4 as magnetically com...

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Main Authors: Helin Ye, Xiaofen Chen, Zufei Feng
Format: Article
Language:English
Published: SAGE Publishing 2017-03-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1177/0263617416667361
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author Helin Ye
Xiaofen Chen
Zufei Feng
author_facet Helin Ye
Xiaofen Chen
Zufei Feng
author_sort Helin Ye
collection DOAJ
description The magnetic molecularly imprinted polymers had been synthesized for the selective extraction and clean-up of 4-methylimidazole in cola, the most popular soft beverage. The magnetic molecularly imprinted polymers were prepared by means of suspension polymerization, using Fe 3 O 4 as magnetically component, 4-methylimidazole as template molecule, methacrylic acid as functional monomers, and ethylene glycol dimethacrylate as a cross-linker, initiated by 2,2′-azobisisobutyronitrile. The obtained magnetic molecularly imprinted polymers were characterized by scanning electron microscopy, Fourier transform infrared, X-ray diffraction, and vibrating sample magnetometer. High performance liquid chromatography was used for the analysis of the target analyte. The polymers were evaluated further by batch rebinding experiments. From the derived Freundlich isotherm equation, their binding capacity and binding strength were determined. Structurally similar compound and a reference compound were used for investigating the selective recognition capability of magnetic molecularly imprinted polymers. The recoveries of spiked samples ranged from 90.19 to 104.29%. The prepared magnetic molecularly imprinted polymers could be applied to selectively preconcentrate and determine 4-methylimidazole in cola samples.
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series Adsorption Science & Technology
spelling doaj-art-da954f6cfd1a49ab8ae7ac2d08a61ed52025-01-02T21:31:26ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382017-03-013510.1177/0263617416667361Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatographyHelin YeXiaofen ChenZufei FengThe magnetic molecularly imprinted polymers had been synthesized for the selective extraction and clean-up of 4-methylimidazole in cola, the most popular soft beverage. The magnetic molecularly imprinted polymers were prepared by means of suspension polymerization, using Fe 3 O 4 as magnetically component, 4-methylimidazole as template molecule, methacrylic acid as functional monomers, and ethylene glycol dimethacrylate as a cross-linker, initiated by 2,2′-azobisisobutyronitrile. The obtained magnetic molecularly imprinted polymers were characterized by scanning electron microscopy, Fourier transform infrared, X-ray diffraction, and vibrating sample magnetometer. High performance liquid chromatography was used for the analysis of the target analyte. The polymers were evaluated further by batch rebinding experiments. From the derived Freundlich isotherm equation, their binding capacity and binding strength were determined. Structurally similar compound and a reference compound were used for investigating the selective recognition capability of magnetic molecularly imprinted polymers. The recoveries of spiked samples ranged from 90.19 to 104.29%. The prepared magnetic molecularly imprinted polymers could be applied to selectively preconcentrate and determine 4-methylimidazole in cola samples.https://doi.org/10.1177/0263617416667361
spellingShingle Helin Ye
Xiaofen Chen
Zufei Feng
Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
Adsorption Science & Technology
title Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
title_full Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
title_fullStr Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
title_full_unstemmed Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
title_short Preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4-methylimidazole in soft beverage by high performance liquid chromatography
title_sort preparations of magnetic molecularly imprinted polymer for selective recognition and determination of 4 methylimidazole in soft beverage by high performance liquid chromatography
url https://doi.org/10.1177/0263617416667361
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AT xiaofenchen preparationsofmagneticmolecularlyimprintedpolymerforselectiverecognitionanddeterminationof4methylimidazoleinsoftbeveragebyhighperformanceliquidchromatography
AT zufeifeng preparationsofmagneticmolecularlyimprintedpolymerforselectiverecognitionanddeterminationof4methylimidazoleinsoftbeveragebyhighperformanceliquidchromatography