Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency

Chantal Emade Nkwelle,1,2 Smith B Babiaka,3,4 Clovis S Metuge,2,3 Kimberly Liang,5 Unique Stephens,5 Seraphine Nkie Esemu,1 David S Zuzga,5 Kristy Shuda McGuire,5 Luis J Montaner,5 Roland N Ndip,1 Ian Tietjen,5 Fidele Ntie-Kang2,3,6 1Department of Microbiology and Parasitology, Faculty of Science, U...

Full description

Saved in:
Bibliographic Details
Main Authors: Emade Nkwelle C, Babiaka SB, Metuge CS, Liang K, Stephens U, Esemu SN, Zuzga DS, Shuda McGuire K, Montaner LJ, Ndip RN, Tietjen I, Ntie-Kang F
Format: Article
Language:English
Published: Dove Medical Press 2024-11-01
Series:Journal of Experimental Pharmacology
Subjects:
Online Access:https://www.dovepress.com/croton-oligandrus-pierre--hutch-euphorbiaceae-extracts-and-isolated-co-peer-reviewed-fulltext-article-JEP
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846163082439557120
author Emade Nkwelle C
Babiaka SB
Metuge CS
Liang K
Stephens U
Esemu SN
Zuzga DS
Shuda McGuire K
Montaner LJ
Ndip RN
Tietjen I
Ntie-Kang F
author_facet Emade Nkwelle C
Babiaka SB
Metuge CS
Liang K
Stephens U
Esemu SN
Zuzga DS
Shuda McGuire K
Montaner LJ
Ndip RN
Tietjen I
Ntie-Kang F
author_sort Emade Nkwelle C
collection DOAJ
description Chantal Emade Nkwelle,1,2 Smith B Babiaka,3,4 Clovis S Metuge,2,3 Kimberly Liang,5 Unique Stephens,5 Seraphine Nkie Esemu,1 David S Zuzga,5 Kristy Shuda McGuire,5 Luis J Montaner,5 Roland N Ndip,1 Ian Tietjen,5 Fidele Ntie-Kang2,3,6 1Department of Microbiology and Parasitology, Faculty of Science, University of Buea, Buea, Cameroon; 2Center for Drug Discovery, Faculty of Science, University of Buea, Buea, Cameroon; 3Department of Chemistry, Faculty of Science, University of Buea, Buea, Cameroon; 4Department of Microbial Bioactive Compound, University of Tübingen, Tübingen, Germany; 5Drug Discovery, The Wistar Institute of Anatomy and Biology, Philadelphia, PA, USA; 6Institute of Pharmacy, Martin-Luther University Halle-Wittenberg, Halle, GermanyCorrespondence: Ian Tietjen, The Wistar Institute, 3601 Spruce Street, Philadelphia, PA, 19104, USA, Tel +1-215-898-3938, Email itietjen@wistar.org Fidele Ntie-Kang, Center for Drug Discovery, Faculty of Science, University of Buea, P. O. Box 63, Buea, Cameroon, Tel +237-673872475, Email fidele.ntie-kang@ubuea.cmBackground: Croton oligandrus Pierre & Hutch is a tropical tree that grows in West and Central Africa, used in ethnomedicine to treat cancer, diabetes, headaches, convulsions, urinary diseases, and inflammatory diseases. As other Croton species have been observed to possess chemical compounds that target HIV latency-reversal, we hypothesized that this species may have similar properties.Aim of the Study: The identification of extracts and compounds of this species, which have HIV-1 latency-reversing activity in J-Lat T cell lines.Methods: The stem bark was obtained, air-dried, powdered, and extracted using dichloromethane. In vitro flow cytometry was used to monitor GFP expression, a marker of HIV latency reversal, following treatment of J-Lat T cells with extracts and compounds.Results: Four extracts were found to reverse HIV latency, the most active extract showing better activity (ie, latency reversal in 69.7 ± 7.1% [mean ± s.e.m.] of J-Lat 10.6 cells at 1 μg/mL) than control agents prostratin (46.2 ± 9.5% at 1.2 μg.mL) and the “Mukungulu” (Croton megalobotrys) extract (34.9 ± 24.2% at 1 μg/mL). Extracts reversed HIV latency through mechanisms over and above protein kinase C (PKC) activation and distinct from histone deacetylase (HDAC) inhibition. The most active extract also synergized with the control HDAC inhibitor romidepsin but did not synergize with other extracts. Isolated compounds (β-Stigmasterol and lupeol) had limited but consistent latency reversal on their own.Conclusion: The plant extracts and compounds reverse HIV latency through mechanisms additional to PKC activation and/or synergize with romidepsin in vitro. Extracts and compounds from this plant may enhance the activity of current HIV latency-reversing agents being assessed in HIV cure studies.Keywords: antiviral, compounds, extracts, HIV-1, latency reversal, screening
format Article
id doaj-art-cafdaa2b6e3d4036ac249dacc21d3ac9
institution Kabale University
issn 1179-1454
language English
publishDate 2024-11-01
publisher Dove Medical Press
record_format Article
series Journal of Experimental Pharmacology
