Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects

We study the spin-polarized electron transport properties of hybrid BN–C nanotubes (BN–CNTs) in their pristine form and with Stone–Wales defects, namely, Cx(BN)10−x, using combined first-principles density functional theory and quantum transport simulations. We show that the band structures of prist...

Full description

Saved in:
Bibliographic Details
Main Authors: Haiqing Wan, Tong Chen, Wei Hu, Yee Sin Ang
Format: Article
Language:English
Published: AIP Publishing LLC 2024-11-01
Series:APL Materials
Online Access:http://dx.doi.org/10.1063/5.0237443
Tags: Add Tag
No Tags, Be the first to tag this record!
_version_ 1846141130133995520
author Haiqing Wan
Tong Chen
Wei Hu
Yee Sin Ang
author_facet Haiqing Wan
Tong Chen
Wei Hu
Yee Sin Ang
author_sort Haiqing Wan
collection DOAJ
description We study the spin-polarized electron transport properties of hybrid BN–C nanotubes (BN–CNTs) in their pristine form and with Stone–Wales defects, namely, Cx(BN)10−x, using combined first-principles density functional theory and quantum transport simulations. We show that the band structures of pristine BN–CNTs can be sensitively tuned by their composition, transiting from the nonmagnetic semiconductor to half-semimetal and finally to a narrow gap semiconductor with increasing x. The spin-dependent current–voltage characteristics are sensitively modulated by x in the hybridized Cx(BN)10−x. The SW defect acts as an active scattering center for BN–CNTs, which decreases the overall conductance of nanotubes. Remarkably, a spin-filtering effect (SFE) with nearly 96% filtering efficiency is observed in C4(BN)6, and such a high SFE remains robust even in the presence of Stone–Wales defects. These results reveal the potential role of hybrid BN–CNT as a building block for spintronic device technology.
format Article
id doaj-art-3bf42716b6da4fb58ad3c2b929d1894a
institution Kabale University
issn 2166-532X
language English
publishDate 2024-11-01
publisher AIP Publishing LLC
record_format Article
series APL Materials
spelling doaj-art-3bf42716b6da4fb58ad3c2b929d1894a2024-12-04T17:09:06ZengAIP Publishing LLCAPL Materials2166-532X2024-11-011211111103111103-710.1063/5.0237443Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defectsHaiqing Wan0Tong Chen1Wei Hu2Yee Sin Ang3Department of Ecology and Environment, Yuzhang Normal University, Nanchang 330029, ChinaEnergy Materials Computing Center, Jiangxi University of Science and Technology, Nanchang 330013, People’s Republic of ChinaDepartment of Ecology and Environment, Yuzhang Normal University, Nanchang 330029, ChinaScience, Mathematics and Technology (SMT), Singapore University of Technology and Design, Singapore 487372, SingaporeWe study the spin-polarized electron transport properties of hybrid BN–C nanotubes (BN–CNTs) in their pristine form and with Stone–Wales defects, namely, Cx(BN)10−x, using combined first-principles density functional theory and quantum transport simulations. We show that the band structures of pristine BN–CNTs can be sensitively tuned by their composition, transiting from the nonmagnetic semiconductor to half-semimetal and finally to a narrow gap semiconductor with increasing x. The spin-dependent current–voltage characteristics are sensitively modulated by x in the hybridized Cx(BN)10−x. The SW defect acts as an active scattering center for BN–CNTs, which decreases the overall conductance of nanotubes. Remarkably, a spin-filtering effect (SFE) with nearly 96% filtering efficiency is observed in C4(BN)6, and such a high SFE remains robust even in the presence of Stone–Wales defects. These results reveal the potential role of hybrid BN–CNT as a building block for spintronic device technology.http://dx.doi.org/10.1063/5.0237443
spellingShingle Haiqing Wan
Tong Chen
Wei Hu
Yee Sin Ang
Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
APL Materials
title Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
title_full Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
title_fullStr Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
title_full_unstemmed Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
title_short Quantum transport properties of hybrid BN–C nanotubes: Strong spin filtering effect robust against Stone–Wales defects
title_sort quantum transport properties of hybrid bn c nanotubes strong spin filtering effect robust against stone wales defects
url http://dx.doi.org/10.1063/5.0237443
work_keys_str_mv AT haiqingwan quantumtransportpropertiesofhybridbncnanotubesstrongspinfilteringeffectrobustagainststonewalesdefects
AT tongchen quantumtransportpropertiesofhybridbncnanotubesstrongspinfilteringeffectrobustagainststonewalesdefects
AT weihu quantumtransportpropertiesofhybridbncnanotubesstrongspinfilteringeffectrobustagainststonewalesdefects
AT yeesinang quantumtransportpropertiesofhybridbncnanotubesstrongspinfilteringeffectrobustagainststonewalesdefects