Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets

As electromagnetic technology advances and demand for electronic devices grows, concerns about electromagnetic pollution intensify. This has spurred focused research on innovative electromagnetic absorbers, particularly chalcogenides, noted for their superior absorption capabilities. In this study,...

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Main Authors: Liquan Fan, Honglin Ai, Meiye Jiao, Yao Li, Yongheng Jin, Yiru Fu, Jing Wang, Yuwei Wang, Deqing Zhang, Guangping Zheng, Junye Cheng
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2024-10-01
Series:Nano Materials Science
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Online Access:http://www.sciencedirect.com/science/article/pii/S2589965124000783
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author Liquan Fan
Honglin Ai
Meiye Jiao
Yao Li
Yongheng Jin
Yiru Fu
Jing Wang
Yuwei Wang
Deqing Zhang
Guangping Zheng
Junye Cheng
author_facet Liquan Fan
Honglin Ai
Meiye Jiao
Yao Li
Yongheng Jin
Yiru Fu
Jing Wang
Yuwei Wang
Deqing Zhang
Guangping Zheng
Junye Cheng
author_sort Liquan Fan
collection DOAJ
description As electromagnetic technology advances and demand for electronic devices grows, concerns about electromagnetic pollution intensify. This has spurred focused research on innovative electromagnetic absorbers, particularly chalcogenides, noted for their superior absorption capabilities. In this study, we successfully synthesize 3R–TaS2 nanosheets using a straightforward calcination method for the first time. These nanosheets exhibit significant absorption capabilities in both the C-band (4–8 ​GHz) and Ku-band (12–18 ​GHz) frequency ranges. By optimizing the calcination process, the complex permittivity of TaS2 is enhanced, specifically for those synthesized at 1000 ​°C for 24 ​h. The nanosheets possess dual-band absorption properties, with a notable minimum reflection loss (RLmin) of −41.4 ​dB in the C-band, and an average absorption intensity exceeding 10 ​dB in C- and Ku-bands, in the absorbers with a thickness of 5.6 ​mm. Additionally, the 3R–TaS2 nanosheets are demonstrated to have an effective absorption bandwidth of 5.04 ​GHz (3.84–8.88 ​GHz) in the absorbers with thicknesses of 3.5–5.5 ​mm. The results highlight the multiple reflection effects in 3R–TaS2 as caused by their stacked structures, which could be promising low-frequency absorbers.
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record_format Article
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spelling doaj-art-5a0c7779eac547989179f2efa8708fc92024-11-28T04:34:57ZengKeAi Communications Co., Ltd.Nano Materials Science2589-96512024-10-0165635646Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheetsLiquan Fan0Honglin Ai1Meiye Jiao2Yao Li3Yongheng Jin4Yiru Fu5Jing Wang6Yuwei Wang7Deqing Zhang8Guangping Zheng9Junye Cheng10College of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaDepartment of Materials Science, Shenzhen MSU-BIT University, Shenzhen, Guangdong Province, 517182, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR ChinaCollege of Materials Science and Engineering, Heilongjiang Provincial Key Laboratory of Polymeric Composite Materials, Qiqihar University, No.42, Wenhua Street, Qiqihar, 161006, PR China; Corresponding author.Department of Mechanical Engineering, Hong Kong Polytechnic University, Hung Hom, Kowloon, Hong Kong, ChinaDepartment of Materials Science, Shenzhen MSU-BIT University, Shenzhen, Guangdong Province, 517182, PR China; Corresponding author.As electromagnetic technology advances and demand for electronic devices grows, concerns about electromagnetic pollution intensify. This has spurred focused research on innovative electromagnetic absorbers, particularly chalcogenides, noted for their superior absorption capabilities. In this study, we successfully synthesize 3R–TaS2 nanosheets using a straightforward calcination method for the first time. These nanosheets exhibit significant absorption capabilities in both the C-band (4–8 ​GHz) and Ku-band (12–18 ​GHz) frequency ranges. By optimizing the calcination process, the complex permittivity of TaS2 is enhanced, specifically for those synthesized at 1000 ​°C for 24 ​h. The nanosheets possess dual-band absorption properties, with a notable minimum reflection loss (RLmin) of −41.4 ​dB in the C-band, and an average absorption intensity exceeding 10 ​dB in C- and Ku-bands, in the absorbers with a thickness of 5.6 ​mm. Additionally, the 3R–TaS2 nanosheets are demonstrated to have an effective absorption bandwidth of 5.04 ​GHz (3.84–8.88 ​GHz) in the absorbers with thicknesses of 3.5–5.5 ​mm. The results highlight the multiple reflection effects in 3R–TaS2 as caused by their stacked structures, which could be promising low-frequency absorbers.http://www.sciencedirect.com/science/article/pii/S25899651240007833R–TaS2NanosheetsElectromagnetic wave absorptionReflection loss
spellingShingle Liquan Fan
Honglin Ai
Meiye Jiao
Yao Li
Yongheng Jin
Yiru Fu
Jing Wang
Yuwei Wang
Deqing Zhang
Guangping Zheng
Junye Cheng
Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
Nano Materials Science
3R–TaS2
Nanosheets
Electromagnetic wave absorption
Reflection loss
title Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
title_full Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
title_fullStr Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
title_full_unstemmed Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
title_short Low-frequency and dual-band microwave absorption properties of novel VB-group disulphides (3R–TaS2) nanosheets
title_sort low frequency and dual band microwave absorption properties of novel vb group disulphides 3r tas2 nanosheets
topic 3R–TaS2
Nanosheets
Electromagnetic wave absorption
Reflection loss
url http://www.sciencedirect.com/science/article/pii/S2589965124000783
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