Electrical generation of surface phonon polaritons

Efficient electrical generation of mid-infrared light is challenging because of the dearth of materials with natural dipole-active electronic transitions in this spectral region. One approach to solve this problem is through quantum-engineering of the electron dispersion to create artificial transit...

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Main Authors: Gubbin Christopher R., De Liberato Simone
Format: Article
Language:English
Published: De Gruyter 2023-05-01
Series:Nanophotonics
Subjects:
Online Access:https://doi.org/10.1515/nanoph-2022-0765
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author Gubbin Christopher R.
De Liberato Simone
author_facet Gubbin Christopher R.
De Liberato Simone
author_sort Gubbin Christopher R.
collection DOAJ
description Efficient electrical generation of mid-infrared light is challenging because of the dearth of materials with natural dipole-active electronic transitions in this spectral region. One approach to solve this problem is through quantum-engineering of the electron dispersion to create artificial transitions, as in quantum cascade devices. In this work we propose an alternative method to generate mid-infrared light, utilizing the coupling between longitudinal and transverse degrees of freedom due to the nonlocal optical response of nanoscopic polar dielectric crystals. Polar crystals support sub-diffraction photonic modes in the mid-infrared. They also support longitudinal phonons, which couple efficiently with electrical currents through the Fröhlich interaction. As we have shown in previous theoretical and experimental works, these two degrees of freedom can hybridize forming longitudinal-transverse polaritons. Here we theoretically demonstrate that longitudinal-transverse polaritons can be efficiently generated by electrical currents, leading to resonant narrowband photonic emission. This approach can therefore be utilised to electrically generate far-field mid-infrared photons in the absence of dipole-active electronic transitions, potentially underpinning a novel generation of mid-infrared optoelectronic devices.
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spelling doaj-art-33a11c3cd33e45e691a88c33d493da632024-11-25T11:19:09ZengDe GruyterNanophotonics2192-86062192-86142023-05-0112142849286410.1515/nanoph-2022-0765Electrical generation of surface phonon polaritonsGubbin Christopher R.0De Liberato Simone1School of Physics and Astronomy, University of Southampton, Southampton, SO17 1BJ, UKSchool of Physics and Astronomy, University of Southampton, Southampton, SO17 1BJ, UKEfficient electrical generation of mid-infrared light is challenging because of the dearth of materials with natural dipole-active electronic transitions in this spectral region. One approach to solve this problem is through quantum-engineering of the electron dispersion to create artificial transitions, as in quantum cascade devices. In this work we propose an alternative method to generate mid-infrared light, utilizing the coupling between longitudinal and transverse degrees of freedom due to the nonlocal optical response of nanoscopic polar dielectric crystals. Polar crystals support sub-diffraction photonic modes in the mid-infrared. They also support longitudinal phonons, which couple efficiently with electrical currents through the Fröhlich interaction. As we have shown in previous theoretical and experimental works, these two degrees of freedom can hybridize forming longitudinal-transverse polaritons. Here we theoretically demonstrate that longitudinal-transverse polaritons can be efficiently generated by electrical currents, leading to resonant narrowband photonic emission. This approach can therefore be utilised to electrically generate far-field mid-infrared photons in the absence of dipole-active electronic transitions, potentially underpinning a novel generation of mid-infrared optoelectronic devices.https://doi.org/10.1515/nanoph-2022-0765electroluminescencefröhlich interactionsurface phonon polaritons
spellingShingle Gubbin Christopher R.
De Liberato Simone
Electrical generation of surface phonon polaritons
Nanophotonics
electroluminescence
fröhlich interaction
surface phonon polaritons
title Electrical generation of surface phonon polaritons
title_full Electrical generation of surface phonon polaritons
title_fullStr Electrical generation of surface phonon polaritons
title_full_unstemmed Electrical generation of surface phonon polaritons
title_short Electrical generation of surface phonon polaritons
title_sort electrical generation of surface phonon polaritons
topic electroluminescence
fröhlich interaction
surface phonon polaritons
url https://doi.org/10.1515/nanoph-2022-0765
work_keys_str_mv AT gubbinchristopherr electricalgenerationofsurfacephononpolaritons
AT deliberatosimone electricalgenerationofsurfacephononpolaritons