Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images

Abstract Magnetic skyrmions are quasi-particles with a swirling spin texture that form two-dimensional lattices. Skyrmion lattices can exhibit defects in response to geometric constraints, variations of temperature or applied magnetic fields. Measuring deformations in skyrmion lattices is important...

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Main Authors: Thibaud Denneulin, András Kovács, Raluca Boltje, Nikolai S. Kiselev, Rafal E. Dunin-Borkowski
Format: Article
Language:English
Published: Nature Portfolio 2024-05-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-024-62873-8
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author Thibaud Denneulin
András Kovács
Raluca Boltje
Nikolai S. Kiselev
Rafal E. Dunin-Borkowski
author_facet Thibaud Denneulin
András Kovács
Raluca Boltje
Nikolai S. Kiselev
Rafal E. Dunin-Borkowski
author_sort Thibaud Denneulin
collection DOAJ
description Abstract Magnetic skyrmions are quasi-particles with a swirling spin texture that form two-dimensional lattices. Skyrmion lattices can exhibit defects in response to geometric constraints, variations of temperature or applied magnetic fields. Measuring deformations in skyrmion lattices is important to understand the interplay between the lattice structure and external influences. Geometric phase analysis (GPA) is a Fourier-based image processing method that is used to measure deformation fields in high resolution transmission electron microscopy (TEM) images of crystalline materials. Here, we show that GPA can be applied quantitatively to Lorentz TEM images of two-dimensional skyrmion lattices obtained from a chiral magnet of FeGe. First, GPA is used to map deformation fields around a 5–7 dislocation and the results are compared with the linear theory of elasticity. Second, rotation angles between skyrmion crystal grains are measured and compared with angles calculated from the density of dislocations. Third, an orientational order parameter and the corresponding correlation function are calculated to describe the evolution of the disorder as a function of applied magnetic field. The influence of sources of artifacts such as geometric distortions and large defoci are also discussed.
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issn 2045-2322
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publishDate 2024-05-01
publisher Nature Portfolio
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series Scientific Reports
spelling doaj-art-d383572fbb9b45d693c09f776521c45d2025-01-05T12:28:21ZengNature PortfolioScientific Reports2045-23222024-05-0114111010.1038/s41598-024-62873-8Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy imagesThibaud Denneulin0András Kovács1Raluca Boltje2Nikolai S. Kiselev3Rafal E. Dunin-Borkowski4Ernst Ruska-Centre for Microscopy and Spectroscopy with Electrons, Forschungszentrum JülichErnst Ruska-Centre for Microscopy and Spectroscopy with Electrons, Forschungszentrum JülichErnst Ruska-Centre for Microscopy and Spectroscopy with Electrons, Forschungszentrum JülichPeter Grünberg Institute and Institute for Advanced Simulation, Forschungszentrum Jülich and JARAErnst Ruska-Centre for Microscopy and Spectroscopy with Electrons, Forschungszentrum JülichAbstract Magnetic skyrmions are quasi-particles with a swirling spin texture that form two-dimensional lattices. Skyrmion lattices can exhibit defects in response to geometric constraints, variations of temperature or applied magnetic fields. Measuring deformations in skyrmion lattices is important to understand the interplay between the lattice structure and external influences. Geometric phase analysis (GPA) is a Fourier-based image processing method that is used to measure deformation fields in high resolution transmission electron microscopy (TEM) images of crystalline materials. Here, we show that GPA can be applied quantitatively to Lorentz TEM images of two-dimensional skyrmion lattices obtained from a chiral magnet of FeGe. First, GPA is used to map deformation fields around a 5–7 dislocation and the results are compared with the linear theory of elasticity. Second, rotation angles between skyrmion crystal grains are measured and compared with angles calculated from the density of dislocations. Third, an orientational order parameter and the corresponding correlation function are calculated to describe the evolution of the disorder as a function of applied magnetic field. The influence of sources of artifacts such as geometric distortions and large defoci are also discussed.https://doi.org/10.1038/s41598-024-62873-8Magnetic skyrmionsLorentz TEMGeometric phase analysisDeformations
spellingShingle Thibaud Denneulin
András Kovács
Raluca Boltje
Nikolai S. Kiselev
Rafal E. Dunin-Borkowski
Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
Scientific Reports
Magnetic skyrmions
Lorentz TEM
Geometric phase analysis
Deformations
title Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
title_full Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
title_fullStr Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
title_full_unstemmed Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
title_short Geometric phase analysis of magnetic skyrmion lattices in Lorentz transmission electron microscopy images
title_sort geometric phase analysis of magnetic skyrmion lattices in lorentz transmission electron microscopy images
topic Magnetic skyrmions
Lorentz TEM
Geometric phase analysis
Deformations
url https://doi.org/10.1038/s41598-024-62873-8
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AT andraskovacs geometricphaseanalysisofmagneticskyrmionlatticesinlorentztransmissionelectronmicroscopyimages
AT ralucaboltje geometricphaseanalysisofmagneticskyrmionlatticesinlorentztransmissionelectronmicroscopyimages
AT nikolaiskiselev geometricphaseanalysisofmagneticskyrmionlatticesinlorentztransmissionelectronmicroscopyimages
AT rafaleduninborkowski geometricphaseanalysisofmagneticskyrmionlatticesinlorentztransmissionelectronmicroscopyimages