Enzymatic Hydrolysis of Pretreated Miscanthus Biomass

Forests being mostly non-renewable, miscanthus seems to be a promising alternative energy resource. This study investigates the enzymatic hydrolysis of pretreated miscanthus biomass. The research featured Miscanthus sinensis Strictus biomass. The methods included raw material pretreatment, enzymatic...

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Main Authors: Olga B. Kalashnikova, Ekaterina A. Budenkova, Elena V. Ulrikh, Evgeny G. Chupakhin, Olga V. Kriger, Yakov A. Masiutin, Maria A. Smaga, Yulia S. Basova
Format: Article
Language:English
Published: Kemerovo State University 2022-06-01
Series:Техника и технология пищевых производств
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Online Access:https://fptt.ru/en/issues/20365/20375/
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author Olga B. Kalashnikova
Ekaterina A. Budenkova
Elena V. Ulrikh
Evgeny G. Chupakhin
Olga V. Kriger
Yakov A. Masiutin
Maria A. Smaga
Yulia S. Basova
author_facet Olga B. Kalashnikova
Ekaterina A. Budenkova
Elena V. Ulrikh
Evgeny G. Chupakhin
Olga V. Kriger
Yakov A. Masiutin
Maria A. Smaga
Yulia S. Basova
author_sort Olga B. Kalashnikova
collection DOAJ
description Forests being mostly non-renewable, miscanthus seems to be a promising alternative energy resource. This study investigates the enzymatic hydrolysis of pretreated miscanthus biomass. The research featured Miscanthus sinensis Strictus biomass. The methods included raw material pretreatment, enzymatic hydrolysis, matrix-assisted laser desorption ionization time-of-flight mass spectrometry (MALDI-TOF) of monosaccharide residues, and nuclear magnetic resonance (1H NMR) spectrometry of non-hydrolyzed lignin. A hammer mill with a particle size of 0.2–0.3 mm proved to be effective for preliminary mechanical processing of miscanthus. This type of treatment provided the maximal yield of carbohydrate-containing biomass (62.33 ± 1.87%). The optimal multi-enzyme composition included Cellulase Ultra obtained from Trichoderma reeseii, xylanase obtained from Thermomyces lanuginosus, and β-gluconase obtained from Myceliophtorafergusii. The fermentation temperature was 50 ± 1°C (72 ± 1 h). At these parameters, the conversion of holocellulose of miscanthus biomass was 96.0 ± 4.8%, and the yield of reducing substances was 97.00 ± 4.85%. The article introduces the optimal enzymatic hydrolysis parameters for pretreating Miscanthus sinensis Strictus biomass as a source of carbohydrate-containing substrates and describes their subsequent use for bacterial cellulose biosynthesis. The carbohydrate composition of hydrolysates included residual lignin, such polysaccharides as glucan and xylan, and various monosaccharides, namely arabinose, xylose, galactose, glucose, and uronic acids. Hydrolyzed miscanthus proved to be an effective renewable and environmentally friendly biodiesel.
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institution Kabale University
issn 2074-9414
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language English
publishDate 2022-06-01
publisher Kemerovo State University
record_format Article
series Техника и технология пищевых производств
spelling doaj-art-6c6ffb72a5294aeb967e09476ffa0ace2024-12-02T04:42:56ZengKemerovo State UniversityТехника и технология пищевых производств2074-94142313-17482022-06-0152225427010.21603/2074-9414-2022-2-2361Enzymatic Hydrolysis of Pretreated Miscanthus BiomassOlga B. Kalashnikova0https://orcid.org/0000-0002-6105-8631Ekaterina A. Budenkova1https://orcid.org/0000-0003-4854-5459Elena V. Ulrikh2https://orcid.org/0000-0003-4107-7277Evgeny G. Chupakhin3https://orcid.org/0000-0001-5284-4748Olga V. Kriger4https://orcid.org/0000-0002-1489-0716Yakov A. Masiutin5https://orcid.org/0000-0003-4347-3425Maria A. Smaga6https://orcid.org/0000-0001-5304-5761Yulia S. Basova7https://orcid.org/0000-0001-5361-5971Immanuel Kant Baltic Federal University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaKaliningrad State Technical University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaImmanuel Kant Baltic Federal University, Kaliningrad, RussiaForests being mostly non-renewable, miscanthus seems to be a promising alternative energy resource. This study investigates the enzymatic hydrolysis of pretreated miscanthus biomass. The research featured Miscanthus sinensis Strictus biomass. The methods included raw material pretreatment, enzymatic hydrolysis, matrix-assisted laser desorption ionization time-of-flight mass spectrometry (MALDI-TOF) of monosaccharide residues, and nuclear magnetic resonance (1H NMR) spectrometry of non-hydrolyzed lignin. A hammer mill with a particle size of 0.2–0.3 mm proved to be effective for preliminary mechanical processing of miscanthus. This type of treatment provided the maximal yield of carbohydrate-containing biomass (62.33 ± 1.87%). The optimal multi-enzyme composition included Cellulase Ultra obtained from Trichoderma reeseii, xylanase obtained from Thermomyces lanuginosus, and β-gluconase obtained from Myceliophtorafergusii. The fermentation temperature was 50 ± 1°C (72 ± 1 h). At these parameters, the conversion of holocellulose of miscanthus biomass was 96.0 ± 4.8%, and the yield of reducing substances was 97.00 ± 4.85%. The article introduces the optimal enzymatic hydrolysis parameters for pretreating Miscanthus sinensis Strictus biomass as a source of carbohydrate-containing substrates and describes their subsequent use for bacterial cellulose biosynthesis. The carbohydrate composition of hydrolysates included residual lignin, such polysaccharides as glucan and xylan, and various monosaccharides, namely arabinose, xylose, galactose, glucose, and uronic acids. Hydrolyzed miscanthus proved to be an effective renewable and environmentally friendly biodiesel.https://fptt.ru/en/issues/20365/20375/miscanthusbiofuelenzymatic hydrolysis pretreatmentreducing sugarsnon-hydrolysed lignincellulose
spellingShingle Olga B. Kalashnikova
Ekaterina A. Budenkova
Elena V. Ulrikh
Evgeny G. Chupakhin
Olga V. Kriger
Yakov A. Masiutin
Maria A. Smaga
Yulia S. Basova
Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
Техника и технология пищевых производств
miscanthus
biofuel
enzymatic hydrolysis pretreatment
reducing sugars
non-hydrolysed lignin
cellulose
title Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
title_full Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
title_fullStr Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
title_full_unstemmed Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
title_short Enzymatic Hydrolysis of Pretreated Miscanthus Biomass
title_sort enzymatic hydrolysis of pretreated miscanthus biomass
topic miscanthus
biofuel
enzymatic hydrolysis pretreatment
reducing sugars
non-hydrolysed lignin
cellulose
url https://fptt.ru/en/issues/20365/20375/
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AT evgenygchupakhin enzymatichydrolysisofpretreatedmiscanthusbiomass
AT olgavkriger enzymatichydrolysisofpretreatedmiscanthusbiomass
AT yakovamasiutin enzymatichydrolysisofpretreatedmiscanthusbiomass
AT mariaasmaga enzymatichydrolysisofpretreatedmiscanthusbiomass
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