Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite

This study emphasizes the synthesis of nickel oxide (NiOx + C) nanoparticles with varied graphite (C) proportions (1%, 2.5%, 5%, 7.5%, and 10%) using Aloe-Vera natural extract as a green reducing agent. Prepared NiOx + C nanostructures exhibited consistent X-ray diffraction patterns with no addition...

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Main Authors: A. K. Mahmud Hasan, D. K. Sarkar, M. S. Basar, Munira Sultana, Mohammad Junaebur Rashid, Mohammod Aminuzzaman, Md. Shahiduzzaman, Hamad F. Alharbi, Md. Akhtaruzzaman
Format: Article
Language:English
Published: Taylor & Francis Group 2024-12-01
Series:Journal of Taibah University for Science
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Online Access:https://www.tandfonline.com/doi/10.1080/16583655.2023.2298524
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author A. K. Mahmud Hasan
D. K. Sarkar
M. S. Basar
Munira Sultana
Mohammad Junaebur Rashid
Mohammod Aminuzzaman
Md. Shahiduzzaman
Hamad F. Alharbi
Md. Akhtaruzzaman
author_facet A. K. Mahmud Hasan
D. K. Sarkar
M. S. Basar
Munira Sultana
Mohammad Junaebur Rashid
Mohammod Aminuzzaman
Md. Shahiduzzaman
Hamad F. Alharbi
Md. Akhtaruzzaman
author_sort A. K. Mahmud Hasan
collection DOAJ
description This study emphasizes the synthesis of nickel oxide (NiOx + C) nanoparticles with varied graphite (C) proportions (1%, 2.5%, 5%, 7.5%, and 10%) using Aloe-Vera natural extract as a green reducing agent. Prepared NiOx + C nanostructures exhibited consistent X-ray diffraction patterns with no additional C peak, signifying enhanced interlayer spacing. The crystalline size (Dp) decreased from 27 nm to 20 nm with an increase in the amount of carbon (C). The determined bandgap (Eg) was 2 eV higher than bulk material due to formation extra energy level at defect sites. The shoulder peak at 1620 cm−1 agrees with the disorder-induced band from C and second-order bands of C at about 2700 cm−1 for NiOx + C. FESEM images confirm the hexagonal morphology. Not much particle aggregation was observed except for 10% C content. The selected area electron diffraction (SAED) confirms the existence of NiOx crystalline orientations including planes (111), (200), (220), (311), and (222).
format Article
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institution Kabale University
issn 1658-3655
language English
publishDate 2024-12-01
publisher Taylor & Francis Group
record_format Article
series Journal of Taibah University for Science
spelling doaj-art-927a0ce7acf6497d9affc0347e3429352024-12-17T11:38:48ZengTaylor & Francis GroupJournal of Taibah University for Science1658-36552024-12-0118110.1080/16583655.2023.2298524Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C compositeA. K. Mahmud Hasan0D. K. Sarkar1M. S. Basar2Munira Sultana3Mohammad Junaebur Rashid4Mohammod Aminuzzaman5Md. Shahiduzzaman6Hamad F. Alharbi7Md. Akhtaruzzaman8Bangladesh Council of Scientific and Industrial Research (BCSIR), Dhaka, BangladeshSolar Energy Research Institute, The National University of Malaysia, Bangi, MalaysiaBangladesh Council of Scientific and Industrial Research (BCSIR), Dhaka, BangladeshBangladesh Council of Scientific and Industrial Research (BCSIR), Dhaka, BangladeshDepartment of Electrical and Electronic Engineering, University of Dhaka, Dhaka, BangladeshDepartment of Chemical Science, Faculty of Science, Universiti Tunku Abdul Rahman, Perak Campus, Jalan Universiti, Kampar, MalaysiaNanomaterials Research Institute, Kanazawa University, Kanazawa, JapanMechanical Engineering Department, College of Engineering, King Saud University, Riyadh, Saudi ArabiaSolar Energy Research Institute, The National University of Malaysia, Bangi, MalaysiaThis study emphasizes the synthesis of nickel oxide (NiOx + C) nanoparticles with varied graphite (C) proportions (1%, 2.5%, 5%, 7.5%, and 10%) using Aloe-Vera natural extract as a green reducing agent. Prepared NiOx + C nanostructures exhibited consistent X-ray diffraction patterns with no additional C peak, signifying enhanced interlayer spacing. The crystalline size (Dp) decreased from 27 nm to 20 nm with an increase in the amount of carbon (C). The determined bandgap (Eg) was 2 eV higher than bulk material due to formation extra energy level at defect sites. The shoulder peak at 1620 cm−1 agrees with the disorder-induced band from C and second-order bands of C at about 2700 cm−1 for NiOx + C. FESEM images confirm the hexagonal morphology. Not much particle aggregation was observed except for 10% C content. The selected area electron diffraction (SAED) confirms the existence of NiOx crystalline orientations including planes (111), (200), (220), (311), and (222).https://www.tandfonline.com/doi/10.1080/16583655.2023.2298524Nickel oxidegraphite alloyinggreen synthesisnatural complexing agent
spellingShingle A. K. Mahmud Hasan
D. K. Sarkar
M. S. Basar
Munira Sultana
Mohammad Junaebur Rashid
Mohammod Aminuzzaman
Md. Shahiduzzaman
Hamad F. Alharbi
Md. Akhtaruzzaman
Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
Journal of Taibah University for Science
Nickel oxide
graphite alloying
green synthesis
natural complexing agent
title Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
title_full Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
title_fullStr Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
title_full_unstemmed Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
title_short Effect of fractional graphite alloying on the properties of aloe-vera mediated green-synthesized NiOx-C composite
title_sort effect of fractional graphite alloying on the properties of aloe vera mediated green synthesized niox c composite
topic Nickel oxide
graphite alloying
green synthesis
natural complexing agent
url https://www.tandfonline.com/doi/10.1080/16583655.2023.2298524
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