Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin

The goal of the present study was to clarify the nature of benzene forming in base catalyzed side-chain alkylation of toluene with methanol. Benzene formation has been observed as a primary product in the very beginning of conversion of toluene/methanol mixture on the basic catalysts. Dynamics of al...

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Main Authors: Yuliya G Voloshyna, Olexandra P Pertko, Serhiy V Konovalov, Lyubov K Patrylak
Format: Article
Language:English
Published: SAGE Publishing 2017-09-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1177/0263617417705963
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author Yuliya G Voloshyna
Olexandra P Pertko
Serhiy V Konovalov
Lyubov K Patrylak
author_facet Yuliya G Voloshyna
Olexandra P Pertko
Serhiy V Konovalov
Lyubov K Patrylak
author_sort Yuliya G Voloshyna
collection DOAJ
description The goal of the present study was to clarify the nature of benzene forming in base catalyzed side-chain alkylation of toluene with methanol. Benzene formation has been observed as a primary product in the very beginning of conversion of toluene/methanol mixture on the basic catalysts. Dynamics of alteration of its content in reaction products has been explained. The nature of sites responsible for benzene formation has been suggested considering conception concerning preferences in toluene or methanol adsorption on the catalyst of different basicity. Toluene has been concluded to be a raw material for benzene formation.
format Article
id doaj-art-99734ae8b3d4447bb9cf5403aaad7b18
institution Kabale University
issn 0263-6174
2048-4038
language English
publishDate 2017-09-01
publisher SAGE Publishing
record_format Article
series Adsorption Science & Technology
spelling doaj-art-99734ae8b3d4447bb9cf5403aaad7b182025-01-02T21:31:19ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382017-09-013510.1177/0263617417705963Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable originYuliya G VoloshynaOlexandra P PertkoSerhiy V KonovalovLyubov K PatrylakThe goal of the present study was to clarify the nature of benzene forming in base catalyzed side-chain alkylation of toluene with methanol. Benzene formation has been observed as a primary product in the very beginning of conversion of toluene/methanol mixture on the basic catalysts. Dynamics of alteration of its content in reaction products has been explained. The nature of sites responsible for benzene formation has been suggested considering conception concerning preferences in toluene or methanol adsorption on the catalyst of different basicity. Toluene has been concluded to be a raw material for benzene formation.https://doi.org/10.1177/0263617417705963
spellingShingle Yuliya G Voloshyna
Olexandra P Pertko
Serhiy V Konovalov
Lyubov K Patrylak
Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
Adsorption Science & Technology
title Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
title_full Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
title_fullStr Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
title_full_unstemmed Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
title_short Benzene as a by-product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
title_sort benzene as a by product of toluene with methanol transformation on the basic zeolite catalysts and its presumable origin
url https://doi.org/10.1177/0263617417705963
work_keys_str_mv AT yuliyagvoloshyna benzeneasabyproductoftoluenewithmethanoltransformationonthebasiczeolitecatalystsanditspresumableorigin
AT olexandrappertko benzeneasabyproductoftoluenewithmethanoltransformationonthebasiczeolitecatalystsanditspresumableorigin
AT serhiyvkonovalov benzeneasabyproductoftoluenewithmethanoltransformationonthebasiczeolitecatalystsanditspresumableorigin
AT lyubovkpatrylak benzeneasabyproductoftoluenewithmethanoltransformationonthebasiczeolitecatalystsanditspresumableorigin