Tutorial on modelling chromatographic surrogation of biological processes

The accurate emulation of biological partition systems through physicochemical models is crucial in pharmacology, toxicology, and environmental science for understanding the ADMET profiles of substances. Direct experimentation on biological systems can be long, expensive, and ethically and practical...

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Main Authors: Elisabet Fuguet, Martí Rosés
Format: Article
Language:English
Published: Elsevier 2024-11-01
Series:Journal of Chromatography Open
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2772391724000768
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author Elisabet Fuguet
Martí Rosés
author_facet Elisabet Fuguet
Martí Rosés
author_sort Elisabet Fuguet
collection DOAJ
description The accurate emulation of biological partition systems through physicochemical models is crucial in pharmacology, toxicology, and environmental science for understanding the ADMET profiles of substances. Direct experimentation on biological systems can be long, expensive, and ethically and practically challenging, so developing reliable physicochemical models is essential. These models help predict compound behaviour in organisms, reduce animal testing, and streamline drug discovery and risk assessment. Chromatographic systems are of particular interest to mimic biological or environmental processes because of its versatility, as they provide a large number of different partition systems only by changing the nature of the mobile and stationary or pseudostationary phases. The effectiveness of any physicochemical system in emulating biological processes is usually evaluated through empirical correlation with biological data. However, the characterization of physicochemical and biological systems using a common model, such as Abraham's solvation model, allows to identify the best physicochemical systems to surrogate particular biological or environmental processes, only by comparison of the system constants of the models. This tutorial demonstrates how to compare, predict, and improve the efficiency of physicochemical systems to surrogate biological or environmental ones without the need for previous empirical correlations. Skin permeation is presented as example of chromatographic surrogation and case study.
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spelling doaj-art-cf4792c3fbe147ef9bea0a298f8e5d4f2024-12-14T06:34:14ZengElsevierJournal of Chromatography Open2772-39172024-11-016100189Tutorial on modelling chromatographic surrogation of biological processesElisabet Fuguet0Martí Rosés1Departament d'Enginyeria Química i Química Analítica, i Institut de Biomedicina de la Universitat de Barcelona (IBUB), Universitat de Barcelona (UB), Martí i Franquès 1-11, E-08028, Barcelona, Spain; Serra Húnter Fellow, Generalitat de Catalunya, SpainDepartament d'Enginyeria Química i Química Analítica, i Institut de Biomedicina de la Universitat de Barcelona (IBUB), Universitat de Barcelona (UB), Martí i Franquès 1-11, E-08028, Barcelona, Spain; Corresponding author.The accurate emulation of biological partition systems through physicochemical models is crucial in pharmacology, toxicology, and environmental science for understanding the ADMET profiles of substances. Direct experimentation on biological systems can be long, expensive, and ethically and practically challenging, so developing reliable physicochemical models is essential. These models help predict compound behaviour in organisms, reduce animal testing, and streamline drug discovery and risk assessment. Chromatographic systems are of particular interest to mimic biological or environmental processes because of its versatility, as they provide a large number of different partition systems only by changing the nature of the mobile and stationary or pseudostationary phases. The effectiveness of any physicochemical system in emulating biological processes is usually evaluated through empirical correlation with biological data. However, the characterization of physicochemical and biological systems using a common model, such as Abraham's solvation model, allows to identify the best physicochemical systems to surrogate particular biological or environmental processes, only by comparison of the system constants of the models. This tutorial demonstrates how to compare, predict, and improve the efficiency of physicochemical systems to surrogate biological or environmental ones without the need for previous empirical correlations. Skin permeation is presented as example of chromatographic surrogation and case study.http://www.sciencedirect.com/science/article/pii/S2772391724000768Chromatographic surrogation, Linear free energy relationshipsAbraham's solvation modelEuclidean distancesPrincipal component analysisSkin permeation
spellingShingle Elisabet Fuguet
Martí Rosés
Tutorial on modelling chromatographic surrogation of biological processes
Journal of Chromatography Open
Chromatographic surrogation, Linear free energy relationships
Abraham's solvation model
Euclidean distances
Principal component analysis
Skin permeation
title Tutorial on modelling chromatographic surrogation of biological processes
title_full Tutorial on modelling chromatographic surrogation of biological processes
title_fullStr Tutorial on modelling chromatographic surrogation of biological processes
title_full_unstemmed Tutorial on modelling chromatographic surrogation of biological processes
title_short Tutorial on modelling chromatographic surrogation of biological processes
title_sort tutorial on modelling chromatographic surrogation of biological processes
topic Chromatographic surrogation, Linear free energy relationships
Abraham's solvation model
Euclidean distances
Principal component analysis
Skin permeation
url http://www.sciencedirect.com/science/article/pii/S2772391724000768
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