Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material

In the present work, coal fly ash-derived mesoporous silica material (CFA-MS) has been successfully fabricated without employing any extra silica source. The obtained CFA-MS was characterized by Fourier transform infrared spectroscopy, nitrogen adsorption–desorption measurement, powder X-ray diffrac...

Full description

Saved in:
Bibliographic Details
Main Authors: Ning Yuan, Hui Cai, Tian Liu, Qi Huang, Xinling Zhang
Format: Article
Language:English
Published: SAGE Publishing 2019-05-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1177/0263617419827438
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1841563225892585472
author Ning Yuan
Hui Cai
Tian Liu
Qi Huang
Xinling Zhang
author_facet Ning Yuan
Hui Cai
Tian Liu
Qi Huang
Xinling Zhang
author_sort Ning Yuan
collection DOAJ
description In the present work, coal fly ash-derived mesoporous silica material (CFA-MS) has been successfully fabricated without employing any extra silica source. The obtained CFA-MS was characterized by Fourier transform infrared spectroscopy, nitrogen adsorption–desorption measurement, powder X-ray diffraction and transmission electron microscopy. Nitrogen adsorption–desorption measurement disclosed that CFA-MS possesses Brunauer–Emmett–Teller-specific surface area of 497 m 2 ·g −1 and pore volume of 0.49 cm 3 ·g −1 , respectively. Furthermore, CFA-MS was evaluated for the adsorptive removal of methylene blue from aqueous solution. Several influence parameters on the removal of methylene blue including contact time, pH, initial concentration and temperature were studied in detail. Moreover, Langmuir, Freundlich, Temkin and Dubinin-Radushkevich isotherm models were employed for interpretation of the adsorption process, while the pseudo-first-order and pseudo-second-order kinetics equations were applied to investigate the adsorption kinetics. Results in the current work demonstrate that CFA-MS can be used as an efficient adsorbent for methylene blue removal.
format Article
id doaj-art-868743422dfb4d38b4a453c1532aebec
institution Kabale University
issn 0263-6174
2048-4038
language English
publishDate 2019-05-01
publisher SAGE Publishing
record_format Article
series Adsorption Science & Technology
spelling doaj-art-868743422dfb4d38b4a453c1532aebec2025-01-03T00:10:25ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382019-05-013710.1177/0263617419827438Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica materialNing YuanHui CaiTian LiuQi HuangXinling ZhangIn the present work, coal fly ash-derived mesoporous silica material (CFA-MS) has been successfully fabricated without employing any extra silica source. The obtained CFA-MS was characterized by Fourier transform infrared spectroscopy, nitrogen adsorption–desorption measurement, powder X-ray diffraction and transmission electron microscopy. Nitrogen adsorption–desorption measurement disclosed that CFA-MS possesses Brunauer–Emmett–Teller-specific surface area of 497 m 2 ·g −1 and pore volume of 0.49 cm 3 ·g −1 , respectively. Furthermore, CFA-MS was evaluated for the adsorptive removal of methylene blue from aqueous solution. Several influence parameters on the removal of methylene blue including contact time, pH, initial concentration and temperature were studied in detail. Moreover, Langmuir, Freundlich, Temkin and Dubinin-Radushkevich isotherm models were employed for interpretation of the adsorption process, while the pseudo-first-order and pseudo-second-order kinetics equations were applied to investigate the adsorption kinetics. Results in the current work demonstrate that CFA-MS can be used as an efficient adsorbent for methylene blue removal.https://doi.org/10.1177/0263617419827438
spellingShingle Ning Yuan
Hui Cai
Tian Liu
Qi Huang
Xinling Zhang
Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
Adsorption Science & Technology
title Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
title_full Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
title_fullStr Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
title_full_unstemmed Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
title_short Adsorptive removal of methylene blue from aqueous solution using coal fly ash-derived mesoporous silica material
title_sort adsorptive removal of methylene blue from aqueous solution using coal fly ash derived mesoporous silica material
url https://doi.org/10.1177/0263617419827438
work_keys_str_mv AT ningyuan adsorptiveremovalofmethylenebluefromaqueoussolutionusingcoalflyashderivedmesoporoussilicamaterial
AT huicai adsorptiveremovalofmethylenebluefromaqueoussolutionusingcoalflyashderivedmesoporoussilicamaterial
AT tianliu adsorptiveremovalofmethylenebluefromaqueoussolutionusingcoalflyashderivedmesoporoussilicamaterial
AT qihuang adsorptiveremovalofmethylenebluefromaqueoussolutionusingcoalflyashderivedmesoporoussilicamaterial
AT xinlingzhang adsorptiveremovalofmethylenebluefromaqueoussolutionusingcoalflyashderivedmesoporoussilicamaterial