Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study

Colour is crucial for enhancing the appetizing value and consumer acceptance of food products. The commonly used food colourants and food preservatives such as Malachite Green (MG) and Copper Sulfate (CS) can cause severe health problems. This study investigates the toxicity of these food-grade colo...

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Main Authors: Haja Nazeer Ahamed, Ismail Y, Irfan Navabshan, Mohammed Zaidh S, Shanmugarajan TS, Ilham Jaleel, Thameemul Ansari LH
Format: Article
Language:English
Published: Elsevier 2024-12-01
Series:Toxicology Reports
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Online Access:http://www.sciencedirect.com/science/article/pii/S221475002400194X
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author Haja Nazeer Ahamed
Ismail Y
Irfan Navabshan
Mohammed Zaidh S
Shanmugarajan TS
Ilham Jaleel
Thameemul Ansari LH
author_facet Haja Nazeer Ahamed
Ismail Y
Irfan Navabshan
Mohammed Zaidh S
Shanmugarajan TS
Ilham Jaleel
Thameemul Ansari LH
author_sort Haja Nazeer Ahamed
collection DOAJ
description Colour is crucial for enhancing the appetizing value and consumer acceptance of food products. The commonly used food colourants and food preservatives such as Malachite Green (MG) and Copper Sulfate (CS) can cause severe health problems. This study investigates the toxicity of these food-grade colourants through acute exposure using in vivo cytotoxicity using the brine shrimp model including 3D surface analysis (3DSA) and in-silico studies Brine shrimp were treated with various concentrations of MG and CS. The cytotoxic effect was confirmed by brine shrimp lethality assay and 3DSA. Molecular docking and Molecular Dynamic simulation were done using hAChE binding cavity. Results showed that concentrations (2.5–10 µg/ml) of MG and CS significantly decreased locomotor behaviour within 1 h, while higher concentrations (10–100 µg/ml) caused high mortality rates. Morphological studies revealed that there is a significant reduction (p<0.05) in shrimp length treated with MG and CS. The 3DSA indicates that there is an inappropriate surface of the shrimp morphology. Interestingly, MG-treated shrimps had shown significant inhibition of AChE in homogenates, indicating cholinergic nerve-mediated toxicity. Computational studies showed MG confined active binding with human acetylcholinesterase (hAChE), with a binding energy MMGBSA of −51.3 kcal/mol. MD simulation confirmed reversible binding stability inside the hAChE pocket. It can be concluded that acute exposure to brine shrimps with MG and CS exhibited cytotoxicity as evidenced by the increase in mortality of the shrimps. This study further warrants the investigation of MG and CS residues from commonly used fruits and vegetables and their putative toxic effect using in-vivo studies.
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spelling doaj-art-366f18a9da6e436f935f95c7fc6499202024-12-19T10:54:53ZengElsevierToxicology Reports2214-75002024-12-0113101811Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational studyHaja Nazeer Ahamed0Ismail Y1Irfan Navabshan2Mohammed Zaidh S3Shanmugarajan TS4Ilham Jaleel5Thameemul Ansari LH6Crescent School of Pharmacy, B.S. Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, India; Correspondinga author at: Crescent School of Pharmacy, BS Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, India.Crescent School of Pharmacy, B.S. Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, IndiaCrescent School of Pharmacy, B.S. Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, IndiaCrescent School of Pharmacy, B.S. Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, IndiaProfessor and Head, Department of Pharmaceutics, School of Pharmaceutical Sciences, Vels Institute of Science, Technology &amp; Advanced Studies (VISTAS), Chennai, IndiaDepartment of Physiology, Panimalar Medical College Hospital &amp; Research Institute, Poonamallee, Chennai, IndiaCrescent School of Pharmacy, B.S. Abdur Rahman Crescent Institute of Science and Technology, Seethakathi Estate, GST Road, Vandalur, Chennai 600048, IndiaColour is crucial for enhancing the appetizing value and consumer acceptance of food products. The commonly used food colourants and food preservatives such as Malachite Green (MG) and Copper Sulfate (CS) can cause severe health problems. This study investigates the toxicity of these food-grade colourants through acute exposure using in vivo cytotoxicity using the brine shrimp model including 3D surface analysis (3DSA) and in-silico studies Brine shrimp were treated with various concentrations of MG and CS. The cytotoxic effect was confirmed by brine shrimp lethality assay and 3DSA. Molecular docking and Molecular Dynamic simulation were done using hAChE binding cavity. Results showed that concentrations (2.5–10 µg/ml) of MG and CS significantly decreased locomotor behaviour within 1 h, while higher concentrations (10–100 µg/ml) caused high mortality rates. Morphological studies revealed that there is a significant reduction (p<0.05) in shrimp length treated with MG and CS. The 3DSA indicates that there is an inappropriate surface of the shrimp morphology. Interestingly, MG-treated shrimps had shown significant inhibition of AChE in homogenates, indicating cholinergic nerve-mediated toxicity. Computational studies showed MG confined active binding with human acetylcholinesterase (hAChE), with a binding energy MMGBSA of −51.3 kcal/mol. MD simulation confirmed reversible binding stability inside the hAChE pocket. It can be concluded that acute exposure to brine shrimps with MG and CS exhibited cytotoxicity as evidenced by the increase in mortality of the shrimps. This study further warrants the investigation of MG and CS residues from commonly used fruits and vegetables and their putative toxic effect using in-vivo studies.http://www.sciencedirect.com/science/article/pii/S221475002400194XArtemia salinaMalachite Green (MG)Copper Sulphate (CS)3-Dimensional Surface Analysis (3DSA)Acetylcholinesterase (AChE)
spellingShingle Haja Nazeer Ahamed
Ismail Y
Irfan Navabshan
Mohammed Zaidh S
Shanmugarajan TS
Ilham Jaleel
Thameemul Ansari LH
Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
Toxicology Reports
Artemia salina
Malachite Green (MG)
Copper Sulphate (CS)
3-Dimensional Surface Analysis (3DSA)
Acetylcholinesterase (AChE)
title Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
title_full Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
title_fullStr Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
title_full_unstemmed Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
title_short Investigating the toxicity of malachite green and copper sulfate in brine shrimp: In-vivo and computational study
title_sort investigating the toxicity of malachite green and copper sulfate in brine shrimp in vivo and computational study
topic Artemia salina
Malachite Green (MG)
Copper Sulphate (CS)
3-Dimensional Surface Analysis (3DSA)
Acetylcholinesterase (AChE)
url http://www.sciencedirect.com/science/article/pii/S221475002400194X
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