The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity

Abstract Cholinergic treatments with an emphasis on M1 muscarinic acetylcholine receptor (mAChR) agonists as potential modulating agents are a new approach in Alzheimer’s disease (AD) therapy. In previous research, we designed and characterized novel thiazolidine-2,4-dione (TZD)-derived compounds th...

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Main Authors: Maryam Taheri, Maryam Afzali Mehr, Hossein Ghafouri
Format: Article
Language:English
Published: Nature Portfolio 2024-11-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-024-80102-0
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author Maryam Taheri
Maryam Afzali Mehr
Hossein Ghafouri
author_facet Maryam Taheri
Maryam Afzali Mehr
Hossein Ghafouri
author_sort Maryam Taheri
collection DOAJ
description Abstract Cholinergic treatments with an emphasis on M1 muscarinic acetylcholine receptor (mAChR) agonists as potential modulating agents are a new approach in Alzheimer’s disease (AD) therapy. In previous research, we designed and characterized novel thiazolidine-2,4-dione (TZD)-derived compounds that possess anti-AD properties and enhance the expression of mAChRM1 in rats. This study evaluated a novel orthosteric agonist of mAChRM1 from related pathways that has shown promising anti-Alzheimer’s disease activity. PC12 cells were exposed to various concentrations of TZ4M before they were exposed to scopolamine (3 µM). Immunocytochemistry and western blot analyses revealed that TZ4M increased the expression of mAChRM1 in differentiated cells induced by scopolamine-treated PC12 cells. The results showed that TZ4M (3 and 5 µM) markedly upregulated PKC and ChAT protein expression, and the cells were significantly protected against increased ROS levels followed by neuronal cell loss, as evidenced by the MTT assay. TUNEL staining indicated that TZ4M impeded the shaping of apoptotic bodies. Analysis of the amino acid sequences of the ligand–protein binding site indicated that TZ4M is bound to the orthosteric site (acetylcholine site). This study revealed that TZ4M, a derivative of TZD, effectively protects against scopolamine-induced damage. TZ4M, a novel mACRM1 orthosteric agonist, is promising for treating AD.
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spelling doaj-art-a841dbea0aba45589ff6543222025fcf2024-11-24T12:26:35ZengNature PortfolioScientific Reports2045-23222024-11-0114111310.1038/s41598-024-80102-0The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activityMaryam Taheri0Maryam Afzali Mehr1Hossein Ghafouri2Department of Biology, Faculty of Basic Sciences, University of GuilanDepartment of Biology, Faculty of Basic Sciences, University of GuilanDepartment of Biology, Faculty of Basic Sciences, University of GuilanAbstract Cholinergic treatments with an emphasis on M1 muscarinic acetylcholine receptor (mAChR) agonists as potential modulating agents are a new approach in Alzheimer’s disease (AD) therapy. In previous research, we designed and characterized novel thiazolidine-2,4-dione (TZD)-derived compounds that possess anti-AD properties and enhance the expression of mAChRM1 in rats. This study evaluated a novel orthosteric agonist of mAChRM1 from related pathways that has shown promising anti-Alzheimer’s disease activity. PC12 cells were exposed to various concentrations of TZ4M before they were exposed to scopolamine (3 µM). Immunocytochemistry and western blot analyses revealed that TZ4M increased the expression of mAChRM1 in differentiated cells induced by scopolamine-treated PC12 cells. The results showed that TZ4M (3 and 5 µM) markedly upregulated PKC and ChAT protein expression, and the cells were significantly protected against increased ROS levels followed by neuronal cell loss, as evidenced by the MTT assay. TUNEL staining indicated that TZ4M impeded the shaping of apoptotic bodies. Analysis of the amino acid sequences of the ligand–protein binding site indicated that TZ4M is bound to the orthosteric site (acetylcholine site). This study revealed that TZ4M, a derivative of TZD, effectively protects against scopolamine-induced damage. TZ4M, a novel mACRM1 orthosteric agonist, is promising for treating AD.https://doi.org/10.1038/s41598-024-80102-0Alzheimer’s disease (AD)Cholinergic pathwayAgonistM1 muscarinic acetylcholine receptorOrthosteric siteThiazolidine-2,4-dione (TZD)
spellingShingle Maryam Taheri
Maryam Afzali Mehr
Hossein Ghafouri
The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
Scientific Reports
Alzheimer’s disease (AD)
Cholinergic pathway
Agonist
M1 muscarinic acetylcholine receptor
Orthosteric site
Thiazolidine-2,4-dione (TZD)
title The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
title_full The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
title_fullStr The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
title_full_unstemmed The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
title_short The novel orthosteric agonist M1 muscarinic acetylcholine receptor reveals anti-Alzheimer’s disease activity
title_sort novel orthosteric agonist m1 muscarinic acetylcholine receptor reveals anti alzheimer s disease activity
topic Alzheimer’s disease (AD)
Cholinergic pathway
Agonist
M1 muscarinic acetylcholine receptor
Orthosteric site
Thiazolidine-2,4-dione (TZD)
url https://doi.org/10.1038/s41598-024-80102-0
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