Advances in regulating the electron spin effect toward electrocatalysis applications
Building highly reactive electrocatalysts is of great significance for addressing the energy crisis and developing green energy. Electrocatalytic reactions occur at the interface of catalysts, where the physicochemical properties of the catalyst surface play a dominant role. In particular, the elect...
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| Format: | Article |
| Language: | English |
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KeAi Communications Co. Ltd.
2025-01-01
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| Series: | eScience |
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| Online Access: | http://www.sciencedirect.com/science/article/pii/S266714172400048X |
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| author | Liu Lin Peiyuan Su Yiting Han Yunming Xu Qiao Ni Xinyue Zhang Peixun Xiong Zemin Sun Genban Sun Xuebo Chen |
| author_facet | Liu Lin Peiyuan Su Yiting Han Yunming Xu Qiao Ni Xinyue Zhang Peixun Xiong Zemin Sun Genban Sun Xuebo Chen |
| author_sort | Liu Lin |
| collection | DOAJ |
| description | Building highly reactive electrocatalysts is of great significance for addressing the energy crisis and developing green energy. Electrocatalytic reactions occur at the interface of catalysts, where the physicochemical properties of the catalyst surface play a dominant role. In particular, the electron spin behavior on the catalyst surface has a decisive impact on the catalytic reaction process. This review initially introduces the definition of electron spin and methods for spin manipulation. Furthermore, we summarize the advanced characterization methods of electron spin. Then, we review the latest research advancements on the spin effect in the oxygen reduction reaction, oxygen evolution reaction, carbon dioxide reduction reaction, and nitrogen reduction reaction. The catalytic mechanisms of spin manipulation in these four reactions are thoroughly discussed. Finally, we propose key directions for the future development of spin effects in the field of electrocatalysis. This review contributes to a deeper understanding of the micromechanisms in electrocatalytic reactions. |
| format | Article |
| id | doaj-art-6caa7488ae3f403294a60513683a114a |
| institution | Kabale University |
| issn | 2667-1417 |
| language | English |
| publishDate | 2025-01-01 |
| publisher | KeAi Communications Co. Ltd. |
| record_format | Article |
| series | eScience |
| spelling | doaj-art-6caa7488ae3f403294a60513683a114a2025-01-04T04:57:21ZengKeAi Communications Co. Ltd.eScience2667-14172025-01-0151100264Advances in regulating the electron spin effect toward electrocatalysis applicationsLiu Lin0Peiyuan Su1Yiting Han2Yunming Xu3Qiao Ni4Xinyue Zhang5Peixun Xiong6Zemin Sun7Genban Sun8Xuebo Chen9College of Arts and Sciences & Center for Advanced Materials Research, Beijing Normal University, Zhuhai 519087, China; Corresponding authors.Synchrotron Soleil, L'Orme des Merisiers, Saint-Aubin 91190, FranceCollege of Arts and Sciences & Center for Advanced Materials Research, Beijing Normal University, Zhuhai 519087, ChinaCollege of Arts and Sciences & Center for Advanced Materials Research, Beijing Normal University, Zhuhai 519087, ChinaCollege of Arts and Sciences & Center for Advanced Materials Research, Beijing Normal University, Zhuhai 519087, ChinaInstitute for Applied Materials (IAM), Karlsruhe Institute of Technology (KIT), Eggenstein-Leopoldshafen 76344, GermanyInorganic Chemistry I, Technische Universität Dresden, Bergstraße 66, Dresden 01069, GermanyCollege of Arts and Sciences & Center for Advanced Materials Research, Beijing Normal University, Zhuhai 519087, China; Corresponding authors.Beijing Key Laboratory of Energy Conversion and Storage Materials Institution, Key Laboratory of Theoretical and Computational Photochemistry of the Chinese Ministry of Education, College of Chemistry, Beijing Normal University, Beijing 100875, China; Corresponding authors.Beijing Key Laboratory of Energy Conversion and Storage Materials Institution, Key Laboratory of Theoretical and Computational Photochemistry of the Chinese Ministry of Education, College of Chemistry, Beijing Normal University, Beijing 100875, China; Corresponding authors.Building highly reactive electrocatalysts is of great significance for addressing the energy crisis and developing green energy. Electrocatalytic reactions occur at the interface of catalysts, where the physicochemical properties of the catalyst surface play a dominant role. In particular, the electron spin behavior on the catalyst surface has a decisive impact on the catalytic reaction process. This review initially introduces the definition of electron spin and methods for spin manipulation. Furthermore, we summarize the advanced characterization methods of electron spin. Then, we review the latest research advancements on the spin effect in the oxygen reduction reaction, oxygen evolution reaction, carbon dioxide reduction reaction, and nitrogen reduction reaction. The catalytic mechanisms of spin manipulation in these four reactions are thoroughly discussed. Finally, we propose key directions for the future development of spin effects in the field of electrocatalysis. This review contributes to a deeper understanding of the micromechanisms in electrocatalytic reactions.http://www.sciencedirect.com/science/article/pii/S266714172400048XElectron spin effectSpin catalysisRegulating strategiesElectrocatalysis |
| spellingShingle | Liu Lin Peiyuan Su Yiting Han Yunming Xu Qiao Ni Xinyue Zhang Peixun Xiong Zemin Sun Genban Sun Xuebo Chen Advances in regulating the electron spin effect toward electrocatalysis applications eScience Electron spin effect Spin catalysis Regulating strategies Electrocatalysis |
| title | Advances in regulating the electron spin effect toward electrocatalysis applications |
| title_full | Advances in regulating the electron spin effect toward electrocatalysis applications |
| title_fullStr | Advances in regulating the electron spin effect toward electrocatalysis applications |
| title_full_unstemmed | Advances in regulating the electron spin effect toward electrocatalysis applications |
| title_short | Advances in regulating the electron spin effect toward electrocatalysis applications |
| title_sort | advances in regulating the electron spin effect toward electrocatalysis applications |
| topic | Electron spin effect Spin catalysis Regulating strategies Electrocatalysis |
| url | http://www.sciencedirect.com/science/article/pii/S266714172400048X |
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