Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea

Abstract The containment history in the coastal zone of the Bohai Sea has not been sufficiently traced because of the difficulty in identifying complex sources of pollutants. This study quantitatively identified various sources of Pb and Sr in two tidal flat sediment cores from Bohai Bay (core BB) a...

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Main Authors: Shuaiya Zhang, Qinyue Li, Yu Zou, Baolin Liu, Juan Yang, Houyi Zheng, Gege Liu
Format: Article
Language:English
Published: Nature Portfolio 2024-12-01
Series:Scientific Reports
Subjects:
Online Access:https://doi.org/10.1038/s41598-024-81493-w
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author Shuaiya Zhang
Qinyue Li
Yu Zou
Baolin Liu
Juan Yang
Houyi Zheng
Gege Liu
author_facet Shuaiya Zhang
Qinyue Li
Yu Zou
Baolin Liu
Juan Yang
Houyi Zheng
Gege Liu
author_sort Shuaiya Zhang
collection DOAJ
description Abstract The containment history in the coastal zone of the Bohai Sea has not been sufficiently traced because of the difficulty in identifying complex sources of pollutants. This study quantitatively identified various sources of Pb and Sr in two tidal flat sediment cores from Bohai Bay (core BB) and Liaodong Bay (core LB) based on their isotope ratios to trace the natural and anthropogenic disturbance history in the Bohai Sea. The results showed that natural inputs of Pb were the main sources for cores BB and LB; however, core LB was more influenced by anthropogenic inputs. Natural inputs were derived mainly from Chinese loess and Yellow River sediments, whereas anthropogenic sources were mainly a mixture of vehicular exhaust emissions before 2000 and coal combustion after 2000. Anthropogenic influence has declined since the late 1990s, especially in Bohai Bay, but has increased in Liaodong Bay from 1998 to 2006.
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spelling doaj-art-4f20f16a22ff45d9a39dd7b4490578d42024-12-08T12:31:25ZengNature PortfolioScientific Reports2045-23222024-12-0114111810.1038/s41598-024-81493-wUsing isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai SeaShuaiya Zhang0Qinyue Li1Yu Zou2Baolin Liu3Juan Yang4Houyi Zheng5Gege Liu6Key Laboratory of Polar Geology and Marine Mineral Resources, Ministry of Education, China University of Geosciences in BeijingKey Laboratory of Polar Geology and Marine Mineral Resources, Ministry of Education, China University of Geosciences in BeijingGuangxi Institute of Geological Exploration, China Chemical Geology and Mine BureauKey Laboratory of Polar Geology and Marine Mineral Resources, Ministry of Education, China University of Geosciences in BeijingKey Laboratory of Polar Geology and Marine Mineral Resources, Ministry of Education, China University of Geosciences in BeijingChina Chemical Geology and Mine BureauKey Laboratory of Polar Geology and Marine Mineral Resources, Ministry of Education, China University of Geosciences in BeijingAbstract The containment history in the coastal zone of the Bohai Sea has not been sufficiently traced because of the difficulty in identifying complex sources of pollutants. This study quantitatively identified various sources of Pb and Sr in two tidal flat sediment cores from Bohai Bay (core BB) and Liaodong Bay (core LB) based on their isotope ratios to trace the natural and anthropogenic disturbance history in the Bohai Sea. The results showed that natural inputs of Pb were the main sources for cores BB and LB; however, core LB was more influenced by anthropogenic inputs. Natural inputs were derived mainly from Chinese loess and Yellow River sediments, whereas anthropogenic sources were mainly a mixture of vehicular exhaust emissions before 2000 and coal combustion after 2000. Anthropogenic influence has declined since the late 1990s, especially in Bohai Bay, but has increased in Liaodong Bay from 1998 to 2006.https://doi.org/10.1038/s41598-024-81493-wPb isotope ratiosSr isotope ratiosSediment coresSource identificationHistorical variation
spellingShingle Shuaiya Zhang
Qinyue Li
Yu Zou
Baolin Liu
Juan Yang
Houyi Zheng
Gege Liu
Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
Scientific Reports
Pb isotope ratios
Sr isotope ratios
Sediment cores
Source identification
Historical variation
title Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
title_full Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
title_fullStr Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
title_full_unstemmed Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
title_short Using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the Bohai Sea
title_sort using isotopic lead and strontium in sediments to trace natural and anthropogenic sources in the bohai sea
topic Pb isotope ratios
Sr isotope ratios
Sediment cores
Source identification
Historical variation
url https://doi.org/10.1038/s41598-024-81493-w
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