spelling doaj-art-cafdaa2b6e3d4036ac249dacc21d3ac92024-11-19T16:55:51ZengDove Medical PressJournal of Experimental Pharmacology1179-14542024-11-01Volume 1641342597420Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 LatencyEmade Nkwelle CBabiaka SBMetuge CSLiang KStephens UEsemu SNZuzga DSShuda McGuire KMontaner LJNdip RNTietjen INtie-Kang FChantal Emade Nkwelle,1,2 Smith B Babiaka,3,4 Clovis S Metuge,2,3 Kimberly Liang,5 Unique Stephens,5 Seraphine Nkie Esemu,1 David S Zuzga,5 Kristy Shuda McGuire,5 Luis J Montaner,5 Roland N Ndip,1 Ian Tietjen,5 Fidele Ntie-Kang2,3,6 1Department of Microbiology and Parasitology, Faculty of Science, University of Buea, Buea, Cameroon; 2Center for Drug Discovery, Faculty of Science, University of Buea, Buea, Cameroon; 3Department of Chemistry, Faculty of Science, University of Buea, Buea, Cameroon; 4Department of Microbial Bioactive Compound, University of Tübingen, Tübingen, Germany; 5Drug Discovery, The Wistar Institute of Anatomy and Biology, Philadelphia, PA, USA; 6Institute of Pharmacy, Martin-Luther University Halle-Wittenberg, Halle, GermanyCorrespondence: Ian Tietjen, The Wistar Institute, 3601 Spruce Street, Philadelphia, PA, 19104, USA, Tel +1-215-898-3938, Email itietjen@wistar.org Fidele Ntie-Kang, Center for Drug Discovery, Faculty of Science, University of Buea, P. O. Box 63, Buea, Cameroon, Tel +237-673872475, Email fidele.ntie-kang@ubuea.cmBackground: Croton oligandrus Pierre & Hutch is a tropical tree that grows in West and Central Africa, used in ethnomedicine to treat cancer, diabetes, headaches, convulsions, urinary diseases, and inflammatory diseases. As other Croton species have been observed to possess chemical compounds that target HIV latency-reversal, we hypothesized that this species may have similar properties.Aim of the Study: The identification of extracts and compounds of this species, which have HIV-1 latency-reversing activity in J-Lat T cell lines.Methods: The stem bark was obtained, air-dried, powdered, and extracted using dichloromethane. In vitro flow cytometry was used to monitor GFP expression, a marker of HIV latency reversal, following treatment of J-Lat T cells with extracts and compounds.Results: Four extracts were found to reverse HIV latency, the most active extract showing better activity (ie, latency reversal in 69.7 ± 7.1% [mean ± s.e.m.] of J-Lat 10.6 cells at 1 μg/mL) than control agents prostratin (46.2 ± 9.5% at 1.2 μg.mL) and the “Mukungulu” (Croton megalobotrys) extract (34.9 ± 24.2% at 1 μg/mL). Extracts reversed HIV latency through mechanisms over and above protein kinase C (PKC) activation and distinct from histone deacetylase (HDAC) inhibition. The most active extract also synergized with the control HDAC inhibitor romidepsin but did not synergize with other extracts. Isolated compounds (β-Stigmasterol and lupeol) had limited but consistent latency reversal on their own.Conclusion: The plant extracts and compounds reverse HIV latency through mechanisms additional to PKC activation and/or synergize with romidepsin in vitro. Extracts and compounds from this plant may enhance the activity of current HIV latency-reversing agents being assessed in HIV cure studies.Keywords: antiviral, compounds, extracts, HIV-1, latency reversal, screeninghttps://www.dovepress.com/croton-oligandrus-pierre--hutch-euphorbiaceae-extracts-and-isolated-co-peer-reviewed-fulltext-article-JEPantiviralcompoundsextractshiv-1latency reversalscreening
spellingShingle Emade Nkwelle C
Babiaka SB
Metuge CS
Liang K
Stephens U
Esemu SN
Zuzga DS
Shuda McGuire K
Montaner LJ
Ndip RN
Tietjen I
Ntie-Kang F
Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
Journal of Experimental Pharmacology
antiviral
compounds
extracts
hiv-1
latency reversal
screening
title Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
title_full Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
title_fullStr Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
title_full_unstemmed Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
title_short Croton oligandrus Pierre & Hutch (Euphorbiaceae) Extracts and Isolated Compounds Reverse HIV-1 Latency
title_sort croton oligandrus pierre amp hutch euphorbiaceae extracts and isolated compounds reverse hiv 1 latency
topic antiviral
compounds
extracts
hiv-1
latency reversal
screening
url https://www.dovepress.com/croton-oligandrus-pierre--hutch-euphorbiaceae-extracts-and-isolated-co-peer-reviewed-fulltext-article-JEP
work_keys_str_mv AT emadenkwellec crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT babiakasb crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT metugecs crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT liangk crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT stephensu crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT esemusn crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT zuzgads crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT shudamcguirek crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT montanerlj crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT ndiprn crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT tietjeni crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency
AT ntiekangf crotonoligandruspierreamphutcheuphorbiaceaeextractsandisolatedcompoundsreversehiv1latency