Electrochemical recycling of lithium‐ion batteries: Advancements and future directions

Abstract Lithium‐ion batteries (LIBs) are at the forefront of technological innovation in the current global energy‐transition paradigm, driving surging demand for electric vehicles and renewable energy‐storage solutions. Despite their widespread use and superior energy densities, the environmental...

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Main Authors: Stefanie Arnold, Jean G. A. Ruthes, Choonsoo Kim, Volker Presser
Format: Article
Language:English
Published: Wiley 2024-11-01
Series:EcoMat
Subjects:
Online Access:https://doi.org/10.1002/eom2.12494
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author Stefanie Arnold
Jean G. A. Ruthes
Choonsoo Kim
Volker Presser
author_facet Stefanie Arnold
Jean G. A. Ruthes
Choonsoo Kim
Volker Presser
author_sort Stefanie Arnold
collection DOAJ
description Abstract Lithium‐ion batteries (LIBs) are at the forefront of technological innovation in the current global energy‐transition paradigm, driving surging demand for electric vehicles and renewable energy‐storage solutions. Despite their widespread use and superior energy densities, the environmental footprint and resource scarcity associated with LIBs necessitate sustainable recycling strategies. This comprehensive review critically examines the existing landscape of battery recycling methodologies, including pyrometallurgical, hydrometallurgical, and direct recycling techniques, along with emerging approaches such as bioleaching and electrochemical separation. Our analysis not only underscores the environmental and efficiency challenges posed by conventional recycling methods but also highlights the promising potential of electrochemical techniques for enhancing selectivity, reducing energy consumption, and mitigating secondary waste production. By delving into recent advancements and juxtaposing various recycling methodologies, we pinpoint electrochemical recycling as a pivotal technology for efficiently recovering valuable metals, such as Li, Ni, Co, and Mn, from spent LIBs in an environmentally benign manner. Our discussion extends to the scalability, economic viability, and future directions of electrochemical recycling, and advocates for their integration into global battery‐recycling infrastructure to address the dual challenges of resource depletion and environmental sustainability.
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spelling doaj-art-cb0910467eea49aaa8f3f7ff5d0d3d9e2024-11-11T02:41:52ZengWileyEcoMat2567-31732024-11-01611n/an/a10.1002/eom2.12494Electrochemical recycling of lithium‐ion batteries: Advancements and future directionsStefanie Arnold0Jean G. A. Ruthes1Choonsoo Kim2Volker Presser3INM—Leibniz Institute for New Materials Saarbrücken GermanyINM—Leibniz Institute for New Materials Saarbrücken GermanyDepartment of Environmental Engineering and Institute of Energy/Environment Convergence Technologies Kongju National University Cheonan Republic of KoreaINM—Leibniz Institute for New Materials Saarbrücken GermanyAbstract Lithium‐ion batteries (LIBs) are at the forefront of technological innovation in the current global energy‐transition paradigm, driving surging demand for electric vehicles and renewable energy‐storage solutions. Despite their widespread use and superior energy densities, the environmental footprint and resource scarcity associated with LIBs necessitate sustainable recycling strategies. This comprehensive review critically examines the existing landscape of battery recycling methodologies, including pyrometallurgical, hydrometallurgical, and direct recycling techniques, along with emerging approaches such as bioleaching and electrochemical separation. Our analysis not only underscores the environmental and efficiency challenges posed by conventional recycling methods but also highlights the promising potential of electrochemical techniques for enhancing selectivity, reducing energy consumption, and mitigating secondary waste production. By delving into recent advancements and juxtaposing various recycling methodologies, we pinpoint electrochemical recycling as a pivotal technology for efficiently recovering valuable metals, such as Li, Ni, Co, and Mn, from spent LIBs in an environmentally benign manner. Our discussion extends to the scalability, economic viability, and future directions of electrochemical recycling, and advocates for their integration into global battery‐recycling infrastructure to address the dual challenges of resource depletion and environmental sustainability.https://doi.org/10.1002/eom2.12494cobaltelectrochemical recoveryelemental selectivitylithiumlithium‐ion battery recyclingnickel
spellingShingle Stefanie Arnold
Jean G. A. Ruthes
Choonsoo Kim
Volker Presser
Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
EcoMat
cobalt
electrochemical recovery
elemental selectivity
lithium
lithium‐ion battery recycling
nickel
title Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
title_full Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
title_fullStr Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
title_full_unstemmed Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
title_short Electrochemical recycling of lithium‐ion batteries: Advancements and future directions
title_sort electrochemical recycling of lithium ion batteries advancements and future directions
topic cobalt
electrochemical recovery
elemental selectivity
lithium
lithium‐ion battery recycling
nickel
url https://doi.org/10.1002/eom2.12494
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AT jeangaruthes electrochemicalrecyclingoflithiumionbatteriesadvancementsandfuturedirections
AT choonsookim electrochemicalrecyclingoflithiumionbatteriesadvancementsandfuturedirections
AT volkerpresser electrochemicalrecyclingoflithiumionbatteriesadvancementsandfuturedirections