Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates

Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth ato...

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Main Authors: Michael Peper, Yiyi Li, Daniel Y. Knapp, Mila Bileska, Shuo Ma, Genyue Liu, Pai Peng, Bichen Zhang, Sebastian P. Horvath, Alex P. Burgers, Jeff D. Thompson
Format: Article
Language:English
Published: American Physical Society 2025-01-01
Series:Physical Review X
Online Access:http://doi.org/10.1103/PhysRevX.15.011009
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author Michael Peper
Yiyi Li
Daniel Y. Knapp
Mila Bileska
Shuo Ma
Genyue Liu
Pai Peng
Bichen Zhang
Sebastian P. Horvath
Alex P. Burgers
Jeff D. Thompson
author_facet Michael Peper
Yiyi Li
Daniel Y. Knapp
Mila Bileska
Shuo Ma
Genyue Liu
Pai Peng
Bichen Zhang
Sebastian P. Horvath
Alex P. Burgers
Jeff D. Thompson
author_sort Michael Peper
collection DOAJ
description Highly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth atoms has not been demonstrated or experimentally validated. Here, we present multichannel quantum defect models for highly excited ^{174}Yb and ^{171}Yb Rydberg states with L≤2. The models are developed using a combination of existing literature data and new, high-precision laser and microwave spectroscopy in an atomic beam, and validated by detailed comparison with experimentally measured Stark shifts and magnetic moments. We then use these models to compute interaction potentials between two Yb atoms, and find excellent agreement with direct measurements in an optical tweezer array. From the computed interaction potential, we identify an anomalous Förster resonance that likely degraded the fidelity of previous entangling gates in ^{171}Yb using F=3/2 Rydberg states. We then identify a more suitable F=1/2 state, and achieve a state-of-the-art controlled-z gate fidelity of F=0.994(1), with the remaining error fully explained by known sources. This work establishes a solid foundation for the continued development of quantum computing, simulation, and entanglement-enhanced metrology with Yb neutral atom arrays.
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spelling doaj-art-b7004c35b8154425b7ab7f16bcd8eb5c2025-01-17T15:05:42ZengAmerican Physical SocietyPhysical Review X2160-33082025-01-0115101100910.1103/PhysRevX.15.011009Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit GatesMichael PeperYiyi LiDaniel Y. KnappMila BileskaShuo MaGenyue LiuPai PengBichen ZhangSebastian P. HorvathAlex P. BurgersJeff D. ThompsonHighly excited Rydberg states and their interactions play an important role in quantum computing and simulation. These properties can be predicted accurately for alkali atoms with simple Rydberg level structures. However, an extension of these methods to more complex atoms such as alkaline-earth atoms has not been demonstrated or experimentally validated. Here, we present multichannel quantum defect models for highly excited ^{174}Yb and ^{171}Yb Rydberg states with L≤2. The models are developed using a combination of existing literature data and new, high-precision laser and microwave spectroscopy in an atomic beam, and validated by detailed comparison with experimentally measured Stark shifts and magnetic moments. We then use these models to compute interaction potentials between two Yb atoms, and find excellent agreement with direct measurements in an optical tweezer array. From the computed interaction potential, we identify an anomalous Förster resonance that likely degraded the fidelity of previous entangling gates in ^{171}Yb using F=3/2 Rydberg states. We then identify a more suitable F=1/2 state, and achieve a state-of-the-art controlled-z gate fidelity of F=0.994(1), with the remaining error fully explained by known sources. This work establishes a solid foundation for the continued development of quantum computing, simulation, and entanglement-enhanced metrology with Yb neutral atom arrays.http://doi.org/10.1103/PhysRevX.15.011009
spellingShingle Michael Peper
Yiyi Li
Daniel Y. Knapp
Mila Bileska
Shuo Ma
Genyue Liu
Pai Peng
Bichen Zhang
Sebastian P. Horvath
Alex P. Burgers
Jeff D. Thompson
Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
Physical Review X
title Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
title_full Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
title_fullStr Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
title_full_unstemmed Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
title_short Spectroscopy and Modeling of ^{171}Yb Rydberg States for High-Fidelity Two-Qubit Gates
title_sort spectroscopy and modeling of 171 yb rydberg states for high fidelity two qubit gates
url http://doi.org/10.1103/PhysRevX.15.011009
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