Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique

The kinetics of the thermal desorption of CO 2 adsorbed on zeolite 13X were obtained using a differential thermogravimetric analyser under two different carrier gas conditions. The varying heating rates were set as 8, 12, 16, and 20 K min −1 , respectively. The desorption activation energy of the ph...

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Main Authors: Yalou Guo, Hui Zhang, Yingshu Liu
Format: Article
Language:English
Published: SAGE Publishing 2018-10-01
Series:Adsorption Science & Technology
Online Access:https://doi.org/10.1177/0263617418772665
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author Yalou Guo
Hui Zhang
Yingshu Liu
author_facet Yalou Guo
Hui Zhang
Yingshu Liu
author_sort Yalou Guo
collection DOAJ
description The kinetics of the thermal desorption of CO 2 adsorbed on zeolite 13X were obtained using a differential thermogravimetric analyser under two different carrier gas conditions. The varying heating rates were set as 8, 12, 16, and 20 K min −1 , respectively. The desorption activation energy of the physisorption sites for this experiment evaluated by an integral method without prediction of the reaction order ranged from 12.15 to 14.12 kJ mol −1 (CO 2 as the carrier gas) and 43.32 to 50.42 kJ mol −1 (Ar as the carrier gas), respectively. The desorption activation energy of the chemisorption sites ranged from 57.95 to 58.53 kJ mol −1 (CO 2 as the carrier gas) and 74.02 to 79.92 kJ mol −1 (Ar as the carrier gas), respectively.
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institution Kabale University
issn 0263-6174
2048-4038
language English
publishDate 2018-10-01
publisher SAGE Publishing
record_format Article
series Adsorption Science & Technology
spelling doaj-art-0d6ac1e6400245abb850a68580fa673f2025-01-02T02:58:22ZengSAGE PublishingAdsorption Science & Technology0263-61742048-40382018-10-013610.1177/0263617418772665Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis techniqueYalou GuoHui ZhangYingshu LiuThe kinetics of the thermal desorption of CO 2 adsorbed on zeolite 13X were obtained using a differential thermogravimetric analyser under two different carrier gas conditions. The varying heating rates were set as 8, 12, 16, and 20 K min −1 , respectively. The desorption activation energy of the physisorption sites for this experiment evaluated by an integral method without prediction of the reaction order ranged from 12.15 to 14.12 kJ mol −1 (CO 2 as the carrier gas) and 43.32 to 50.42 kJ mol −1 (Ar as the carrier gas), respectively. The desorption activation energy of the chemisorption sites ranged from 57.95 to 58.53 kJ mol −1 (CO 2 as the carrier gas) and 74.02 to 79.92 kJ mol −1 (Ar as the carrier gas), respectively.https://doi.org/10.1177/0263617418772665
spellingShingle Yalou Guo
Hui Zhang
Yingshu Liu
Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
Adsorption Science & Technology
title Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
title_full Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
title_fullStr Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
title_full_unstemmed Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
title_short Desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis/differential thermogravimetric analysis technique
title_sort desorption characteristics and kinetic parameters determination of molecular sieve by thermogravimetric analysis differential thermogravimetric analysis technique
url https://doi.org/10.1177/0263617418772665
work_keys_str_mv AT yalouguo desorptioncharacteristicsandkineticparametersdeterminationofmolecularsievebythermogravimetricanalysisdifferentialthermogravimetricanalysistechnique
AT huizhang desorptioncharacteristicsandkineticparametersdeterminationofmolecularsievebythermogravimetricanalysisdifferentialthermogravimetricanalysistechnique
AT yingshuliu desorptioncharacteristicsandkineticparametersdeterminationofmolecularsievebythermogravimetricanalysisdifferentialthermogravimetricanalysistechnique