Multiphase superconductivity in PdBi2

Abstract Unconventional superconductivity, where electron pairing does not involve electron-phonon interactions, is often attributed to magnetic correlations in a material. Well known examples include high-T c cuprates and uranium-based heavy fermion superconductors. Less explored are unconventional...

Full description

Saved in:
Bibliographic Details
Main Authors: Lewis Powell, Wenjun Kuang, Gabriel Hawkins-Pottier, Rashid Jalil, John Birkbeck, Ziyi Jiang, Minsoo Kim, Yichao Zou, Sofiia Komrakova, Sarah Haigh, Ivan Timokhin, Geetha Balakrishnan, Andre K. Geim, Niels Walet, Alessandro Principi, Irina V. Grigorieva
Format: Article
Language:English
Published: Nature Portfolio 2025-01-01
Series:Nature Communications
Online Access:https://doi.org/10.1038/s41467-024-54867-x
Tags: Add Tag
No Tags, Be the first to tag this record!
Description
Summary:Abstract Unconventional superconductivity, where electron pairing does not involve electron-phonon interactions, is often attributed to magnetic correlations in a material. Well known examples include high-T c cuprates and uranium-based heavy fermion superconductors. Less explored are unconventional superconductors with strong spin-orbit coupling, where interactions between spin-polarised electrons and external magnetic field can result in multiple superconducting phases and field-induced transitions between them, a rare phenomenon in the superconducting state. Here we report a magnetic-field driven phase transition in β-PdBi2, a layered non-magnetic superconductor. Our tunnelling spectroscopy on thin PdBi2 monocrystals incorporated in planar superconductor-insulator-normal metal junctions reveals a marked discontinuity in the superconducting properties with increasing in-plane field, which is consistent with a transition from conventional (s-wave) to nodal pairing. Our theoretical analysis suggests that this phase transition may arise from spin polarisation and spin-momentum locking caused by locally broken inversion symmetry, with p-wave pairing becoming energetically favourable in high fields. Our findings also reconcile earlier predictions of unconventional multigap superconductivity in β-PdBi2 with previous experiments where only a single s-wave gap could be detected.
ISSN:2041-1723