The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration

This study aims to determine the effect of nanoparticles (NPs), namely graphene oxide (GO), multilayer carbon tubes (MWCNTs + Fe), magnetite (Fe3O4) and in situ forming brushite (DCPD) in chitosan (CS) based matrices on the cytotoxicity, Pregabalin (PG) release, and in vivo behavior of mechanically...

Full description

Saved in:
Bibliographic Details
Main Authors: Liudmyla Sukhodub, Mariia Kumeda, Leonid Sukhodub, Oleksandr Tsyndrenko, Oleksandr Petrenko, Volodymyr Prokopiuk, Anton Tkachenko
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Carbohydrate Polymer Technologies and Applications
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2666893924001087
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846125038696136704
author Liudmyla Sukhodub
Mariia Kumeda
Leonid Sukhodub
Oleksandr Tsyndrenko
Oleksandr Petrenko
Volodymyr Prokopiuk
Anton Tkachenko
author_facet Liudmyla Sukhodub
Mariia Kumeda
Leonid Sukhodub
Oleksandr Tsyndrenko
Oleksandr Petrenko
Volodymyr Prokopiuk
Anton Tkachenko
author_sort Liudmyla Sukhodub
collection DOAJ
description This study aims to determine the effect of nanoparticles (NPs), namely graphene oxide (GO), multilayer carbon tubes (MWCNTs + Fe), magnetite (Fe3O4) and in situ forming brushite (DCPD) in chitosan (CS) based matrices on the cytotoxicity, Pregabalin (PG) release, and in vivo behavior of mechanically stabilized conductive nerve conduits (NCs). NPs change the composites’ hydrophilicity in the order: DCPD (46.8) < MWCNT (54.21) ∼ Fe3O4 (54.44) < GO (65.99) and the water contact angle (47–66°) corresponds to the conditions of cell adhesion. NPs of ≤ 150 μg/ml reduce cell adhesion but don't trigger oxidative stress and toxic effects. Magnetite NPs of 300 µg/ml promote apoptosis in nerve cells. The introduction of PG at stage b during the DCPD formation provides the drug release kinetics closest to the zero-order kinetic model. The most electrically conductive GO- and MWCNTs + Fe - containing NCs have a prolonged biodegradation period of about 6 months, which makes them promising for the regeneration of damaged peripheral nerves in humans.
format Article
id doaj-art-9d924fb8b1b94f93ae5ffaa72b2490d3
institution Kabale University
issn 2666-8939
language English
publishDate 2024-12-01
publisher Elsevier
record_format Article
series Carbohydrate Polymer Technologies and Applications
spelling doaj-art-9d924fb8b1b94f93ae5ffaa72b2490d32024-12-13T11:06:16ZengElsevierCarbohydrate Polymer Technologies and Applications2666-89392024-12-018100528The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regenerationLiudmyla Sukhodub0Mariia Kumeda1Leonid Sukhodub2Oleksandr Tsyndrenko3Oleksandr Petrenko4Volodymyr Prokopiuk5Anton Tkachenko6Sumy State University, Sumy, 40007, Ukraine; Corresponding author.Sumy State University, Sumy, 40007, UkraineSumy State University, Sumy, 40007, UkraineSumy State University, Sumy, 40007, UkraineDepartment of Cryobiochemistry, Institute for Problems of Cryobiology and Cryomedicine of the National Academy of Sciences of Ukraine, Kharkiv, 61015, UkraineResearch Institute of Experimental and Clinical Medicine, Kharkiv National Medical University, Kharkiv, 61022, Ukraine; Department of Cryobiochemistry, Institute for Problems of Cryobiology and Cryomedicine of the National Academy of Sciences of Ukraine, Kharkiv, 61015, UkraineDepartment of Cryobiochemistry, Institute for Problems of Cryobiology and Cryomedicine of the National Academy of Sciences of Ukraine, Kharkiv, 61015, UkraineThis study aims to determine the effect of nanoparticles (NPs), namely graphene oxide (GO), multilayer carbon tubes (MWCNTs + Fe), magnetite (Fe3O4) and in situ forming brushite (DCPD) in chitosan (CS) based matrices on the cytotoxicity, Pregabalin (PG) release, and in vivo behavior of mechanically stabilized conductive nerve conduits (NCs). NPs change the composites’ hydrophilicity in the order: DCPD (46.8) < MWCNT (54.21) ∼ Fe3O4 (54.44) < GO (65.99) and the water contact angle (47–66°) corresponds to the conditions of cell adhesion. NPs of ≤ 150 μg/ml reduce cell adhesion but don't trigger oxidative stress and toxic effects. Magnetite NPs of 300 µg/ml promote apoptosis in nerve cells. The introduction of PG at stage b during the DCPD formation provides the drug release kinetics closest to the zero-order kinetic model. The most electrically conductive GO- and MWCNTs + Fe - containing NCs have a prolonged biodegradation period of about 6 months, which makes them promising for the regeneration of damaged peripheral nerves in humans.http://www.sciencedirect.com/science/article/pii/S2666893924001087ChitosanCarbon nanoparticlesCytotoxicityDrug releaseNerve conduitIn vivo biocompatibility
spellingShingle Liudmyla Sukhodub
Mariia Kumeda
Leonid Sukhodub
Oleksandr Tsyndrenko
Oleksandr Petrenko
Volodymyr Prokopiuk
Anton Tkachenko
The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
Carbohydrate Polymer Technologies and Applications
Chitosan
Carbon nanoparticles
Cytotoxicity
Drug release
Nerve conduit
In vivo biocompatibility
title The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
title_full The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
title_fullStr The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
title_full_unstemmed The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
title_short The effect of carbon and magnetic nanoparticles on the properties of chitosan-based neural tubes: Cytotoxicity, drug release, In Vivo nerve regeneration
title_sort effect of carbon and magnetic nanoparticles on the properties of chitosan based neural tubes cytotoxicity drug release in vivo nerve regeneration
topic Chitosan
Carbon nanoparticles
Cytotoxicity
Drug release
Nerve conduit
In vivo biocompatibility
url http://www.sciencedirect.com/science/article/pii/S2666893924001087
work_keys_str_mv AT liudmylasukhodub theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT mariiakumeda theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT leonidsukhodub theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT oleksandrtsyndrenko theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT oleksandrpetrenko theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT volodymyrprokopiuk theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT antontkachenko theeffectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT liudmylasukhodub effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT mariiakumeda effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT leonidsukhodub effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT oleksandrtsyndrenko effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT oleksandrpetrenko effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT volodymyrprokopiuk effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration
AT antontkachenko effectofcarbonandmagneticnanoparticlesonthepropertiesofchitosanbasedneuraltubescytotoxicitydrugreleaseinvivonerveregeneration