A material design guideline for self-assembled vertically aligned nanocomposite thin films

Nanocomposite thin films, comprising two or more distinct materials at nanoscale, have attracted significant research interest considering their potential of integrating multiple functionalities for advanced applications in electronics, energy storage, photonics, photovoltaics, and sensing. Among va...

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Main Authors: Jiawei Song, Haiyan Wang
Format: Article
Language:English
Published: IOP Publishing 2025-01-01
Series:JPhys Materials
Subjects:
Online Access:https://doi.org/10.1088/2515-7639/ad9bee
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author Jiawei Song
Haiyan Wang
author_facet Jiawei Song
Haiyan Wang
author_sort Jiawei Song
collection DOAJ
description Nanocomposite thin films, comprising two or more distinct materials at nanoscale, have attracted significant research interest considering their potential of integrating multiple functionalities for advanced applications in electronics, energy storage, photonics, photovoltaics, and sensing. Among various fabrication technologies, a one-step pulsed laser deposition process enables the self-assembly of materials into vertically aligned nanocomposites (VANs). The demonstrated VAN systems include oxide–oxide, oxide–metal, and nitride–metal VAN films and their growth mechanisms are vastly different. These complexities pose challenges in the designs, materials selection, and prediction of the resulted VAN morphologies and properties. The review examines the key roles that surface energy plays in the VAN growth and provides a generalized materials design guideline combining the two key factors of surface energy and lattice strain/mismatch, along with other factors related to growth kinetics that collectively influence the morphology of VAN films. This review aims to offer valuable guidelines for future material selection and microstructure design in the development of self-assembled VAN films.
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spelling doaj-art-ce7ee105056048cab1c713c802722d8f2025-01-06T06:58:07ZengIOP PublishingJPhys Materials2515-76392025-01-018101200210.1088/2515-7639/ad9beeA material design guideline for self-assembled vertically aligned nanocomposite thin filmsJiawei Song0https://orcid.org/0000-0003-4013-1200Haiyan Wang1https://orcid.org/0000-0002-7397-1209School of Materials Engineering, Purdue University , West Lafayette 47907, United States of AmericaSchool of Materials Engineering, Purdue University , West Lafayette 47907, United States of America; School of Electrical and Computer Engineering, Purdue University , West Lafayette 47907, United States of AmericaNanocomposite thin films, comprising two or more distinct materials at nanoscale, have attracted significant research interest considering their potential of integrating multiple functionalities for advanced applications in electronics, energy storage, photonics, photovoltaics, and sensing. Among various fabrication technologies, a one-step pulsed laser deposition process enables the self-assembly of materials into vertically aligned nanocomposites (VANs). The demonstrated VAN systems include oxide–oxide, oxide–metal, and nitride–metal VAN films and their growth mechanisms are vastly different. These complexities pose challenges in the designs, materials selection, and prediction of the resulted VAN morphologies and properties. The review examines the key roles that surface energy plays in the VAN growth and provides a generalized materials design guideline combining the two key factors of surface energy and lattice strain/mismatch, along with other factors related to growth kinetics that collectively influence the morphology of VAN films. This review aims to offer valuable guidelines for future material selection and microstructure design in the development of self-assembled VAN films.https://doi.org/10.1088/2515-7639/ad9beenanocompositesvertically aligned nanocomposites (VANs)self-assemblysurface energygrowth mechanism
spellingShingle Jiawei Song
Haiyan Wang
A material design guideline for self-assembled vertically aligned nanocomposite thin films
JPhys Materials
nanocomposites
vertically aligned nanocomposites (VANs)
self-assembly
surface energy
growth mechanism
title A material design guideline for self-assembled vertically aligned nanocomposite thin films
title_full A material design guideline for self-assembled vertically aligned nanocomposite thin films
title_fullStr A material design guideline for self-assembled vertically aligned nanocomposite thin films
title_full_unstemmed A material design guideline for self-assembled vertically aligned nanocomposite thin films
title_short A material design guideline for self-assembled vertically aligned nanocomposite thin films
title_sort material design guideline for self assembled vertically aligned nanocomposite thin films
topic nanocomposites
vertically aligned nanocomposites (VANs)
self-assembly
surface energy
growth mechanism
url https://doi.org/10.1088/2515-7639/ad9bee
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