Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)

The accumulation of greenhouse gasses (CH<sub>4</sub> and CO<sub>2</sub>) results in an increase in the temperature of the atmosphere. The conversion of greenhouse gasses into chemicals and fuels with high added value benefits not only the environment but also energy developm...

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Main Authors: Derun Hua, Jian Li, Xiaowen Guo, Xinning Lu, Hao Ding, Rengui He
Format: Article
Language:English
Published: MDPI AG 2024-11-01
Series:Nanomaterials
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Online Access:https://www.mdpi.com/2079-4991/14/23/1877
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author Derun Hua
Jian Li
Xiaowen Guo
Xinning Lu
Hao Ding
Rengui He
author_facet Derun Hua
Jian Li
Xiaowen Guo
Xinning Lu
Hao Ding
Rengui He
author_sort Derun Hua
collection DOAJ
description The accumulation of greenhouse gasses (CH<sub>4</sub> and CO<sub>2</sub>) results in an increase in the temperature of the atmosphere. The conversion of greenhouse gasses into chemicals and fuels with high added value benefits not only the environment but also energy development. A promising and well-studied process is the reforming of methane, where CH<sub>4</sub> and CO<sub>2</sub> are converted into syngas (CO and H<sub>2</sub>). However, catalysts hinder the development of the process. In this paper, we investigate the conversion of CH<sub>4</sub> and CO<sub>2</sub> into syngas using a thermal conversion method. The catalysis performance was evaluated by reforming methane. Ni-based catalysts were prepared by different methods. All prepared catalysts were characterized (XRD, HRTEM et al.), and the process of reforming carbon dioxide–methane was carried out in a fixed bed reactor under atmospheric pressure and a high temperature. Ni(M) @CeO<sub>2</sub> is one of the most popular options due to the role of CeO<sub>2</sub>. The deposition of coke in Ni-based catalysts was investigated.
format Article
id doaj-art-5f5cce46586e44db9804d6e6f6866eb8
institution Kabale University
issn 2079-4991
language English
publishDate 2024-11-01
publisher MDPI AG
record_format Article
series Nanomaterials
spelling doaj-art-5f5cce46586e44db9804d6e6f6866eb82024-12-13T16:29:13ZengMDPI AGNanomaterials2079-49912024-11-011423187710.3390/nano14231877Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)Derun Hua0Jian Li1Xiaowen Guo2Xinning Lu3Hao Ding4Rengui He5Key Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaKey Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaKey Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaKey Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaKey Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaKey Laboratory of Functional Materials Chemistry, Gannan Normal University, Ganzhou 341003, ChinaThe accumulation of greenhouse gasses (CH<sub>4</sub> and CO<sub>2</sub>) results in an increase in the temperature of the atmosphere. The conversion of greenhouse gasses into chemicals and fuels with high added value benefits not only the environment but also energy development. A promising and well-studied process is the reforming of methane, where CH<sub>4</sub> and CO<sub>2</sub> are converted into syngas (CO and H<sub>2</sub>). However, catalysts hinder the development of the process. In this paper, we investigate the conversion of CH<sub>4</sub> and CO<sub>2</sub> into syngas using a thermal conversion method. The catalysis performance was evaluated by reforming methane. Ni-based catalysts were prepared by different methods. All prepared catalysts were characterized (XRD, HRTEM et al.), and the process of reforming carbon dioxide–methane was carried out in a fixed bed reactor under atmospheric pressure and a high temperature. Ni(M) @CeO<sub>2</sub> is one of the most popular options due to the role of CeO<sub>2</sub>. The deposition of coke in Ni-based catalysts was investigated.https://www.mdpi.com/2079-4991/14/23/1877reformingCore@Shell materialMOF
spellingShingle Derun Hua
Jian Li
Xiaowen Guo
Xinning Lu
Hao Ding
Rengui He
Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
Nanomaterials
reforming
Core@Shell material
MOF
title Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
title_full Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
title_fullStr Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
title_full_unstemmed Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
title_short Syngas from Reforming Methane and Carbon Dioxide on Ni@M(SiO<sub>2</sub> and CeO<sub>2</sub>)
title_sort syngas from reforming methane and carbon dioxide on ni m sio sub 2 sub and ceo sub 2 sub
topic reforming
Core@Shell material
MOF
url https://www.mdpi.com/2079-4991/14/23/1877
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