Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling

The increasing demand for cobalt reduction and high energy density in lithium-ion batteries has accelerated the development of cathode-active materials based on Ni-rich layered oxides. However, Ni-rich cathodes, such as LiNi0.8Mn0.1Co0.1O2 (NMC811), suffer from capacity degradation due to factors in...

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Main Authors: Daisuke SHIBATA, Rinka YAMAMOTO, Mao MATSUMOTO, Haruno MURAYAMA, Chengchao ZHONG, Keiji SHIMODA, Ken-ichi OKAZAKI, Shohei YAMASHITA, Yuki ORIKASA
Format: Article
Language:English
Published: The Electrochemical Society of Japan 2025-06-01
Series:Electrochemistry
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Online Access:https://www.jstage.jst.go.jp/article/electrochemistry/93/6/93_25-71043/_html/-char/en
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author Daisuke SHIBATA
Rinka YAMAMOTO
Mao MATSUMOTO
Haruno MURAYAMA
Chengchao ZHONG
Keiji SHIMODA
Ken-ichi OKAZAKI
Shohei YAMASHITA
Yuki ORIKASA
author_facet Daisuke SHIBATA
Rinka YAMAMOTO
Mao MATSUMOTO
Haruno MURAYAMA
Chengchao ZHONG
Keiji SHIMODA
Ken-ichi OKAZAKI
Shohei YAMASHITA
Yuki ORIKASA
author_sort Daisuke SHIBATA
collection DOAJ
description The increasing demand for cobalt reduction and high energy density in lithium-ion batteries has accelerated the development of cathode-active materials based on Ni-rich layered oxides. However, Ni-rich cathodes, such as LiNi0.8Mn0.1Co0.1O2 (NMC811), suffer from capacity degradation due to factors including crystal structure changes, particle fractures, and the formation of surface resistive layers. While these degradation mechanisms have been extensively studied, the specific effects of high current density on capacity fading remains unclear. In this study, we investigate the degradation mechanisms of NMC811 cathodes cycled at 0.1C and 2C rates. Cycling at 2C rate results in severe capacity fading over 50 cycles. Synchrotron X-ray diffraction confirms the preservation of the crystal structure without evidence of Li–Ni site exchange. X-ray computed tomography reveals surface breakdown of primary particles following high-rate cycling. X-ray absorption spectroscopy and hard X-ray photoelectron spectroscopy indicate the formation of a thick resistive surface layer after the cycling at 2C rate. This layer, formed due to high polarization and intensified side reactions, impedes lithium-ion transport, leading to significant capacity degradation.
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institution Kabale University
issn 2186-2451
language English
publishDate 2025-06-01
publisher The Electrochemical Society of Japan
record_format Article
series Electrochemistry
spelling doaj-art-5f1ab3b0adba4cb788adc7c3b26a9f502025-08-20T03:47:20ZengThe Electrochemical Society of JapanElectrochemistry2186-24512025-06-0193606301606301610.5796/electrochemistry.25-71043electrochemistryAnalysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge CyclingDaisuke SHIBATA0Rinka YAMAMOTO1Mao MATSUMOTO2Haruno MURAYAMA3https://orcid.org/0000-0002-3283-9084Chengchao ZHONG4https://orcid.org/0000-0002-3089-6974Keiji SHIMODA5https://orcid.org/0000-0003-4600-3437Ken-ichi OKAZAKI6https://orcid.org/0000-0003-0800-712XShohei YAMASHITA7https://orcid.org/0000-0002-0842-6239Yuki ORIKASA8https://orcid.org/0000-0002-9869-9520Research Organization of Science and Technology, Ritsumeikan UniversityDepartment of Applied Chemistry, Ritsumeikan UniversityDepartment of Applied Chemistry, Ritsumeikan UniversityDepartment of Applied Chemistry and Bioscience, Kanagawa Institute of TechnologyDepartment of Applied Chemistry, Ritsumeikan UniversityRitsumeikan Global Innovation Research Organization, Ritsumeikan UniversityResearch Organization of Science and Technology, Ritsumeikan UniversityInstitute of Materials Structure Science Photon Factory, High Energy Accelerator Research Organization (KEK)Department of Applied Chemistry, Ritsumeikan UniversityThe increasing demand for cobalt reduction and high energy density in lithium-ion batteries has accelerated the development of cathode-active materials based on Ni-rich layered oxides. However, Ni-rich cathodes, such as LiNi0.8Mn0.1Co0.1O2 (NMC811), suffer from capacity degradation due to factors including crystal structure changes, particle fractures, and the formation of surface resistive layers. While these degradation mechanisms have been extensively studied, the specific effects of high current density on capacity fading remains unclear. In this study, we investigate the degradation mechanisms of NMC811 cathodes cycled at 0.1C and 2C rates. Cycling at 2C rate results in severe capacity fading over 50 cycles. Synchrotron X-ray diffraction confirms the preservation of the crystal structure without evidence of Li–Ni site exchange. X-ray computed tomography reveals surface breakdown of primary particles following high-rate cycling. X-ray absorption spectroscopy and hard X-ray photoelectron spectroscopy indicate the formation of a thick resistive surface layer after the cycling at 2C rate. This layer, formed due to high polarization and intensified side reactions, impedes lithium-ion transport, leading to significant capacity degradation.https://www.jstage.jst.go.jp/article/electrochemistry/93/6/93_25-71043/_html/-char/enlithium-ion batterycathodelayered rock-salt oxidedegradation
spellingShingle Daisuke SHIBATA
Rinka YAMAMOTO
Mao MATSUMOTO
Haruno MURAYAMA
Chengchao ZHONG
Keiji SHIMODA
Ken-ichi OKAZAKI
Shohei YAMASHITA
Yuki ORIKASA
Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
Electrochemistry
lithium-ion battery
cathode
layered rock-salt oxide
degradation
title Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
title_full Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
title_fullStr Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
title_full_unstemmed Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
title_short Analysis of Degradation Mechanisms in LiNi0.8Mn0.1Co0.1O2 Lithium-ion Battery Cathodes During High-Rate Charge–Discharge Cycling
title_sort analysis of degradation mechanisms in lini0 8mn0 1co0 1o2 lithium ion battery cathodes during high rate charge discharge cycling
topic lithium-ion battery
cathode
layered rock-salt oxide
degradation
url https://www.jstage.jst.go.jp/article/electrochemistry/93/6/93_25-71043/_html/-char/en
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