Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction

To determine the optimal conditions of pressurized liquid extraction (PLE) and microwave-assisted extraction (MAE) of polyphenols from black chokeberry leaves (BCL), temperature, time and sample-to-solvent ratio (SSR) were varied to obtain maximum polyphenols yield. The extracts were analyzed for to...

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Main Authors: Maja Repajić, Ivona Elez Garofulić, Ena Cegledi, Erika Dobroslavić, Sandra Pedisić, Ksenija Durgo, Ana Huđek Turković, Jasna Mrvčić, Karla Hanousek Čiča, Verica Dragović-Uzelac
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Language:English
Published: MDPI AG 2024-12-01
Series:Antioxidants
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Online Access:https://www.mdpi.com/2076-3921/13/12/1582
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author Maja Repajić
Ivona Elez Garofulić
Ena Cegledi
Erika Dobroslavić
Sandra Pedisić
Ksenija Durgo
Ana Huđek Turković
Jasna Mrvčić
Karla Hanousek Čiča
Verica Dragović-Uzelac
author_facet Maja Repajić
Ivona Elez Garofulić
Ena Cegledi
Erika Dobroslavić
Sandra Pedisić
Ksenija Durgo
Ana Huđek Turković
Jasna Mrvčić
Karla Hanousek Čiča
Verica Dragović-Uzelac
author_sort Maja Repajić
collection DOAJ
description To determine the optimal conditions of pressurized liquid extraction (PLE) and microwave-assisted extraction (MAE) of polyphenols from black chokeberry leaves (BCL), temperature, time and sample-to-solvent ratio (SSR) were varied to obtain maximum polyphenols yield. The extracts were analyzed for total polyphenols (TP) as well as individual ones (UPLC ESI MS<sup>2</sup>) and antioxidant capacity (FRAP, DPPH and ORAC). Moreover, the biological activity of the selected extracts was additionally determined. The optimal PLE and MAE conditions were 150 °C, 5 min extraction time and SSR 1:30 g/mL (TP 80.0 mg GAE/g dm), and 70 °C, extraction time 5 min and SSR 1:30 g/mL (TP 36.4 mg GAE/g dm), respectively. Both methods yielded similar polyphenol profiles (43 compounds) but differed quantitatively. MAE extracts contained more flavonols and phenolic acids, while PLE extracts had higher procyanidins and flavan-3-ols. Furthermore, the PLE extract exhibited a superior antioxidant capacity. This BCL extract also showed that it can protect against oxidative and DNA damage and can induce free radical formation and DNA damage, albeit at different doses. Moreover, it had a moderate antimicrobial activity against <i>S. aureus</i> and <i>B. subtilis</i>, while no antimicrobial activity was observed against Gram-negative bacteria as well as yeasts, lactic acid bacteria and molds.
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series Antioxidants
spelling doaj-art-a8b4e292294e4ae4bf985420bd22c13b2024-12-27T14:07:02ZengMDPI AGAntioxidants2076-39212024-12-011312158210.3390/antiox13121582Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted ExtractionMaja Repajić0Ivona Elez Garofulić1Ena Cegledi2Erika Dobroslavić3Sandra Pedisić4Ksenija Durgo5Ana Huđek Turković6Jasna Mrvčić7Karla Hanousek Čiča8Verica Dragović-Uzelac9University of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Dubrovnik, Department of Applied Ecology, Ćira Carića 4, 20000 Dubrovnik, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaUniversity of Zagreb, Faculty of Food Technology and Biotechnology, Pierottijeva 6, 10000 Zagreb, CroatiaTo determine the optimal conditions of pressurized liquid extraction (PLE) and microwave-assisted extraction (MAE) of polyphenols from black chokeberry leaves (BCL), temperature, time and sample-to-solvent ratio (SSR) were varied to obtain maximum polyphenols yield. The extracts were analyzed for total polyphenols (TP) as well as individual ones (UPLC ESI MS<sup>2</sup>) and antioxidant capacity (FRAP, DPPH and ORAC). Moreover, the biological activity of the selected extracts was additionally determined. The optimal PLE and MAE conditions were 150 °C, 5 min extraction time and SSR 1:30 g/mL (TP 80.0 mg GAE/g dm), and 70 °C, extraction time 5 min and SSR 1:30 g/mL (TP 36.4 mg GAE/g dm), respectively. Both methods yielded similar polyphenol profiles (43 compounds) but differed quantitatively. MAE extracts contained more flavonols and phenolic acids, while PLE extracts had higher procyanidins and flavan-3-ols. Furthermore, the PLE extract exhibited a superior antioxidant capacity. This BCL extract also showed that it can protect against oxidative and DNA damage and can induce free radical formation and DNA damage, albeit at different doses. Moreover, it had a moderate antimicrobial activity against <i>S. aureus</i> and <i>B. subtilis</i>, while no antimicrobial activity was observed against Gram-negative bacteria as well as yeasts, lactic acid bacteria and molds.https://www.mdpi.com/2076-3921/13/12/1582<i>Aronia melanocarpa</i> L.polyphenolsantioxidant capacitycytotoxicityantiproliferative activityDNA damage
spellingShingle Maja Repajić
Ivona Elez Garofulić
Ena Cegledi
Erika Dobroslavić
Sandra Pedisić
Ksenija Durgo
Ana Huđek Turković
Jasna Mrvčić
Karla Hanousek Čiča
Verica Dragović-Uzelac
Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
Antioxidants
<i>Aronia melanocarpa</i> L.
polyphenols
antioxidant capacity
cytotoxicity
antiproliferative activity
DNA damage
title Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
title_full Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
title_fullStr Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
title_full_unstemmed Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
title_short Bioactive and Biological Potential of Black Chokeberry Leaves Under the Influence of Pressurized Liquid Extraction and Microwave-Assisted Extraction
title_sort bioactive and biological potential of black chokeberry leaves under the influence of pressurized liquid extraction and microwave assisted extraction
topic <i>Aronia melanocarpa</i> L.
polyphenols
antioxidant capacity
cytotoxicity
antiproliferative activity
DNA damage
url https://www.mdpi.com/2076-3921/13/12/1582
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