Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries

Highlights NaTFSI/SUL:OTE:FEC facilitates the formation of S, N-rich, dense and robust cathode–electrolyte interphase on NaNMF cathode, which improves the cycling stability under high voltage. By utilizing NaTFSI/SUL:OTE:FEC, the Na||NaNMF batteries achieved an impressive retention of 81.15% after 4...

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Main Authors: Xuanlong He, Jie Peng, Qingyun Lin, Meng Li, Weibin Chen, Pei Liu, Tao Huang, Zhencheng Huang, Yuying Liu, Jiaojiao Deng, Shenghua Ye, Xuming Yang, Xiangzhong Ren, Xiaoping Ouyang, Jianhong Liu, Biwei Xiao, Jiangtao Hu, Qianling Zhang
Format: Article
Language:English
Published: SpringerOpen 2024-10-01
Series:Nano-Micro Letters
Subjects:
Online Access:https://doi.org/10.1007/s40820-024-01546-7
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author Xuanlong He
Jie Peng
Qingyun Lin
Meng Li
Weibin Chen
Pei Liu
Tao Huang
Zhencheng Huang
Yuying Liu
Jiaojiao Deng
Shenghua Ye
Xuming Yang
Xiangzhong Ren
Xiaoping Ouyang
Jianhong Liu
Biwei Xiao
Jiangtao Hu
Qianling Zhang
author_facet Xuanlong He
Jie Peng
Qingyun Lin
Meng Li
Weibin Chen
Pei Liu
Tao Huang
Zhencheng Huang
Yuying Liu
Jiaojiao Deng
Shenghua Ye
Xuming Yang
Xiangzhong Ren
Xiaoping Ouyang
Jianhong Liu
Biwei Xiao
Jiangtao Hu
Qianling Zhang
author_sort Xuanlong He
collection DOAJ
description Highlights NaTFSI/SUL:OTE:FEC facilitates the formation of S, N-rich, dense and robust cathode–electrolyte interphase on NaNMF cathode, which improves the cycling stability under high voltage. By utilizing NaTFSI/SUL:OTE:FEC, the Na||NaNMF batteries achieved an impressive retention of 81.15% after 400 cycles at 2 C with the cutoff voltage of 4.2 V. The study offers a reference for the utilization of sulfolane-based electrolytes in sodium-ion batteries (SIBs), while the nonflammability of the NaTFSI/SUL:OTE:FEC enhances the safety of SIBs.
format Article
id doaj-art-9b4d1fb6543743b582611b73ece50f3f
institution Kabale University
issn 2311-6706
2150-5551
language English
publishDate 2024-10-01
publisher SpringerOpen
record_format Article
series Nano-Micro Letters
spelling doaj-art-9b4d1fb6543743b582611b73ece50f3f2025-08-20T04:03:01ZengSpringerOpenNano-Micro Letters2311-67062150-55512024-10-0117111910.1007/s40820-024-01546-7Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion BatteriesXuanlong He0Jie Peng1Qingyun Lin2Meng Li3Weibin Chen4Pei Liu5Tao Huang6Zhencheng Huang7Yuying Liu8Jiaojiao Deng9Shenghua Ye10Xuming Yang11Xiangzhong Ren12Xiaoping Ouyang13Jianhong Liu14Biwei Xiao15Jiangtao Hu16Qianling Zhang17Graphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityCenter of Electron Microscopy, State Key Laboratory of Silicon and Advanced Semiconductor Materials, School of Materials Science and Engineering, Zhejiang UniversityGRINM (Guangdong) Research Institute for Advanced Materials and TechnologyGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityCollege of Energy Engineering, Zhejiang UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGRINM (Guangdong) Research Institute for Advanced Materials and TechnologyGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityGraphene Composite Research Center, College of Chemistry and Environmental Engineering, Shenzhen UniversityHighlights NaTFSI/SUL:OTE:FEC facilitates the formation of S, N-rich, dense and robust cathode–electrolyte interphase on NaNMF cathode, which improves the cycling stability under high voltage. By utilizing NaTFSI/SUL:OTE:FEC, the Na||NaNMF batteries achieved an impressive retention of 81.15% after 400 cycles at 2 C with the cutoff voltage of 4.2 V. The study offers a reference for the utilization of sulfolane-based electrolytes in sodium-ion batteries (SIBs), while the nonflammability of the NaTFSI/SUL:OTE:FEC enhances the safety of SIBs.https://doi.org/10.1007/s40820-024-01546-7Sodium-ion batteriesSulfolane-based electrolyteHigh voltageLayered oxide cathodeFlame retardant
spellingShingle Xuanlong He
Jie Peng
Qingyun Lin
Meng Li
Weibin Chen
Pei Liu
Tao Huang
Zhencheng Huang
Yuying Liu
Jiaojiao Deng
Shenghua Ye
Xuming Yang
Xiangzhong Ren
Xiaoping Ouyang
Jianhong Liu
Biwei Xiao
Jiangtao Hu
Qianling Zhang
Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
Nano-Micro Letters
Sodium-ion batteries
Sulfolane-based electrolyte
High voltage
Layered oxide cathode
Flame retardant
title Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
title_full Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
title_fullStr Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
title_full_unstemmed Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
title_short Sulfolane-Based Flame-Retardant Electrolyte for High-Voltage Sodium-Ion Batteries
title_sort sulfolane based flame retardant electrolyte for high voltage sodium ion batteries
topic Sodium-ion batteries
Sulfolane-based electrolyte
High voltage
Layered oxide cathode
Flame retardant
url https://doi.org/10.1007/s40820-024-01546-7
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