Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes

Herein, we report the first example of molybdenum-catalyzed (<i>E</i>)-Selective anti-Markovnikov hydrosilylation of alkynes. The reaction operates effectively with the utilization of minute amounts of the inexpensive, bench-stable pre-catalyst and ligand under mild conditions. Moreover,...

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Main Authors: Feihua Ye, Zhaoyang Huang, Jiahao Li, Qiumin Wang, Lihuan Wu, Xiang Li
Format: Article
Language:English
Published: MDPI AG 2024-12-01
Series:Molecules
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Online Access:https://www.mdpi.com/1420-3049/29/24/5952
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author Feihua Ye
Zhaoyang Huang
Jiahao Li
Qiumin Wang
Lihuan Wu
Xiang Li
author_facet Feihua Ye
Zhaoyang Huang
Jiahao Li
Qiumin Wang
Lihuan Wu
Xiang Li
author_sort Feihua Ye
collection DOAJ
description Herein, we report the first example of molybdenum-catalyzed (<i>E</i>)-Selective anti-Markovnikov hydrosilylation of alkynes. The reaction operates effectively with the utilization of minute amounts of the inexpensive, bench-stable pre-catalyst and ligand under mild conditions. Moreover, this molybdenum-catalyzed hydrosilylation process features the advantages of simple operation, excellent selectivity, and broad functional groups tolerance.
format Article
id doaj-art-4278da82713e4dba91f4c31425d62077
institution Kabale University
issn 1420-3049
language English
publishDate 2024-12-01
publisher MDPI AG
record_format Article
series Molecules
spelling doaj-art-4278da82713e4dba91f4c31425d620772024-12-27T14:42:45ZengMDPI AGMolecules1420-30492024-12-012924595210.3390/molecules29245952Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of AlkynesFeihua Ye0Zhaoyang Huang1Jiahao Li2Qiumin Wang3Lihuan Wu4Xiang Li5School of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaSchool of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaSchool of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaSchool of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaSchool of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaSchool of Environmental and Chemical Engineering, Zhaoqing University, Zhaoqing 526061, ChinaHerein, we report the first example of molybdenum-catalyzed (<i>E</i>)-Selective anti-Markovnikov hydrosilylation of alkynes. The reaction operates effectively with the utilization of minute amounts of the inexpensive, bench-stable pre-catalyst and ligand under mild conditions. Moreover, this molybdenum-catalyzed hydrosilylation process features the advantages of simple operation, excellent selectivity, and broad functional groups tolerance.https://www.mdpi.com/1420-3049/29/24/5952(<i>E</i>)-vinysilaneshydrosilylationalkynesmolybdenum catalystsynthetic method
spellingShingle Feihua Ye
Zhaoyang Huang
Jiahao Li
Qiumin Wang
Lihuan Wu
Xiang Li
Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
Molecules
(<i>E</i>)-vinysilanes
hydrosilylation
alkynes
molybdenum catalyst
synthetic method
title Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
title_full Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
title_fullStr Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
title_full_unstemmed Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
title_short Molybdenum-Catalyzed (<i>E</i>)-Selective Anti-Markovnikov Hydrosilylation of Alkynes
title_sort molybdenum catalyzed i e i selective anti markovnikov hydrosilylation of alkynes
topic (<i>E</i>)-vinysilanes
hydrosilylation
alkynes
molybdenum catalyst
synthetic method
url https://www.mdpi.com/1420-3049/29/24/5952
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AT qiuminwang molybdenumcatalyzedieiselectiveantimarkovnikovhydrosilylationofalkynes
AT lihuanwu molybdenumcatalyzedieiselectiveantimarkovnikovhydrosilylationofalkynes
AT xiangli molybdenumcatalyzedieiselectiveantimarkovnikovhydrosilylationofalkynes