Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect

The relationship between magnetization and light has been the subject of intensive research for the past century. Herein, the impact of magnetization on light polarization is well understood. Conversely, the manipulation of magnetism with polarized light is being investigated to achieve all‐optical...

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Main Authors: Sergii Parchenko, Kevin Hofhuis, Agne Åberg Larsson, Vassilios Kapaklis, Valerio Scagnoli, Laura Jane Heyderman, Armin Kleibert
Format: Article
Language:English
Published: Wiley-VCH 2025-01-01
Series:Advanced Photonics Research
Subjects:
Online Access:https://doi.org/10.1002/adpr.202400083
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author Sergii Parchenko
Kevin Hofhuis
Agne Åberg Larsson
Vassilios Kapaklis
Valerio Scagnoli
Laura Jane Heyderman
Armin Kleibert
author_facet Sergii Parchenko
Kevin Hofhuis
Agne Åberg Larsson
Vassilios Kapaklis
Valerio Scagnoli
Laura Jane Heyderman
Armin Kleibert
author_sort Sergii Parchenko
collection DOAJ
description The relationship between magnetization and light has been the subject of intensive research for the past century. Herein, the impact of magnetization on light polarization is well understood. Conversely, the manipulation of magnetism with polarized light is being investigated to achieve all‐optical control of magnetism, driven by potential technological implementation in spintronics. Remarkable discoveries, such as the single‐pulse all‐optical switching of magnetization in thin films and submicrometer structures, have been reported. However, the demonstration of local optical control of magnetism at the nanoscale has remained elusive. Herein, it is demonstrated that exciting gold nanodiscs with circularly polarized femtosecond laser pulses lead to ultrafast, local, and deterministic control of magnetization in an adjacent magnetic film. This control is achieved by exploiting the magnetic moment generated in plasmonic nanodiscs through the inverse Faraday effect. The results pave the way for light‐driven control in nanoscale spintronic devices and provide important insights into the generation of magnetic fields in plasmonic nanostructures.
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institution Kabale University
issn 2699-9293
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publishDate 2025-01-01
publisher Wiley-VCH
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series Advanced Photonics Research
spelling doaj-art-4cbb4a77f141401889bf3f44b66fc48e2025-01-06T02:15:54ZengWiley-VCHAdvanced Photonics Research2699-92932025-01-0161n/an/a10.1002/adpr.202400083Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday EffectSergii Parchenko0Kevin Hofhuis1Agne Åberg Larsson2Vassilios Kapaklis3Valerio Scagnoli4Laura Jane Heyderman5Armin Kleibert6Laboratory for Mesoscopic Systems Department of Materials ETH Zurich 8093 Zurich SwitzerlandLaboratory for Mesoscopic Systems Department of Materials ETH Zurich 8093 Zurich SwitzerlandDepartment of Physics and Astronomy Uppsala University Box 516 751 20 Uppsala SwedenDepartment of Physics and Astronomy Uppsala University Box 516 751 20 Uppsala SwedenLaboratory for Mesoscopic Systems Department of Materials ETH Zurich 8093 Zurich SwitzerlandLaboratory for Mesoscopic Systems Department of Materials ETH Zurich 8093 Zurich SwitzerlandSwiss Light Source Paul Scherrer Institute 5232 Villigen PSI SwitzerlandThe relationship between magnetization and light has been the subject of intensive research for the past century. Herein, the impact of magnetization on light polarization is well understood. Conversely, the manipulation of magnetism with polarized light is being investigated to achieve all‐optical control of magnetism, driven by potential technological implementation in spintronics. Remarkable discoveries, such as the single‐pulse all‐optical switching of magnetization in thin films and submicrometer structures, have been reported. However, the demonstration of local optical control of magnetism at the nanoscale has remained elusive. Herein, it is demonstrated that exciting gold nanodiscs with circularly polarized femtosecond laser pulses lead to ultrafast, local, and deterministic control of magnetization in an adjacent magnetic film. This control is achieved by exploiting the magnetic moment generated in plasmonic nanodiscs through the inverse Faraday effect. The results pave the way for light‐driven control in nanoscale spintronic devices and provide important insights into the generation of magnetic fields in plasmonic nanostructures.https://doi.org/10.1002/adpr.202400083inverse Faraday effectmagnetization controlnanoplasmonicsultrafast dynamics
spellingShingle Sergii Parchenko
Kevin Hofhuis
Agne Åberg Larsson
Vassilios Kapaklis
Valerio Scagnoli
Laura Jane Heyderman
Armin Kleibert
Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
Advanced Photonics Research
inverse Faraday effect
magnetization control
nanoplasmonics
ultrafast dynamics
title Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
title_full Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
title_fullStr Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
title_full_unstemmed Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
title_short Plasmon‐Enhanced Optical Control of Magnetism at the Nanoscale via the Inverse Faraday Effect
title_sort plasmon enhanced optical control of magnetism at the nanoscale via the inverse faraday effect
topic inverse Faraday effect
magnetization control
nanoplasmonics
ultrafast dynamics
url https://doi.org/10.1002/adpr.202400083
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AT vassilioskapaklis plasmonenhancedopticalcontrolofmagnetismatthenanoscaleviatheinversefaradayeffect
AT valerioscagnoli plasmonenhancedopticalcontrolofmagnetismatthenanoscaleviatheinversefaradayeffect
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