Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers

Abstract Negative differential resistance (NDR) is the key feature of resonant tunneling diodes exploited for high‐frequency and low‐power devices and recent studies have focused on NDR in van der Waals heterostructures and nanoscale materials. Here, strong NDR confined along a 1‐nm‐wide 1D channel...

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Main Authors: Qirong Yao, Jae Whan Park, Choongjae Won, Sang‐Wook Cheong, Han Woong Yeom
Format: Article
Language:English
Published: Wiley 2025-01-01
Series:Advanced Science
Subjects:
Online Access:https://doi.org/10.1002/advs.202408090
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author Qirong Yao
Jae Whan Park
Choongjae Won
Sang‐Wook Cheong
Han Woong Yeom
author_facet Qirong Yao
Jae Whan Park
Choongjae Won
Sang‐Wook Cheong
Han Woong Yeom
author_sort Qirong Yao
collection DOAJ
description Abstract Negative differential resistance (NDR) is the key feature of resonant tunneling diodes exploited for high‐frequency and low‐power devices and recent studies have focused on NDR in van der Waals heterostructures and nanoscale materials. Here, strong NDR confined along a 1‐nm‐wide 1D channel within a van der Waals layer 1T‐TaS2 is reported. Using scanning tunneling microscopy, a double 1D NDR channel formed along the sides of a charge–density‐wave domain wall of 1T‐TaS2 is found. The density functional theory calculation elucidates that the strong local band‐bending at the domain wall and the interlayer orbital overlap cooperate to bring about 1D NDR channels. Furthermore, the NDR is well controlled by changing the tunneling junction distance. This result would be important for nanoscale device applications based on strong nonlinear resistance within van der Waals material architectures.
format Article
id doaj-art-3b403c2386a04e4f9e2f7d56c7e5cb81
institution Kabale University
issn 2198-3844
language English
publishDate 2025-01-01
publisher Wiley
record_format Article
series Advanced Science
spelling doaj-art-3b403c2386a04e4f9e2f7d56c7e5cb812025-01-13T15:29:43ZengWileyAdvanced Science2198-38442025-01-01122n/an/a10.1002/advs.202408090Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals LayersQirong Yao0Jae Whan Park1Choongjae Won2Sang‐Wook Cheong3Han Woong Yeom4Center for Artificial Low Dimensional Electronic Systems Institute for Basic Science (IBS) Pohang 37673 South KoreaCenter for Artificial Low Dimensional Electronic Systems Institute for Basic Science (IBS) Pohang 37673 South KoreaLaboratory for Pohang Emergent Materials Department of Physics Pohang University of Science and Technology Pohang 37673 South KoreaLaboratory for Pohang Emergent Materials Department of Physics Pohang University of Science and Technology Pohang 37673 South KoreaCenter for Artificial Low Dimensional Electronic Systems Institute for Basic Science (IBS) Pohang 37673 South KoreaAbstract Negative differential resistance (NDR) is the key feature of resonant tunneling diodes exploited for high‐frequency and low‐power devices and recent studies have focused on NDR in van der Waals heterostructures and nanoscale materials. Here, strong NDR confined along a 1‐nm‐wide 1D channel within a van der Waals layer 1T‐TaS2 is reported. Using scanning tunneling microscopy, a double 1D NDR channel formed along the sides of a charge–density‐wave domain wall of 1T‐TaS2 is found. The density functional theory calculation elucidates that the strong local band‐bending at the domain wall and the interlayer orbital overlap cooperate to bring about 1D NDR channels. Furthermore, the NDR is well controlled by changing the tunneling junction distance. This result would be important for nanoscale device applications based on strong nonlinear resistance within van der Waals material architectures.https://doi.org/10.1002/advs.2024080901T‐TaS2density‐functional calculationsinterlayer orbital overlapnegative differential resistancescanning tunneling microscopy and spectroscopy
spellingShingle Qirong Yao
Jae Whan Park
Choongjae Won
Sang‐Wook Cheong
Han Woong Yeom
Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
Advanced Science
1T‐TaS2
density‐functional calculations
interlayer orbital overlap
negative differential resistance
scanning tunneling microscopy and spectroscopy
title Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
title_full Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
title_fullStr Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
title_full_unstemmed Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
title_short Nanometer‐Scale 1D Negative Differential Resistance Channels in Van Der Waals Layers
title_sort nanometer scale 1d negative differential resistance channels in van der waals layers
topic 1T‐TaS2
density‐functional calculations
interlayer orbital overlap
negative differential resistance
scanning tunneling microscopy and spectroscopy
url https://doi.org/10.1002/advs.202408090
work_keys_str_mv AT qirongyao nanometerscale1dnegativedifferentialresistancechannelsinvanderwaalslayers
AT jaewhanpark nanometerscale1dnegativedifferentialresistancechannelsinvanderwaalslayers
AT choongjaewon nanometerscale1dnegativedifferentialresistancechannelsinvanderwaalslayers
AT sangwookcheong nanometerscale1dnegativedifferentialresistancechannelsinvanderwaalslayers
AT hanwoongyeom nanometerscale1dnegativedifferentialresistancechannelsinvanderwaalslayers