Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys

Pure and low-alloy zinc holds significant potential for use in biodegradable devices, such as coronary stents. However, its thermal stability has not yet been thoroughly characterized. This study focuses on the effect of magnesium addition on the mechanical and microstructural stability of zinc allo...

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Main Authors: Magdalena Gieleciak, Anna Jarzębska, Łukasz Maj, Paweł Petrzak, Mariusz Kulczyk, Łukasz Rogal, Magdalena Bieda
Format: Article
Language:English
Published: KeAi Communications Co., Ltd. 2025-02-01
Series:Bioactive Materials
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Online Access:http://www.sciencedirect.com/science/article/pii/S2452199X24004316
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author Magdalena Gieleciak
Anna Jarzębska
Łukasz Maj
Paweł Petrzak
Mariusz Kulczyk
Łukasz Rogal
Magdalena Bieda
author_facet Magdalena Gieleciak
Anna Jarzębska
Łukasz Maj
Paweł Petrzak
Mariusz Kulczyk
Łukasz Rogal
Magdalena Bieda
author_sort Magdalena Gieleciak
collection DOAJ
description Pure and low-alloy zinc holds significant potential for use in biodegradable devices, such as coronary stents. However, its thermal stability has not yet been thoroughly characterized. This study focuses on the effect of magnesium addition on the mechanical and microstructural stability of zinc alloys with 0.6 and 1.3 wt% Mg, subjected to hot extrusion and hydrostatic extrusion. Pure zinc was used as a reference material to provide a comprehensive comparison. Electron Backscatter Diffraction (EBSD) analysis revealed that the addition of magnesium enhanced thermal stability by forming intermetallic Mg2Zn11 phases, that hindered grain growth as compared with pure zinc. The Zn-0.6 Mg alloy exhibited faster static recrystallization compared to the Zn-1.3 Mg alloy, attributed to its lower initial average grain size and higher density of low-angle grain boundaries. These microstructural changes correlated with mechanical properties, as all materials showed increased strength after heating to 50 °C, which was attributed to dislocation annihilation and the formation of low-angle grain boundaries, as observed through transmission electron microscopy (TEM). Static compression tests demonstrated that the Zn-1.3 Mg alloy maintained a high compressive yield strength of ≈350 MPa, even after heating to 150 °C, highlighting its potential for safe future processing into stents.
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institution Kabale University
issn 2452-199X
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publisher KeAi Communications Co., Ltd.
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series Bioactive Materials
spelling doaj-art-39b18ebb0e70472c9930041f9cd3fa682024-12-14T06:31:38ZengKeAi Communications Co., Ltd.Bioactive Materials2452-199X2025-02-0144114Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloysMagdalena Gieleciak0Anna Jarzębska1Łukasz Maj2Paweł Petrzak3Mariusz Kulczyk4Łukasz Rogal5Magdalena Bieda6Institute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, PolandInstitute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, Poland; Corresponding author.Institute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, PolandInstitute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, PolandInstitute of High Pressure Physics, Polish Academy of Sciences, Warszawa, PolandInstitute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, PolandInstitute of Metallurgy and Materials Science, Polish Academy of Sciences, Reymonta 25, 30-059 Kraków, PolandPure and low-alloy zinc holds significant potential for use in biodegradable devices, such as coronary stents. However, its thermal stability has not yet been thoroughly characterized. This study focuses on the effect of magnesium addition on the mechanical and microstructural stability of zinc alloys with 0.6 and 1.3 wt% Mg, subjected to hot extrusion and hydrostatic extrusion. Pure zinc was used as a reference material to provide a comprehensive comparison. Electron Backscatter Diffraction (EBSD) analysis revealed that the addition of magnesium enhanced thermal stability by forming intermetallic Mg2Zn11 phases, that hindered grain growth as compared with pure zinc. The Zn-0.6 Mg alloy exhibited faster static recrystallization compared to the Zn-1.3 Mg alloy, attributed to its lower initial average grain size and higher density of low-angle grain boundaries. These microstructural changes correlated with mechanical properties, as all materials showed increased strength after heating to 50 °C, which was attributed to dislocation annihilation and the formation of low-angle grain boundaries, as observed through transmission electron microscopy (TEM). Static compression tests demonstrated that the Zn-1.3 Mg alloy maintained a high compressive yield strength of ≈350 MPa, even after heating to 150 °C, highlighting its potential for safe future processing into stents.http://www.sciencedirect.com/science/article/pii/S2452199X24004316Biodegradable metalsZincHydrostatic extrusionThermal stability
spellingShingle Magdalena Gieleciak
Anna Jarzębska
Łukasz Maj
Paweł Petrzak
Mariusz Kulczyk
Łukasz Rogal
Magdalena Bieda
Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
Bioactive Materials
Biodegradable metals
Zinc
Hydrostatic extrusion
Thermal stability
title Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
title_full Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
title_fullStr Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
title_full_unstemmed Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
title_short Influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
title_sort influence of magnesium addition on microstructural and mechanical stability of hydrostatically extruded biodegradable zinc alloys
topic Biodegradable metals
Zinc
Hydrostatic extrusion
Thermal stability
url http://www.sciencedirect.com/science/article/pii/S2452199X24004316
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