Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering

Piezoelectric multilayer actuators (MLAs) possess unique advantages of lower driving voltages and more compact structures than bulk ceramic actuators. However, the internal electrode layers in MLAs inevitably weaken the output and result in relatively lower strain. The hysteresis property of piezoel...

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Main Authors: Yingchun Liu, Hongjun Zhang, Wenming Shi, Kai Li, Bin Yang, Wenwu Cao, Jiubin Tan
Format: Article
Language:English
Published: Elsevier 2025-03-01
Series:Journal of Materiomics
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Online Access:http://www.sciencedirect.com/science/article/pii/S2352847824001084
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author Yingchun Liu
Hongjun Zhang
Wenming Shi
Kai Li
Bin Yang
Wenwu Cao
Jiubin Tan
author_facet Yingchun Liu
Hongjun Zhang
Wenming Shi
Kai Li
Bin Yang
Wenwu Cao
Jiubin Tan
author_sort Yingchun Liu
collection DOAJ
description Piezoelectric multilayer actuators (MLAs) possess unique advantages of lower driving voltages and more compact structures than bulk ceramic actuators. However, the internal electrode layers in MLAs inevitably weaken the output and result in relatively lower strain. The hysteresis property of piezoelectric ceramics also significantly limits the positioning accuracy of MLAs. In this work, we adopted a synergistic strategy of crystallographic texturing and domain engineering in BaTiO3-based MLAs to enhance strains by improving piezoelectricity while simultaneously restraining the ultra-low hysteresis. We prepared [001]c-oriented (Ba0.95Ca0.05)(Ti0.94Zr0.055Sn0.005)O3 (BCTZS) ceramic layers in MLAs through the template grain growth (TGG) method with a texture degree of ∼95%. The textured BCTZS MLAs had a large displacement of 196 nm at 200 V (∼2.4 times that of randomly oriented ones) and achieved ultra-low strain hysteresis (Hs<9%). These almost identical displacement and strain hysteresis in textured MLAs before and after polarization at 200 V indicated better positioning repeatability under various voltage experiences. This finding can be attributed to easier domain switchings, because the high texture degree and the dominant “4O” domain configurations in textured grains accommodated the clamping stress, which decreased the domain wall energy but increased the domain flexibility.
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institution Kabale University
issn 2352-8478
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publishDate 2025-03-01
publisher Elsevier
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series Journal of Materiomics
spelling doaj-art-12b90f188c7846c5951a4ffdf4ccc22d2025-01-14T04:12:29ZengElsevierJournal of Materiomics2352-84782025-03-01112100882Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineeringYingchun Liu0Hongjun Zhang1Wenming Shi2Kai Li3Bin Yang4Wenwu Cao5Jiubin Tan6Functional Materials and Acoustooptic Instruments Institute, Harbin Institute of Technology, Harbin, 150080, ChinaFunctional Materials and Acoustooptic Instruments Institute, Harbin Institute of Technology, Harbin, 150080, China; Corresponding author.Functional Materials and Acoustooptic Instruments Institute, Harbin Institute of Technology, Harbin, 150080, ChinaGuangdong Provincial Key Laboratory of Electronic Functional Materials and Devices, Huizhou University, Huizhou, 516001, ChinaFunctional Materials and Acoustooptic Instruments Institute, Harbin Institute of Technology, Harbin, 150080, ChinaDepartment of Mathematics and Materials Research Institute, The Pennsylvania State University, University Park, PA, 16802, USAUltra-precision Optical &amp; Electronic Instrument Engineering Center, Harbin Institute of Technology, Harbin, 150001, ChinaPiezoelectric multilayer actuators (MLAs) possess unique advantages of lower driving voltages and more compact structures than bulk ceramic actuators. However, the internal electrode layers in MLAs inevitably weaken the output and result in relatively lower strain. The hysteresis property of piezoelectric ceramics also significantly limits the positioning accuracy of MLAs. In this work, we adopted a synergistic strategy of crystallographic texturing and domain engineering in BaTiO3-based MLAs to enhance strains by improving piezoelectricity while simultaneously restraining the ultra-low hysteresis. We prepared [001]c-oriented (Ba0.95Ca0.05)(Ti0.94Zr0.055Sn0.005)O3 (BCTZS) ceramic layers in MLAs through the template grain growth (TGG) method with a texture degree of ∼95%. The textured BCTZS MLAs had a large displacement of 196 nm at 200 V (∼2.4 times that of randomly oriented ones) and achieved ultra-low strain hysteresis (Hs<9%). These almost identical displacement and strain hysteresis in textured MLAs before and after polarization at 200 V indicated better positioning repeatability under various voltage experiences. This finding can be attributed to easier domain switchings, because the high texture degree and the dominant “4O” domain configurations in textured grains accommodated the clamping stress, which decreased the domain wall energy but increased the domain flexibility.http://www.sciencedirect.com/science/article/pii/S2352847824001084Piezoelectric multilayer actuatorsLead-freeTGGStrain hysteresis
spellingShingle Yingchun Liu
Hongjun Zhang
Wenming Shi
Kai Li
Bin Yang
Wenwu Cao
Jiubin Tan
Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
Journal of Materiomics
Piezoelectric multilayer actuators
Lead-free
TGG
Strain hysteresis
title Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
title_full Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
title_fullStr Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
title_full_unstemmed Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
title_short Ultra-low strain hysteresis in BaTiO3-based piezoelectric multilayer actuators via microstructural texture engineering
title_sort ultra low strain hysteresis in batio3 based piezoelectric multilayer actuators via microstructural texture engineering
topic Piezoelectric multilayer actuators
Lead-free
TGG
Strain hysteresis
url http://www.sciencedirect.com/science/article/pii/S2352847824001084
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