Green solvent extraction of health boosting phenolics from pigeon pea husk

Abstract The optimization of phenolic compound extraction from pigeon pea (Cajanus cajan L.) husk was explored by manipulating three key process variables: aqueous ethanol concentration (20–60% v/v), extraction temperature (30–60 °C), and extraction time (2–6 h). Utilizing a Box-Behnken design under...

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Main Authors: Deepika Goswami, Manju Bala, D. Mridula, Rajesh Kumar Vishwakarma, P. N. Guru
Format: Article
Language:English
Published: Nature Portfolio 2025-08-01
Series:Scientific Reports
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Online Access:https://doi.org/10.1038/s41598-025-14197-4
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author Deepika Goswami
Manju Bala
D. Mridula
Rajesh Kumar Vishwakarma
P. N. Guru
author_facet Deepika Goswami
Manju Bala
D. Mridula
Rajesh Kumar Vishwakarma
P. N. Guru
author_sort Deepika Goswami
collection DOAJ
description Abstract The optimization of phenolic compound extraction from pigeon pea (Cajanus cajan L.) husk was explored by manipulating three key process variables: aqueous ethanol concentration (20–60% v/v), extraction temperature (30–60 °C), and extraction time (2–6 h). Utilizing a Box-Behnken design under Response Surface Methodology (RSM), we meticulously optimized these variables to maximize extract yield, total phenolic content, and DPPH radical scavenging activity. The ideal extraction conditions determined via desirability function analysis were found to be 41.83% (v/v) ethanol concentration, 59.36 °C extraction temperature, and 6 h extraction time. These parameters yielded an impressive 9.67 ± 0.02% extract yield, 47.99 ± 0.60 mg GAE/g total phenolic content, and 51.24 ± 0.43% DPPH radical scavenging activity, closely aligning with predicted values. LC-MS (ESI-Q-TOF) metabolite profiling of the optimized extract revealed a rich presence of flavonoids, alkaloids, terpenoids, lignans, phenols, xanthones, and glycosides. This study underscores the valorisation potential of pigeon pea husk—a typically discarded by-product—for sustainable extraction of valuable phenolic compounds under optimal conditions.
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spelling doaj-art-7f6a97c44d9c4ee8b6825d7d5282a9052025-08-20T04:03:12ZengNature PortfolioScientific Reports2045-23222025-08-0115111010.1038/s41598-025-14197-4Green solvent extraction of health boosting phenolics from pigeon pea huskDeepika Goswami0Manju Bala1D. Mridula2Rajesh Kumar Vishwakarma3P. N. Guru4Food Grains and Oilseeds Processing Division, ICAR-Central Institute of Post Harvest Engineering and TechnologyFood Grains and Oilseeds Processing Division, ICAR-Central Institute of Post Harvest Engineering and TechnologyFood Grains and Oilseeds Processing Division, ICAR-Central Institute of Post Harvest Engineering and TechnologyFood Grains and Oilseeds Processing Division, ICAR-Central Institute of Post Harvest Engineering and TechnologyFood Grains and Oilseeds Processing Division, ICAR-Central Institute of Post Harvest Engineering and TechnologyAbstract The optimization of phenolic compound extraction from pigeon pea (Cajanus cajan L.) husk was explored by manipulating three key process variables: aqueous ethanol concentration (20–60% v/v), extraction temperature (30–60 °C), and extraction time (2–6 h). Utilizing a Box-Behnken design under Response Surface Methodology (RSM), we meticulously optimized these variables to maximize extract yield, total phenolic content, and DPPH radical scavenging activity. The ideal extraction conditions determined via desirability function analysis were found to be 41.83% (v/v) ethanol concentration, 59.36 °C extraction temperature, and 6 h extraction time. These parameters yielded an impressive 9.67 ± 0.02% extract yield, 47.99 ± 0.60 mg GAE/g total phenolic content, and 51.24 ± 0.43% DPPH radical scavenging activity, closely aligning with predicted values. LC-MS (ESI-Q-TOF) metabolite profiling of the optimized extract revealed a rich presence of flavonoids, alkaloids, terpenoids, lignans, phenols, xanthones, and glycosides. This study underscores the valorisation potential of pigeon pea husk—a typically discarded by-product—for sustainable extraction of valuable phenolic compounds under optimal conditions.https://doi.org/10.1038/s41598-025-14197-4Pigeon peaCajanus CajanHuskBy-productPhenolic compoundsRSM
spellingShingle Deepika Goswami
Manju Bala
D. Mridula
Rajesh Kumar Vishwakarma
P. N. Guru
Green solvent extraction of health boosting phenolics from pigeon pea husk
Scientific Reports
Pigeon pea
Cajanus Cajan
Husk
By-product
Phenolic compounds
RSM
title Green solvent extraction of health boosting phenolics from pigeon pea husk
title_full Green solvent extraction of health boosting phenolics from pigeon pea husk
title_fullStr Green solvent extraction of health boosting phenolics from pigeon pea husk
title_full_unstemmed Green solvent extraction of health boosting phenolics from pigeon pea husk
title_short Green solvent extraction of health boosting phenolics from pigeon pea husk
title_sort green solvent extraction of health boosting phenolics from pigeon pea husk
topic Pigeon pea
Cajanus Cajan
Husk
By-product
Phenolic compounds
RSM
url https://doi.org/10.1038/s41598-025-14197-4
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