Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3

The Er3+ doped lead–bismuth–gallium oxide glasses were prepared by melt quenching technique. The spectral and luminescent properties were analyzed based on experimental and theoretical calculations. Analysis of Er3+ concentration dependences of density and electronic optical polarizability was carri...

Full description

Saved in:
Bibliographic Details
Main Authors: V.A. Klinkov, A.V. Semencha, A. Babkina, E.A. Tsimerman
Format: Article
Language:English
Published: Elsevier 2024-09-01
Series:Journal of Non-Crystalline Solids: X
Subjects:
Online Access:http://www.sciencedirect.com/science/article/pii/S2590159124000116
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846123336099168256
author V.A. Klinkov
A.V. Semencha
A. Babkina
E.A. Tsimerman
author_facet V.A. Klinkov
A.V. Semencha
A. Babkina
E.A. Tsimerman
author_sort V.A. Klinkov
collection DOAJ
description The Er3+ doped lead–bismuth–gallium oxide glasses were prepared by melt quenching technique. The spectral and luminescent properties were analyzed based on experimental and theoretical calculations. Analysis of Er3+ concentration dependences of density and electronic optical polarizability was carried out. The radiative lifetime values for 4S3/2 and 4F9/2 energy states were calculated using Judd-Ofelt theory. In the glassy system under study, the concentration quenching of state 4S3/2 was discovered at content of erbium ions above 0.869 × 1020 cm−3. It was also shown that 4F9/2 energy state was isolated from concentration effects and showed an increase in luminescence intensity with increasing concentration of activator ions. The luminescence quantum efficiency for transition 4S3/2 → 4I15/2 was about 40%, which allows us to consider this system as a glassy matrix effective for activation by rare-earth ions.
format Article
id doaj-art-54e2a95c72a4464b81c94d11761b58c4
institution Kabale University
issn 2590-1591
language English
publishDate 2024-09-01
publisher Elsevier
record_format Article
series Journal of Non-Crystalline Solids: X
spelling doaj-art-54e2a95c72a4464b81c94d11761b58c42024-12-14T06:32:41ZengElsevierJournal of Non-Crystalline Solids: X2590-15912024-09-0123100216Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3V.A. Klinkov0A.V. Semencha1A. Babkina2E.A. Tsimerman3Peter the Great St. Petersburg Polytechnic University (SPbPU), St. Petersburg 195251, Russia; Corresponding author.Peter the Great St. Petersburg Polytechnic University (SPbPU), St. Petersburg 195251, RussiaITMO University, Kronverksky Avenue 49, St. Petersburg 197101, RussiaPeter the Great St. Petersburg Polytechnic University (SPbPU), St. Petersburg 195251, RussiaThe Er3+ doped lead–bismuth–gallium oxide glasses were prepared by melt quenching technique. The spectral and luminescent properties were analyzed based on experimental and theoretical calculations. Analysis of Er3+ concentration dependences of density and electronic optical polarizability was carried out. The radiative lifetime values for 4S3/2 and 4F9/2 energy states were calculated using Judd-Ofelt theory. In the glassy system under study, the concentration quenching of state 4S3/2 was discovered at content of erbium ions above 0.869 × 1020 cm−3. It was also shown that 4F9/2 energy state was isolated from concentration effects and showed an increase in luminescence intensity with increasing concentration of activator ions. The luminescence quantum efficiency for transition 4S3/2 → 4I15/2 was about 40%, which allows us to consider this system as a glassy matrix effective for activation by rare-earth ions.http://www.sciencedirect.com/science/article/pii/S2590159124000116Heavy metal oxide glassesJudd-Ofelt theoryDecay curvesLuminescenceEr-doped glasses
spellingShingle V.A. Klinkov
A.V. Semencha
A. Babkina
E.A. Tsimerman
Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
Journal of Non-Crystalline Solids: X
Heavy metal oxide glasses
Judd-Ofelt theory
Decay curves
Luminescence
Er-doped glasses
title Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
title_full Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
title_fullStr Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
title_full_unstemmed Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
title_short Analysis of luminescent properties of 40PbO–35Bi2O3–25Ga2O3 glasses doped with Er2O3
title_sort analysis of luminescent properties of 40pbo 35bi2o3 25ga2o3 glasses doped with er2o3
topic Heavy metal oxide glasses
Judd-Ofelt theory
Decay curves
Luminescence
Er-doped glasses
url http://www.sciencedirect.com/science/article/pii/S2590159124000116
work_keys_str_mv AT vaklinkov analysisofluminescentpropertiesof40pbo35bi2o325ga2o3glassesdopedwither2o3
AT avsemencha analysisofluminescentpropertiesof40pbo35bi2o325ga2o3glassesdopedwither2o3
AT ababkina analysisofluminescentpropertiesof40pbo35bi2o325ga2o3glassesdopedwither2o3
AT eatsimerman analysisofluminescentpropertiesof40pbo35bi2o325ga2o3glassesdopedwither2o3